相关论文: Spectroscopy of high pressure rubidium-noble gas m…
Optical spectroscopy of atoms and molecules is a field where one usually operates very far from thermal equilibrium conditions. A prominent example is spectroscopy of thin vapors, where the pump irradiation leads to a non equilibrium…
We describe experiments on the laser cooling of both helium-rubidium and argon-rubidium gas mixtures by collisional redistribution of radiation. Frequent alkali-noble gas collisions in the ultradense gas, with typically 200\,bar of noble…
Accurate absorption models for gases at high pressure and temperature support advanced optical combustion diagnostics and aid in the study of harsh planetary atmospheres. Developing and validating absorption models for these applications…
We describe measurements demonstrating laser cooling of an atomic gas by means of collisional redistribution of radiation. The experiment uses rubidium atoms in the presence of several hundred bar of argon buffer gas pressure. Frequent…
We have recorded fluorescence spectra of the atomic rubidium D-lines in the presence of several hundreds of bars buffer gas pressure. With additional saturation broadening a spectral linewidth comparable to the thermal energy of the atoms…
We study laser cooling of atomic gases by collisional redistribution of fluorescence. In a high pressure buffer gas regime, frequent collisions perturb the energy levels of alkali atoms, which allows for the absorption of a far red detuned…
Laser spectroscopy of hot atomic vapours has been studied extensively. Theoretical models that predict the absolute value of the electric susceptibility are crucial for optimising the design of photonic devices that use hot vapours, and for…
Nonlinear selective reflection from the interface YAG window-high density rubidium vapor in the high-temperature cell is studied at the transition 5S$_{1/2}$-5P$_{3/2}$. In the experiment tunable pump and probe lasers are used. The…
We describe the design of a soldered sapphire optical viewport, useful for spectroscopic applications of samples at high temperatures and high pressures. The sapphire window is bonded via active soldering to a metal flange with a structure…
We report a combined experimental and theoretical investigation of near resonance light scattering from a high-density and ultracold atomic $^{87}$Rb gas. The atomic sample, having a peak density $\sim 5\cdot10^{13}$ atoms/cm$^{3}$,…
The degree of thermalization of electronically excited state manifolds of an absorber can be tested via optical spectroscopy. In the thermalized-manifold case, the ratio of absorption and emission is expected to follow a universal…
We have extended the range of the high-pressure optical spectroscopy to the far-infrared region keeping the accuracy of ambient-pressure experiments. The newly-developed method offers a powerful tool for the study of pressure-induced phase…
High-resolution absorption spectra of \NH\ in the region 2100 - 5500 \cm\ at 1027 $^{\circ}$C and atmospheric pressure (1045 $\pm$ 3 mbar) are measured. An \NH\ concentration of 10\% in volume fraction is used in the measurements. Spectra…
A glass ultrahigh vacuum chamber with rubidium alkali metal dispensers and non-evaporable getter pumps has been developed and used to create a cold atomic sample in a chamber that operates with only passive vacuum pumps. The ion-mass…
We have demonstrated a high temperature vapor cell for absorption spectroscopy on the Ca intercombination line. The cell uses a dual chamber design to achieve the high temperatures necessary for an optically dense vapor while avoiding the…
We study laser cooling of atomic gases by collisional redistribution, a technique applicable to ultradense atomic ensembles at a pressure of a few hundred bar. Frequent collisions of an optically active atom with a buffer gas shift atoms…
Molecules with heavy, radioactive nuclei promise extreme sensitivity to fundamental nuclear and particle physics. However, these nuclei are available in limited quantities, which challenges their use in precision measurements. Here we…
Between the absorption and the emission spectral lineshapes of dense atomic and molecular media, such as dye solutions and alkali-noble buffer gas mixtures at high pressure, in many cases there exists a universal scaling, the…
To understand the optical properties of atoms in solid state matrices, the absorption, excitation and emission spectra of rubidium doped thin-films of argon, krypton and xenon were investigated in detail. A two-dimensional spectral analysis…
Currently, there is great interest in laser cooling of barium monofluoride (BaF) molecules for precision tests of fundamental symmetries. We use high-resolution absorption spectroscopy to characterize several as yet imprecisely known…