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Stoichiometric materials of Eu(III) offer a promising platform for quantum memories attributable to their unique capability to display a distinctive, nondegenerate J = 0 transition, which enables precise mapping of optical quantum states…

We use molecular dynamics simulations with machine-learned atomistic force fields to simulate photoexcitation of BaTiO3 by a femtosecond laser pulse whose photon energy exceeds the optical gap. We demonstrate selective displacive excitation…

材料科学 · 物理学 2024-07-30 Fangyuan Gu , Paul Tangney

The electrical transport properties of graphene are greatly influenced by its environment. Owing to its high dielectric constant, strontium titanate (STO) is expected to suppress the long-range charged impurity scattering and consequently…

介观与纳米尺度物理 · 物理学 2014-12-04 Ray Sachs , Zhisheng Lin , Jing Shi

We investigate spin dynamics in the antiferromagnetic (AFM) multiferroic TbMnO3 using optical- pump, terahertz (THz)-probe spectroscopy. Photoexcitation results in a broadband THz transmission change, with an onset time of 25 ps at 6 K that…

In the endeavour of developing quantum memories, Er$^{3+}$:CaWO$_4$ has emerged as a promising rare-earth ion-doped (REID) crystal platform due to its long optical coherence times and compatibility with the 1550 nm telecommunications band.…

Micrometric domains of precise ferroelectric polarization have been written into a 20 nm thick epitaxial thin film of BaTiO3(001) (BTO) on a Nb doped SrTiO3 (STO) substrate using PiezoForce Microscopy (PFM). The domain dependent electronic…

材料科学 · 物理学 2018-06-06 N. Barrett , J. Rault , I. Krug , B. Vilquin , G. Niu , B. Gautier , D. Albertini , O. Renault

Spintronic terahertz (THz) emitters (STE) based on the inverse spin Hall effect in ferromagnetic/heavy metal (FM/HM) heterostructures have become important sources for THz pulse generation. The design, materials and control of these…

Recent experiments in the original cuprate high temperature superconductor, La$_2-x$Ba$_x$CuO$_4$, have revealed a remarkable sequence of transitions [1]. Here we investigate such crystals with Kerr effect which is sensitive to…

超导电性 · 物理学 2012-10-10 Hovnatan Karapetyan , M. Hucker , G. D. Gu , J. M. Tranquada , M. M. Fejer , Jing Xia , A. Kapitulnik

We study ultrafast magneto-photocurrents in a three-dimensional topological insulator. For this purpose, we excite (In$_r$Bi$_{1-r}$)$_2$Se$_3$ thin films with a femtosecond laser pulse in the presence of an external magnetic field…

介观与纳米尺度物理 · 物理学 2026-01-06 Chihun In , Genaro Bierhance , Deepti Jain , Tom S. Seifert , Oliver Gueckstock , Roberto Mantovan , Seongshik Oh , Tobias Kampfrath

We investigate the persistent orientation of asymmetric-top molecules induced by time-delayed THz pulses that are either collinearly or cross polarized. Our theoretical and numerical results demonstrate that the orthogonal configuration…

化学物理 · 物理学 2023-12-05 Long Xu , Ilia Tutunnikov , Yehiam Prior , Ilya Sh. Averbukh

Intense, single-cycle terahertz (THz) pulses offer a promising approach for understanding and controlling the properties of a material on an ultrafast time scale. In particular, resonantly exciting phonons leads to a better understanding of…

Terahertz (THz) generation by optical rectification in LiNbO$_3$ (LN) is a widely used technique for generating intense THz radiation. The spatiotemporal characterization of THz pulses from these sources is currently limited to far-field…

Despite its simple structure and low degree of electronic correlation, SrTiO$_3$ (STO) features collective phenomena linked to charge transport and, ultimately, superconductivity, that are not yet fully explained. Thus, a better insight in…

We investigated domain kinetics by measuring the polarization switching behaviors of polycrystalline Pb(Zr,Ti)O$_{3}$ films, which are widely used in ferroelectric memory devices. Their switching behaviors at various electric fields and…

材料科学 · 物理学 2009-11-13 J. Y. Jo , H. S. Han , J. -G. Yoon , T. K. Song , S. -H. Kim , T. W. Noh

The temperature-dependent polarization of SrTiO_3 thin films is investigated using confocal scanning optical microscopy. A homogeneous out-of-plane and inhomogeneous in-plane ferroelectric phase are identified from images of the linear…

材料科学 · 物理学 2009-11-07 Oleg Tikhomirov , Hua Jiang , Jeremy Levy

Full pattern Le-Bail refinement using x-ray powder diffraction profiles of Sr1-xCaxTiO3 for x=0.02, 0.04 in the temperature range 12 to 300 K reveals anomalies in the unit cell parameters at 170, 225 K due to an antiferrodistortive (cubic…

材料科学 · 物理学 2015-05-13 Sanjay Kumar Mishra , Dhananjai Pandey

Coherent radiation with frequencies ranging from 0.3 to 30 THz has recently become accessible by femtosecond laser technology. Terahertz (THz) waves have already found many applications in spectroscopy and imaging, and they can be…

The speed of magnetization reversal is a key feature in magnetic data storage. Magnetic fields from intense THz pulses have been recently shown to induce small magnetization dynamics in Cobalt thin film on the sub-picosecond time scale.…

光学 · 物理学 2016-02-17 Mostafa Shalaby , Carlo Vicario , Christoph P. Hauri

Ferroelectric materials embedded with dielectric inclusions offer a unique platform for exploring novel topological polar textures. Using first-principles-based atomistic simulations, we investigate the polarization behavior of a BaTiO$_3$…

材料科学 · 物理学 2026-03-12 R. Machado , F. Di Rino , M. Sepliarsky , M. G. Stachiotti

Breaking the memory wall in advanced computing architectures will require complex 3D integration of emerging memory materials such as ferroelectrics-either within the back-end-of-line (BEOL) of CMOS front-end processes or through advanced…