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Nature is remarkably adept at using interfaces to build structures, encapsulate reagents, and regulate biological processes. Inspired by Nature, we describe flexible polymer-based ribbons, termed "mesoscale polymers" (MSPs), to modulate…

软凝聚态物质 · 物理学 2021-08-23 Dylan M. Barber , Zhefei Yang , Lucas Prevost , Olivia du Roure , Anke Lindner , Todd Emrick , Alfred J. Crosby

We present a theoretical description of the dynamics of a semi-flexible polymer being pulled through a nanopore by an external force acting at the pore. Our theory is based on the tensile blob picture of Pincus in which the front of the…

统计力学 · 物理学 2015-09-16 Pui-Man Lam , Yi Zhen

Advances in DNA nanotechnology have stimulated the search for simple motifs that can be used to control the properties of DNA nanostructures. One such motif, which has been used extensively in structures such as polyhedral cages,…

软凝聚态物质 · 物理学 2015-06-10 John S. Schreck , Thomas E. Ouldridge , Flavio Romano , Ard A. Louis , Jonathan P. K. Doye

Dynamics of spreading of small droplets on surfaces has been studied by the molecular dynamics method. Simulations have been performed for mixtures of solvent and dimer, and solvent and tetramer droplets. For solvent particles and dimers,…

凝聚态物理 · 物理学 2009-10-22 J. A. Nieminen , T. Ala- Nissila

Our study aims at a better control and understanding of the transfer of a complex [DNA supercoiled plasmid - dodecyltrimethylammonium surfactant] layer from a liquid-vapour water interface onto a silicon surface without any additional…

化学物理 · 物理学 2008-01-18 Frédérique Battin-Leclerc , A. A. Konnov , J. L. Jaffrezo , M. Legrand

Active polymers play a central role in many biological systems, from bacterial flagella to cellular cytoskeletons. Minimal models of semiflexible active filaments have been used to study a variety of interesting phenomena in active systems,…

软凝聚态物质 · 物理学 2020-02-19 Matthew S. E. Peterson , Michael F. Hagan , Aparna Baskaran

Extended depth of field microscopy encodes axial information into a single acquisition through engineered point spread functions, but conventional and deep optics approaches are subject to degradation in scattering tissue. We introduce…

We investigate diffusion-limited reactions between a diffusing particle and a target site on a semiflexible polymer, a key factor determining the kinetics of DNA-protein binding and polymerization of cytoskeletal filaments. Our theory…

软凝聚态物质 · 物理学 2010-12-08 Yann von Hansen , Roland R. Netz , Michael Hinczewski

We use a mesoscale simulation approach to explore the impact of different capsid geometries on the packaging and ejection dynamics of polymers of different flexibility. We find that both packing and ejection times are faster for flexible…

软凝聚态物质 · 物理学 2009-11-11 I. Ali , D. Marenduzzo , J. M. Yeomans

Two-dimensional simulations are used to explore topological transitions that occur during the formation of films grown from grains that are seeded on substrates. This is done for a relatively large range of the initial value $\Phi_s$ of the…

材料科学 · 物理学 2022-01-21 Stoffel D. Janssens , David Vázquez-Cortés , Eliot Fried

This review summarizes recent progress in investigating polymer systems by using Differential dynamic microscopy (DDM), a rapidly emerging approach that transforms a commercial microscope by combining real-space information with the…

软凝聚态物质 · 物理学 2021-06-07 Roberto Cerbino , Fabio Giavazzi , Matthew E. Helgeson

What can cells gain by using disordered, rather than folded, proteins in the architecture of their skeleton? Disordered proteins take multiple co-existing conformations, and often contain segments which act as random-walk-shaped polymers.…

软凝聚态物质 · 物理学 2016-10-05 Micha Kornreich , Eti Malka-Gibor , Ben Zuker , Adi Laser-Azogui , Roy Beck

Grafting polymer chains on nanoparticles surfaces is a well-known route to control their self assembly and distribution in a polymer matrix. A wide variety of self assembled structures are achieved by changing the grafting patterns on an…

材料科学 · 物理学 2022-07-19 Sachin Gautham , Tarak Patra

The influence of surface constraints on the self-assembly of liquid droplets is investigated. A semi-quantitative explanation for large scale pattern formation consisting of small scale closely arranged droplets inside the large scale…

软凝聚态物质 · 物理学 2019-06-28 K Nilavarasi , S G Ramkumar , V Madhurima

The necking instability is a precursor to tensile failure and rupture of materials. A quasistatically loaded free-standing uniaxial specimen typically exhibits necking at a single location, corresponding to a long wavelength bifurcation…

软凝聚态物质 · 物理学 2023-01-04 Jian Li , Hannah Varner , Tal Cohen

Single-filament tracing has been a valuable tool to directly determine geometrical and mechanical properties of entangled polymer networks. However, systematically verifying how the stiffness of the tracer filament or its molecular…

软凝聚态物质 · 物理学 2022-01-05 Tina Händler , Cary Tutmarc , Martin Glaser , Jessica S. Freitag , David M. Smith , Jörg Schnauß

Photonic crystals -- a class of materials whose optical properties derive from their structure in addition to their composition -- can be created by self-assembling particles whose sizes are comparable to the wavelengths of visible light.…

软凝聚态物质 · 物理学 2023-08-02 Alexander Hensley , Thomas E. Videbaek , Hunter Seyforth , William M. Jacobs , W. Benjamin Rogers

Molecular dynamics simulations are used to study the spreading of binary polymer nanodroplets in a cylindrical geometry. The polymers, described by the bead-spring model, spread on a flat surface with a surface-coupled Langevin thermostat…

软凝聚态物质 · 物理学 2007-05-23 David R. Heine , Gary S. Grest , Edmund B. Webb

The mechanics of animal cells is strongly determined by stress fibers, which are contractile filament bundles that form dynamically in response to extracellular cues. Stress fibers allow the cell to adapt its mechanics to environmental…

Elastic MicroPhase Separation (EMPS) provides a simple route to create soft materials with homogeneous microstructures by leveraging the supersaturation of crosslinked polymer networks with liquids. At low supersaturation, network…