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Magnetic excitations in van der Waals (vdW) materials, especially in the two-dimensional (2D) limit, are an exciting research topic from both the fundamental and applied perspectives. Using temperature-dependent, magneto-Raman spectroscopy,…

The recently discovered two-dimensional (2D) van der Waals magnet NiPS$_3$ provides a new route to examine many-body quasiparticles under 2D confinement. Excitons are of particular interest due to their strong coupling to the magnetic…

强关联电子 · 物理学 2022-10-07 Christopher Lane , Jian-Xin Zhu

We combine polarized infrared magneto-transmission and Faraday angle rotation measurements to map the collective excitations of the van der Waals antiferromagnet FePS$_3$. Below the N\'{e}el temperature ($T_\mathrm{N} \approx 118$ K), the…

强关联电子 · 物理学 2025-08-21 Kartik Panda , Itzik Kapon , Dumitru Dumcenco , Dirk van der Marel , Alexey Kuzmenko , Nimrod Bachar

Two-dimensional van der Waals (vdW) ferromagnets drive the advancement in spintronic applications and enable the exploration of exotic magnetism in low-dimensional systems. The entanglement of dual $-$ localized and itinerant $-$ nature of…

The ability to assemble layers of two-dimensional (2D) materials to form permutations of van der Waals heterostructures provides significant opportunities in materials design and synthesis. Interlayer interactions provide a path to new…

介观与纳米尺度物理 · 物理学 2023-01-09 Zachariah Hennighausen , Jisoo Moon , Kathleen M. McCreary , Connie H. Li , Olaf M. J. van `t Erve , Berend T. Jonker

The Raman scattering response of the biaxial antiferromagnet CoPS$_3$ has been investigated as a function of both magnetic field and temperature. The peaks observed in the low-frequency spectral range (90--200~cm$^{-1}$) have been…

The phenomena of pronounced electron-electron and electron-phonon interactions in one-dimensional (1D) systems are ubiquitous, which are well described by frameworks of Luttinger liquid, Peierls instability and concomitant charge density…

介观与纳米尺度物理 · 物理学 2025-04-01 Shaoqi Sun , Qingyun Lin , Yihuan Li , Daichi Kozawa , Huizhen Wu , Shigeo Maruyama , Pilkyung Moon , Toshikaze Kariyado , Ryo Kitaura , Sihan Zhao

The hybridization of magnons (spin waves) with phonons, if sufficiently strong and comprising long wavelength excitations, may offer a new playground when manipulating the magnetically ordered systems with light. Applying a magnetic field…

NiPS3 is a Van der Waals antiferromagnet that has been found to display spin-charge and spin-phonon coupling in its antiferromagnetically ordered state below TN = 155 K. Here, we study high-quality crystals of site-diluted Ni1-xZnxPS3 (0 <…

The emergence of a long-range magnetic order in the atomically thin, two-dimensional (2D) limit has long remained a fundamental question in condensed matter physics. The advent of exfoliable van der Waals (vdW) materials, particularly…

材料科学 · 物理学 2026-03-03 Rahul Kumar , Je-Geun Park

We present a fully analytical model of hybridization between magnon, and phonons observed experimentally in magneto-Raman scattering in van der Waals (vdW) antiferromagnets (AFM). Here, the representative material, FePS3, has been shown to…

介观与纳米尺度物理 · 物理学 2025-01-03 Somsubhra Ghosh , Mainak Palit , Sujan Maity , Subhadeep Datta

Interlayer van der Waals (vdW) coupling is generic in two-dimensional materials such as graphene and transition metal dichalcogenides, which can induce very low-energy phonon modes. Using high-resolution inelastic hard x-ray scattering, we…

This study presents a comprehensive analysis of the band structure in NiPS$_3$, a van der Waals layered antiferromagnet, utilizing high-resolution synchrotron-based angle-resolved photoemission spectroscopy (ARPES) and corroborative density…

Strong coupling between light and elementary excitations is emerging as a powerful tool to engineer the properties of solid-state systems. Spin-correlated excitations that couple strongly to optical cavities promise control over collective…

Two-dimensional (2D) van der Waals (vdW) magnets with spin-phonon coupling are crucial for next-generation spintronics. Among them, Fe3GaTe2 has attracted widespread attention due to above-room-temperature intrinsic ferromagnetism and large…

材料科学 · 物理学 2024-12-02 Gaojie Zhang , Hao Wu , Li Yang , Wen Jin , Bichen Xiao , Wenfeng Zhang , Haixin Chang

Magnetoelastic coupling in van der Waals (vdW) magnetic materials enables a unique interplay between the spin and lattice degrees of freedom. Characterizing the elastic responses with atomic and femtosecond resolution across the magnetic…

Van der Waals magnets are uniquely positioned at the intersection between two-dimensional materials, antiferromagnetic spintronics, and magnonics. The interlayer exchange interaction in these materials enables antiferromagnetic resonances…

材料科学 · 物理学 2021-04-14 Joseph Sklenar , Wei Zhang

The control of antiferromagnets with ultrashort optical pulses has emerged as a prominent field of research. Tailored laser excitation can launch coherent spin waves at terahertz frequencies, yet a comprehensive description of their…

Excitonic states of tightly-bound electron-hole pairs dominate the optical response in a growing class of two-dimensional (2D) materials and their van der Waals (vdW) heterostructures. In transition metal dichalcogenides (TMDs) a useful…

介观与纳米尺度物理 · 物理学 2025-10-17 Jiayu David Cao , Konstantin S. Denisov , Igor Zutic

Strong interactions between different degrees of freedom lead to exotic phases of matter with complex order parameters and emergent collective excitations. Conventional techniques, such as scattering and transport, probe the amplitudes of…

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