相关论文: Probing phonon dynamics with multi-dimensional hig…
Using sub-picosecond optical pump-probe techniques, coherent zone-folded longitudinal acoustic phonons (ZFLAPs) were generated and controlled in an InGaN multiple quantum well structure. A one-pump, one-probe differential transmission…
High-order harmonic generation (HHG) in gases has been studied for almost 40 years in many different conditions, varying the laser wavelength, intensity, focusing geometry, target design, gas species, etc. However, no systematic…
The detection of electron motion and electronic wavepacket dynamics is one of the core goals of attosecond science. Recently, choosing the nitric oxide (NO) molecule as an example, we have introduced and demonstrated a new experimental…
Attosecond pulse trains (APTs) are indispensable for probing electron dynamics at their intrinsic timescales. High harmonic generation (HHG) has long been a successful and widely used technique in producing extreme ultraviolet APTs. While…
The interpretation of high-harmonic generation (HHG) in solids typically relies on phenomenological dephasing times far shorter than what is expected from microscopic scattering processes. Here we show that zero-point fluctuations…
We theoretically investigate high-harmonic generation (HHG) in honeycomb-lattice graphene models when subjected to a DC electric field. By integrating the quantum master equation with the Boltzmann equation, we develop a numerical method to…
We tailor the shape and phase of the pump pulse spectrum in order to study the coherent lattice dynamics in tellurium. Employing the coherent control via splitting the pump pulse into a two-pulse sequence, we show that the oscillations due…
High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…
High harmonic generation (HHG) is an extreme nonlinear process where intense pulses of light drive matter to emit high harmonics of the driving frequency, reaching the extreme ultraviolet (XUV) and x-ray spectral ranges. So far, the HHG…
We propose a theoretical framework for the detection of order parameter fluctuations in three dimensions using ultrafast coherent phonon spectroscopy. We focus our attention on long wavelength charge density fluctuations (plasmons), and…
For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high…
We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…
Non-perturbative and phase-sensitive light-matter interactions have led to the generation of attosecond pulses of light and the control electrical currents on the same timescale. Traditionally, probing these effects via high harmonic…
High-harmonic generation (HHG) in strongly correlated Mott insulators is investigated using exact diagonalization and time-dependent density-matrix propagation of a laser-driven one-dimensional Hubbard chain. By projecting onto equilibrium…
We have performed ultrafast pump-probe spectroscopy studies on a series of InAs/GaSb-based short-period superlattice (SL) samples with periods ranging from 46 \AA to 71 \AA. We observe two types of oscillations in the differential…
High-harmonic generation (HHG) in solids is an emerging method to probe ultrafast electron dynamics in solids at attosecond timescale. In this work, we study HHG from monolayer and bilayer graphene. Bilayer graphenes with AA and AB stacking…
Transient reflectivity spectroscopy is widely used to study ultrafast carrier- and phonon-dynamics in semiconductors. In their heterostructures, it is often not straightforward to distinguish contributions to the signal from the various…
High-harmonic generation (HHG) of a two-level-system driven by an intense monochromatic phase-locked laser is studied in terms of complex spectral analysis with the Floquet method. In contrast to the phenomenological approaches, this…
We have examined the effect of pump-probe photon energy on the amplitude of coherent optical phonons in a prototypical phase change material using a femtosecond time-resolved transmission technique. The photon energy was varied between 0.8…
High-order harmonic generation (HHG) in solids is profoundly influenced by the dephasing of the coherent electron-hole motion driven by an external laser field. The exact physical mechanisms underlying this dephasing, crucial for accurately…