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The process of photosynthesis, the main source of energy in the animate world, converts sunlight into chemical energy. The surprisingly high efficiency of this process is believed to be enabled by an intricate interplay between the quantum…

In recent years, Born-Markov master equations based on tracing out the electromagnetic degrees of freedom have been extensively employed in the description of quantum optical phenomena originating from photon-mediated interactions in…

Artificially reproducing the biological light reactions responsible for the remarkably efficient photon-to-charge conversion in photosynthetic complexes represents a new direction for the future development of photovoltaic devices. Here, we…

量子物理 · 物理学 2013-12-25 C. Creatore , M. A. Parker , S. Emmott , A. W. Chin

Near-unity energy transfer efficiency has been widely observed in natural photosynthetic complexes. This phenomenon has attracted broad interest from different fields, such as physics, biology, chemistry and material science, as it may…

We investigate the influence of electron-phonon interactions on the dynamical properties of a quantum-dot-cavity QED system. We show that non-Markovian effects in the phonon reservoir lead to strong changes in the dynamics, arising from…

介观与纳米尺度物理 · 物理学 2010-04-29 P. Kaer , T. R. Nielsen , P. Lodahl , A. -P. Jauho , J. Mork

Multi-photon processes are the essence of nonlinear optics. Optical harmonics generation and multi-photon absorption, ionization, polymerization or spectroscopy are widely used in practical applications. Generally, the rate of an n-photon…

We propose a dynamic mechanism for the reversible regulation of photosynthesis in varying light environments. We employ a three-level quantum model to take into account the correlations between charge donors and charge acceptors immediately…

生物物理 · 物理学 2024-11-13 Guang Yang , Gen Tatara

In this paper we investigate non-Markovian evolution of a two-level system (qubit) in a bosonic bath under influence of an external classical fluctuating environment. The interaction with the bath has the Lorentzian spectral density, and…

量子物理 · 物理学 2020-07-03 V. A. Mikhailov , N. V. Troshkin

Photosynthesis is a biological process that involves the highly-efficient transport of energy captured from the sun to a reaction center, where conversion into useful biochemical energy takes place. Even though one can always use a quantum…

生物物理 · 物理学 2013-06-07 R. de J. León-Montiel , Juan P. Torres

We model the quantum electron transfer (ET) in the photosynthetic reaction center (RC), using a non-Hermitian Hamiltonian approach. Our model includes (i) two protein cofactors, donor and acceptor, with discrete energy levels and (ii) a…

量子物理 · 物理学 2012-11-16 Alexander I. Nesterov , Gennady P. Berman , Alan R. Bishop

The Fano effect arises from the interference between a continuum of propagating modes and a localised resonance. By using this resonance as one of the mirrors in an optical cavity, a localised mode with a highly asymmetric line shape is…

量子物理 · 物理学 2019-12-18 Emil V Denning , Jake Iles-Smith , Jesper Mork

In this paper, we present a theoretical description to the quantum coherence and decoherence phenomena of energy transfer in photosynthesis observed in a recent experiment [see Science 316, 1462 (2007)]. As a successive two-color laser…

量子物理 · 物理学 2010-01-28 Xian-Ting Liang , Wei-Min Zhang , Yi-Zhong Zhuo

Quantum non-Markovianity modifies the environmental decoherence of a system. This situation is enriched in complex systems owing to interactions among subsystems. We consider the problem of distinguishing the multiple sources of…

量子物理 · 物理学 2021-03-03 Subhashish Banerjee , Javid Naikoo , R. Srikanth

In this paper we present a Markovian representation approach to constructing quantum filters for a class of non-Markovian quantum systems disturbed by Lorenztian noise. An ancillary system is introduced to convert white noise into…

量子物理 · 物理学 2017-02-20 Shibei Xue , Matthew R. James , Alireza Shabani , Valery Ugrinovskii , Ian R. Petersen

Non-Markovian effects in the evolution of open quantum systems have recently attracted widespread interest, particularly in the context of assessing the efficiency of energy and charge transfer in nanoscale biomolecular networks and quantum…

化学物理 · 物理学 2016-02-10 S. Oviedo-Casado , J. Prior , A. W. Chin , R. Rosenbach , S. F. Huelga , M. B. Plenio

The illumination of catalytic surfaces with a continuous or pulsed stream of photons dynamically modulates surface chemistry for faster rates, higher conversion, or product selectivity control. To establish fundamental principles of dynamic…

化学物理 · 物理学 2025-11-24 Paul J Dauenhauer

In this paper, a quantum filter for estimating the states of a non-Markovian qubit system is presented in an augmented Markovian system framework including both the qubit system of interest and multi-ancillary systems for representing the…

量子物理 · 物理学 2017-02-20 Shibei Xue , Matthew R. James , Alireza Shabani , Valery Ugrinovskii , Ian R. Petersen

We investigate the quantum dynamics of energy and charge transfer in a wheel-shaped artificial photosynthetic antenna-reaction center complex.This complex consists of six light-harvesting chromophores and an electron-acceptor fullerene. To…

生物物理 · 物理学 2015-05-28 Pulak Kumar Ghosh , Anatoly Yu. Smirnov , Franco Nori

The quantum dynamics of entanglement is widely revealed in photosynthetic light-harvesting complexes. Different from the previous work, we explore the properties of exciton transport and photosynthesis assisted by the quantum entanglement…

应用物理 · 物理学 2024-03-12 Lu-Xin Xu , Shun-Cai Zhao , Ling-Fang Li

Phonon interactions are inevitable in cavity quantum electrodynamical systems based on solid-state emitters or fluorescent molecules, where vibrations of the lattice or chemical bonds couple to the electronic degrees of freedom. Due to the…

量子物理 · 物理学 2021-06-16 Matias Bundgaard-Nielsen , Jesper Mørk , Emil Vosmar Denning