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We present a novel derivation of resonant inelastic x-ray scattering (RIXS) which yields an expression for the RIXS cross section in terms of emission pathways between intermediate and final many-body states. Thereby electron-hole…

材料科学 · 物理学 2020-10-14 Christian Vorwerk , Francesco Sottile , Claudia Draxl

We develop a formalism for calculating resonant inelastic x-ray scattering (RIXS) spectra in systems of itinerant electrons with arbitrary band structures, accounting for the effect of the positively-charged core hole exactly. We apply this…

超导电性 · 物理学 2013-12-24 David Benjamin , Israel Klich , Eugene Demler

We develop a formalism to study the Resonant Inelastic X-ray Scattering (RIXS) response in metals based on the diagrammatic expansion for its cross section. The standard approach to the solution of the RIXS problem relies on two key…

强关联电子 · 物理学 2019-11-20 A. M. Tsvelik , R. M. Konik , N. V. Prokof'ev , I. S. Tupitsyn

We investigate theoretically the resonant inelastic x-ray scattering (RIXS) at the $K$ edge of Si on the basis of an ab initio calculation. We calculate the RIXS spectra with systematically varying transfered-momenta, incident-photon energy…

材料科学 · 物理学 2007-05-23 Yunori Nisikawa , Manabu Usuda , Jun-ichi Igarashi

We present a computational study of $L$-edge resonant inelastic x-ray scattering (RIXS) in correlated 3$d$ transition-metal oxides using an $ab$ $initio$ method based on local density approximation + dynamical mean-field theory (DMFT). The…

强关联电子 · 物理学 2020-03-25 Atsushi Hariki , Mathias Winder , Takayuki Uozumi , Jan Kuneš

We present a detailed analysis of resonant inelastic scattering (RIXS) from Fe$_{1.087}$Te with unprecedented energy resolution. In contrast to the sharp peaks typically seen in insulating systems at the transition metal $L_3$ edge, we…

We present an ab initio study of neutral core and valence electronic excitations in {\alpha}-Al2O3 by solving the Bethe-Salpeter equation (BSE) of many-body perturbation theory within an all-electron framework. Calculated spectra at the Al…

材料科学 · 物理学 2024-01-26 M. Laura Urquiza , Matteo Gatti , Francesco Sottile

We study the resonant inelastic x-ray scattering (RIXS) at the $K$ edge of Ge. We measure RIXS spectra with systematically varying momenta in the final state. The spectra are a measure of exciting an electron-hole pair. We find a single…

材料科学 · 物理学 2007-05-23 Yunori Nisikawa , Manabu Usuda , Jun-ichi Igarashi , Hironobu Shoji , Toshiaki Iwazumi

We develop a theory of resonant inelastic x-ray scattering (RIXS) at the $K$ edge in La$_2$CuO$_4$ on the basis of the Keldysh Green's function formalism. In our previous analysis (Phys. Rev. B 71, 035110 (2005)), the scattering by the…

强关联电子 · 物理学 2015-06-25 Jun-ichi Igarashi , Takuji Nomura , Manabu Takahashi

We present a theory of the resonant inelastic x-ray scattering (RIXS) to study electronic excitations in orbital ordered manganites. The charge and orbital excitations of the Mn 3d electron are caused by the Coulomb interactions in the…

强关联电子 · 物理学 2009-10-31 H. Kondo , S. Ishihara , S. Maekawa

In the past decade, Resonant Inelastic X-ray Scattering (RIXS) has made remarkable progress as a spectroscopic technique. This is a direct result of the availability of high-brilliance synchrotron X-ray radiation sources and of advanced…

The study of elementary bosonic excitations is essential toward a complete description of quantum electronic solids. In this context, resonant inelastic X-ray scattering (RIXS) has recently risen to becoming a versatile probe of electronic…

We investigate resonant inelastic X-ray scattering (RIXS) at the O $K$-edge in insulating cuprates by means of three methods: cluster perturbation theory (CPT), Hartree--Fock approximation (HFA) and exact diagonalization (ED) method. We…

强关联电子 · 物理学 2023-02-22 Yukihiro Matsubayashi , Sumio Ishihara

Resonant inelastic X-ray scattering (RIXS) spectra of model copper- and nickel-based transition metal oxides are measured over a wide range of energies near the M-edge (h$\nu$=60-80eV) to better understand the properties of resonant…

强关联电子 · 物理学 2012-11-20 L. Andrew Wray , Wanli Yang , Hiroshi Eisaki , Zahid Hussain , Yi-De Chuang

Core hole resonance is used in X-ray spectroscopy to incisively probe the local electronic states of many-body systems. Here, resonant inelastic X-ray scattering (RIXS) is studied as a function of incident photon energy on Mott insulators…

Using a model Hamiltonian, we discuss how we could interpret data obtained from transition metal $K$-edge resonant inelastic x-ray scattering (RIXS) experiments. By analyzing the creation of valence excitations from the screening of the…

材料科学 · 物理学 2008-08-08 K. H. Ahn , A. J. Fedro , Michel van Veenendaal

In indirect resonant inelastic X-ray scattering (RIXS) an intermediate state is created with a core-hole that has a ultrashort lifetime. The core-hole potential therefore acts as a femtosecond pulse on the valence electrons. We show that…

强关联电子 · 物理学 2009-11-11 Luuk J. P. Ament , Filomena Forte , Jeroen van den Brink

The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic x-ray scattering (RIXS) at the forefront of photon science. Here we develop the scattering theory for RIXS…

超导电性 · 物理学 2015-04-10 Pasquale Marra , Steffen Sykora , Krzysztof Wohlfeld , Jeroen van den Brink

Resonant inelastic x-ray scattering (RIXS) is a spectroscopic technique which has been widely used to study various elementary excitations in correlated and other condensed matter systems. For strongly correlated materials, besides boosting…

强关联电子 · 物理学 2012-12-27 C. J. Jia , C. -C. Chen , A. P. Sorini , B. Moritz , T. P. Devereaux

Resonant Inelastic X-ray Scattering (RIXS) in the soft x-ray range is an element-specific energy-loss spectroscopy used to probe the electronic and magnetic excitations in strongly correlated solids. In the recent years, RIXS has been…

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