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Pressure-induced phase transitions of spin-crossover materials were simulated by a Monte Carlo simulation in the constant pressure ensemble for the first time. Here, as the origin of the cooperative interaction, we adopt elastic interaction…

材料科学 · 物理学 2008-04-09 Yusuke Konishi , Hiroko Tokoro , Masamichi Nishino , Seiji Miyashita

We study the two-step spin crossover in a double-layered elastic model based on transition metal complexes each taking high spin (HS) and low spin (LS) states. Here, only the simplest elastic interactions between adjacent molecules are…

材料科学 · 物理学 2017-11-15 Daisuke Taniguchi , Jun Okabayashi , Chisa Hotta

Nuclear inelastic scattering (NIS) spectra were recorded for the spin-crossover complexes STP and ETP (STP = [Fe(1,1,1-trisf[N-(2-pyridylmethyl)-N-methylamino]methylg- ethane)](ClO4)2 and ETP =…

In spin crossover materials, an abrupt phase transition between a low spin state and a high spin state can be driven by temperature, pressure or by light irradiation. Of a special relevance are Fe(II) based coordination polymers where, in…

Hybrid perovskites have been at the forefront of condensed matter research particularly in context of device applications primarily in relation to applications in the field of solar cells. In this article, we demonstrate that several new…

材料科学 · 物理学 2022-04-04 Hrishit Banerjee , Angela Rittsteuer , Markus Aichhorn

Under the hydrostatic pressure $P=1.48$ GPa, polarized neutron elastic scattering experiments have been carried out on the coupled spin dimer system TlCuCl$_3$ with the gapped ground state at ambient pressure. Pressure-induced magnetic…

强关联电子 · 物理学 2009-11-10 A. Oosawa , K. Kakurai , T. Osakabe , M. Nakamura , M. Takeda , H. Tanaka

Magnetoresistance measurements on the quasi one-dimensional organic conductor (TMTSF)_2PF_6 performed in magnetic fields B up to 16T, temperatures T down to 0.12K and under pressures P up to 14kbar have revealed new phases on its P-B-T…

After the discovery of the phenomena of light-induced excited spin state trapping (LIESST), the functional properties of metal complexes have been studied intensively. Among them, cooperative phenomena involving low spin-high spin…

材料科学 · 物理学 2009-11-11 Kamel Boukheddaden , Masamichi Nishino , Seiji Miyashita , Francois Varret

Ab initio calculations predict a metal-insulator transition at zero temperature to occur in La$_4$Ni$_3$O$_8$ at moderate pressures as a result of a pressure-induced spin-state transition. The spin-state transition that is seen at 105 K at…

强关联电子 · 物理学 2015-05-28 Victor Pardo , Warren E. Pickett

Rapidly developing science and technology demand new materials with versatile and promising properties for practical applications. In this context, pseudo-octahedral iron(II) spin crossover (SCO) complexes are particularly appealing - not…

Photo-induced switching from the low-spin state to the high-spin state is studied in a model of spin-crossover materials, in which long-range interactions are induced by elastic distortions due to different molecular sizes the two spin…

A wide family of cobalt oxides of formulation (Pr,Ln,Ca)CoO3 (Ln being a lanthanide) exhibits a coupled valence and spin-state transition (VSST) at a temperature T*, which involves two concomitant modifications: (i) a change in the spin…

强关联电子 · 物理学 2015-06-15 V. Hardy , F. Guillou , Y. Bréard

In studies of the QCD deconfining phase transition or crossover by means of heavy ion experiments, one ought to be concerned about non-equilibrium effects due to heating and cooling of the system. Motivated by this, we look at hysteresis…

高能物理 - 格点 · 物理学 2009-11-10 Bernd A. Berg , Urs M. Heller , Hildegard Meyer-Ortmanns , Alexander Velytsky

A hybrid Potts model where a random concentration $p$ of the spins assume $q_0$ states and a random concentration $1-p$ of the spins assume $q>q_0$ states is introduced. It is known that when the system is homogeneous, with an integer spin…

统计力学 · 物理学 2022-05-03 Nir Schreiber , Reuven Cohen , Gideon Amir , Simi Haber

A gradual spin-state transition occurs in LaCoO3 around T~80-120 K, whose detailed nature remains controversial. We studied this transition by means of inelastic neutron scattering (INS), and found that with increasing temperature an…

强关联电子 · 物理学 2008-02-22 A. Podlesnyak , S. Streule , J. Mesot , M. Medarde , E. Pomjakushina , K. Conder , M. W. Haverkort , D. I. Khomskii

Spin-exchange collisions have been widely studied in recent years, and various quantum-mechanical scattering approaches have been developed to calculate the rates. However, these methods based on global knowledge of wavefunctions can be…

化学物理 · 物理学 2026-01-28 Debaarjun Mukherjee , Jeremy O. Richardson

Spin-crossover complexes exhibit two stable configurations with distinct spin states. The investigation of these molecules using low-temperature scanning tunneling microscopy has opened new perspectives for understanding the associated…

介观与纳米尺度物理 · 物理学 2026-01-05 Jonas Fußangel , Björn Sothmann , Sven Johannsen , Sascha Ossinger , Felix Tuczek , Richard Berndt , Jürgen König , Manuel Gruber

We investigate the spin-squeezing behavior under thermal effects in a one-dimensional transverse field XY model with spin-1/2. The exact solution of the model helps us to compute the spin-squeezing parameter as a function of temperature and…

量子物理 · 物理学 2024-12-09 Saeed Mahdavifar , Hadi Cheraghi , Kourosh Afrousheh

We analyze pressure effects on stripe states within a selfconsistent Hartree-Fock calculation for a model of a striped nickelates. The results show a transition induced by high pressure and predict possible new spin states. We describe…

强关联电子 · 物理学 2009-11-13 E. Kaneshita , A. R. Bishop

We discuss the phenomenology of phase transitions studied with two control variables. Such measurements have become routine with magnetic field and temperature being varied for 1st order magnetic transitions with an ease not conceivable…

材料科学 · 物理学 2014-03-26 P Chaddah
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