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Light-induced states are commonly observed in the photoionization spectra of laser-dressed atoms. The properties of autoionizing polaritons, entangled states of light and Auger resonances, however, are largely unexplored. We employ…

原子物理 · 物理学 2021-07-14 Nathan Harkema , Coleman Cariker , Eva Lindroth , Luca Argenti , Arvinder Sandhu

In this work, we irradiate a superconducting artificial molecule composed of two coupled tunable transmons with microwave light while monitoring its state via joint dispersive readout. Performing high-power spectroscopy, we observe and…

We study the photoionization of argon atoms close to the 3s$^2$3p$^6$ $\rightarrow$ 3s$^1$3p$^6$4p $\leftrightarrow$ 3s$^2$3p$^5$ $\varepsilon \ell$, $\ell$=s,d Fano window resonance. An interferometric technique using an attosecond pulse…

Excitons in a monolayer transition metal dichalcogenide (1L-TMD) are highly bound states characterized by a Rydberg-like spectrum of discrete energy levels. Among these, states with odd-parity are known as dark excitons due to selection…

Molecular polaritons are hybrid states of photonic and molecular character that form when molecules strongly interact with light. Strong coupling tunes energy levels and importantly, can modify molecular properties (e.g. photoreaction…

化学物理 · 物理学 2023-02-14 Francesca Fassioli , Kyu Hyung Park , Sarah E. Bard , Gregory D. Scholes

We study the nonlinear optical response of argon to a four-wave-mixing pulse sequence consisting of an extreme ultraviolet pulse, an overlapping collinear IR and an non-collinear delayed IR pulses. Absorption of an extreme ultraviolet and…

原子物理 · 物理学 2024-12-03 Sergio Yanez-Pagans , Nathan Harkema , Arvinder Sandhu , Coleman Cariker , Luca Argenti

Controlling light-matter based quantum systems in the strong coupling regime allows for exploring quantum simulation of many-body physics in nowadays architectures. For instance, the atom-field interaction in a cavity QED network provides…

量子物理 · 物理学 2021-05-26 Diego Tancara , Ariel Norambuena , Rubén Peña , Guillermo Romero , Felipe Torres , Raúl Coto

Intense laser pulses have the capability to couple resonances in the continuum, leading to the formation of a split pair of autoionizing polaritons. These polaritons can exhibit extended lifetimes due to interference between radiative and…

Strong light-matter coupling to form exciton- and vibropolaritons is increasingly touted as a powerful tool to alter the fundamental properties of organic materials. It is proposed that these states and their facile tunability can be used…

Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…

Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details…

Exciton polaritons, arising from the interaction of electronic transitions with confined electromagnetic fields, have emerged as a powerful tool to manipulate the properties of organic materials. However, standard experimental and…

Formation of dressed light-matter states in optical structures, manifested as Rabi splitting of the eigen energies of a coupled system, is one of the key effects in quantum optics. In pursuing this regime with semiconductors, light is…

Resonance-enhanced multiphoton ionization (REMPI) in potassium atom is investigated within the strong coupling regime using photoelectron momentum imaging techniques. The kinetic energy distribution of the ionized electrons reveals the…

原子物理 · 物理学 2025-03-10 Wankai Li , Yixuan Wang , Xing Li , Tao Yang , Dongdong Zhang , Dajun Ding

Exciton-polaritons are quasiparticles with mixed photon and exciton character that demonstrate rich quantum phenomena, novel optoelectronic devices and the potential to modify chemical properties of materials. Organic semiconductors are of…

The possibility for controlling the probe-field optical gain and absorption switching and photon conversion by a surface-plasmon-polariton near field is explored for a quantum dot above the surface of a metal. In contrast to the linear…

介观与纳米尺度物理 · 物理学 2023-07-19 Danhong Huang , Michelle Easter , Godfrey Gumbs , A. A. Maradudin , Shawn-Yu Lin , Dave Cardimona , Xiang Zhang

We study ultrafast ionization dynamics using orthogonally polarized two-color (OTC) laser pulses involving the resonant "first plus second" ($\omega+2\omega$) scheme. The scheme is illustrated by numerical simulations of the time-dependent…

原子物理 · 物理学 2019-12-16 Hicham Agueny

Strong light-matter coupling gives rise to polaritons - hybrid excitations whose mixed photonic and matter character enables control over optical, electronic and chemical properties. This Feature Article surveys the main architectures…

Features of complex vector light become important in any interference effects, including scattering, diffraction, and non-linear processes. Here we are investigating the role of polarization-structured light in atomic state interferometers.…

原子物理 · 物理学 2025-10-24 Kuntal Samanta , Sphinx J. Svensson , Sonja Franke-Arnold , Niclas Westerberg

Polaritonic chemistry investigates the possible modification of chemical and photochemical reactions by means of strong light-matter coupling in optical cavities, as demonstrated in numerous experiments over the last few years. These…

量子物理 · 物理学 2025-07-30 Lucas Borges , Thomas Schnappinger , Markus Kowalewski
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