相关论文: LiYbSe2: Frustrated Magnetism in a New Pyrochlore …
The Yb based triangular lattice delafossites $A$Yb$X_2$ ($A$ = alkali metal, $X$ = O, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of CuYbSe$_2$ with a perfect…
Geometric frustration inhibits magnetic systems from ordering, opening a window to unconventional phases of matter. The paradigmatic frustrated lattice in three dimensions to host a spin liquid is the pyrochlore, although there remain few…
The triangular lattice compound TlYbS$_2$ was prepared as large single crystals via a molten flux growth technique using sodium chloride. Anisotropic magnetic susceptibility measurements down to 0.4 K indicate a complete absence of…
Square-lattice systems offer a direct route for realizing 2D quantum magnetism with frustration induced by competing interactions. In this work, the square-lattice materials YbBi2IO4 and YbBi2ClO4 were investigated using a combination of…
Our polycrystalline sample study on the Yb-based chalcogenide spinels $A$Yb$_2$$X_4$ ($A =$ Cd, Mg, $X =$ S, Se) has revealed frustrated magnetism due to the antiferromagnetically coupled Heisenberg spin on the pyrochlore lattice. Our…
The rich phase diagrams of magnetically frustrated pyrochlores have maintained a high level of interest over the past 20 years. To experimentally explore these phase diagrams requires a means of tuning the relevant interactions. One…
We have synthesized single crystals of Yb$_{2}$Pt$_{2}$Pb, which crystallize in the layered U$_{2}$Pt$_{2}$Sn-type structure, where planes of Yb ions lie on a triangular network. We report here the first results of magnetization, specific…
Pyrochlore lattices, which are found in two important classes of materials -- the $A_2B_2X_7$ pyrochlore family and the $AB_2X_4$ spinel family -- are the quintessential 3-dimensional frustrated lattice architecture. While historically…
Metastable Co$_2$Ti$_3$O$_8$ was synthesized through a topochemical reaction using Li$_2$CoTi$_3$O$_8$ as the precursor, resulting in a vacancy-ordered spinel structure. Crystal structure analysis confirmed that Co ions selectively occupy…
A triangular lattice selenide series of rare earth (RE), CsRESe2, were synthesized as large single crystals using a flux growth method. This series stabilized in either trigonal (R-3m) or hexagonal (P63/mmc) crystal systems. Physical…
The interplay between competing degrees of freedom can stabilize non-trivial magnetic states in correlated electron materials. Frustration-induced strong quantum fluctuations can evade long-range magnetic ordering leading to exotic quantum…
The discovery of new magnetic ground states in geometrically frustrated lattices remains a central challenge in materials science. Here, we report the synthesis, structural characterization, and frustrated magnetic properties of…
A unique type of frustrated lattice is found in two A-site ordered spinel oxides, LiGaCr4O8 and LiInCr4O8. Because of the large size mismatch between Li+ and Ga3+/In3+ ions at the A site, the pyrochlore lattice, made up of Cr3+ ions…
Quantum spin liquid (QSL) state in rare-earth triangular lattice has attracted much attention recently due to its potential application in quantum computing and communication. Here we report the single-crystal growth synthesis, crystal…
We synthesized a quasi-two-dimensional distorted triangular lattice antiferromagnet Ca$_3$CoNb$_2$O$_9$, in which the effective spin of Co$^{2+}$ is 1/2 at low temperatures, whose magnetic properties were studied by dc susceptibility and…
Quantum spin systems such as magnetic insulators usually show classical magnetic order, but such classical states can give way to quantum liquids with exotic entanglement through two known mechanisms of frustration: geometric frustration in…
Two-dimensional triangular-lattice materials with spin-1/2 are perfect platforms for investigating quantum frustrated physics with spin fluctuations. Here we report the structure, magnetization, heat capacity and inelastic neutron…
Quantum spin liquids~(QSLs) represent a unique quantum disordered state of matter that hosts long-range quantum entanglement and fractional excitations. However, structural disorder resulting from site mixing between different types of ions…
Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…
The delafossite-like compound NaYbO$_2$ hosts a triangular lattice of Yb$^{3+}$ moments and is a promising candidate for the realization of a quantum spin liquid ground state -- an exotic, quantum-disordered magnetic phase featuring…