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Many reports on stimulated Raman scattering in mixtures of Raman-active and noble gases indicate that the addition of a dispersive buffer gas increases the phase-mismatch to higher-order Stokes and antiStokes sidebands, resulting in…

光学 · 物理学 2017-12-27 Pooria Hosseini , David Novoa , Amir Abdolvand , Philip St. J. Russell

While Si clathrates have been explored as promising direct bandgap semiconductors, their practical optoelectronic performance has been limited by high doping levels and structural defects. Hydrogen has long been used to improve the…

Like single perovskites, halide double perovskites (HDP) have truly emerged as efficient optoelectronic materials since they display superior stability and are free of toxicity. However, challenges still exist due to either wide and…

材料科学 · 物理学 2023-09-13 Mayank Gupta , Susmita Jana , B. R. K. Nanda

Raman scattering is a ubiquitous phenomenon in light-matter interactions which reveals a material's electronic, structural and thermal properties. Controlling this process would enable new ways of studying and manipulating fundamental…

We report high-pressure photoluminescence, Raman scattering, and x-ray diffraction measurements on a lead-free halide perovskite $Cs_3Sb_2Br_9$. At about 3 GPa, an electronic transition manifests itself through a broad minimum in linewidth,…

Dimensionality engineering in A$_{n+1}$B$_n$X$_{3n+1}$ Ruddlesden-Popper (RP) perovskite phases has emerged as a promising strategy to enhance optoelectronic properties. These properties are highly material-dependent, requiring detailed…

材料科学 · 物理学 2025-03-04 Surajit Adhikari , Aksaj Bharatwaj , Priya Johari

The optical properties of the two-dimensional (2D) crystals are dominated by tightly bound electron-hole pairs (excitons) and lattice vibration modes (phonons). The exciton-phonon interaction is fundamentally important to understand the…

材料科学 · 物理学 2021-02-09 Qing-Hai Tan , Yu-Jia Sun , Xue-Lu Liu , Yanyuan Zhao , Qihua Xiong , Ping-Heng Tan , Jun Zhang

The application of ultrathin two-dimensional (2D) perovskites in near-infrared and visible-range optoelectronics has been limited owing to their inherent wide bandgaps, large excitonic binding energies and low optical absorption at higher…

介观与纳米尺度物理 · 物理学 2022-05-06 Abin Varghese , Yuefeng Yin , Mingchao Wang , Saurabh Lodha , Nikhil V. Medhekar

Metal-halide perovskites are a versatile material platform for light-harvesting and light-emitting applications as their variable chemical composition allows the optoelectronic properties to be tailored to specific applications. Halide…

Raman spectroscopy plays a key role in studies of graphene and related carbon systems. Graphene is perhaps the most promising material of recent times for many novel applications, including electronics. In this paper, the traditional and…

材料科学 · 物理学 2015-12-07 Eric J. Heller , Yuan Yang , Lucas Kocia , Wei Chen , Shiang Fang , Mario Borunda , Efthimios Kaxiras

Natural van der Waals (vdW) crystals with hyperbolic dispersion challenge artificial metamaterials but remain confined to the mid-infrared spectrum. The emergence of MoOCl2, a quasi-one-dimensional metal with in-plane hyperbolicity,…

Optically active defects often play a crucial role in governing the light emission as well as the electronic properties of materials. Moreover, defect-mediated states in the mid-gap region can trap electrons, thus opening a path for the…

材料科学 · 物理学 2025-01-03 Aprajita Joshi , Sajid Saikia , Shalini Badola , Angshuman Nag , Surajit Saha

Hydrogen detection is of great importance in chemical and energy industries. Optical fiber hydrogen sensors show flexibility and compactness and have the potential for distributed analysis. However, traditional fiber sensors encounter a…

光学 · 物理学 2019-05-16 F. Yang , Y. Zhao , Y. Qi , Y. Z. Tan , H. L. Ho , W. Jin

Halide perovskites are promising materials for light-emitting and light-harvesting applications. In this context, two-dimensional perovskites such as nanoplatelets or Ruddlesden-Popper and Dion-Jacobson layered structures are important…

应用物理 · 物理学 2021-10-25 Sushant Ghimire , Christian Klinke

We report an investigation of perovskite-type SmScO3 and NdScO3 single crystals by Raman scattering in various scattering configurations and at different wavelengths. The reported Raman spectra, together with the phonon mode assignment, set…

材料科学 · 物理学 2011-05-09 O. Chaix-Pluchery , J. Kreisel

Two-dimensional (2D) van der Waals nanomaterials have attracted considerable attention for potential use in photonic and optoelectronic applications in the nanoscale, due to their outstanding electrical and optical properties, differing…

We demonstrate a machine learning (ML) approach that accurately predicts the current-voltage behavior of 3D/2D-structured (FAMA)Pb(IBr)3/OABr hybrid organic-inorganic halide perovskite (HOIP) solar cells under AM1.5 illumination. Our neural…

Surface phonon polaritons (SPhPs) in polar dielectrics offer new opportunities for infrared nanophotonics due to sub-diffraction confinement with low optical losses. Though the polaritonic field confinement can be significantly improved by…

Molecular optomechanics stems from the description of Raman scattering in the presence of an optical resonator using a cavity optomechanics formalism. We extend the molecular optomechanics formalism to the case of hybrid…

The excellent optoelectronic properties, straightforward synthesis, and robust material stability of quasi-2D metal halide perovskites have made them a hot research topic for optoelectronic devices. In layered organic-inorganic perovskites,…

材料科学 · 物理学 2025-10-31 Brindhu Malani S , Eugen Klein , Rostyslav Lesyuk , Christian Klinke