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We present a structural analysis of the substituted system (Ba$_{1-x}$Sr$_{x}$)CuSi$_{2}$O$_{6}$, which reveals a stable tetragonal crystal structure down to 1.5 K. We explore the structural details with lowtemperature neutron and…

The standard approach to realize a spin liquid state is through magnetically frustrated states, relying on ingredients such as the lattice geometry, dimensionality, and magnetic interaction type of the spins. While Heisenberg spins on a…

强关联电子 · 物理学 2025-04-10 Margarita G. Dronova , Vaclav Petricek , Zachary Morgan , Feng Ye , Daniel M. Silevitch , Yejun Feng

Neutron scattering studies on a single crystal of the highly-correlated electron system, La1-xSrxMnO3 with x~0.3, have been carried out elucidating both the spin and lattice dynamics of this metallic ferromagnet. We report a large measured…

凝聚态物理 · 物理学 2009-10-28 Michael C. Martin , G. Shirane , Y. Endoh , K. Hirota , Y. Moritomo , Y. Tokura

We explore orbital dynamics in the spin liquid candidate Ba3CuSb2O9 using multi-frequency electron spin resonance. We prepared two high quality single crystals. The crystal with a slight copper deficiency shows a structural phase transition…

强关联电子 · 物理学 2015-12-09 Yibo Han , Masayuki Hagiwara , Takehito Nakano , Yasuo Nozue , Kenta Kimura , Mario Halim , Satoru Nakatsuji

We study geometrically frustrated antiferromagnets with magnetoelastic coupling. Frustration in these systems may be relieved by a structural transition to a low temperature phase with reduced lattice symmetry. We examine the statistical…

强关联电子 · 物理学 2008-06-30 Timothy E. Saunders , John T. Chalker

Structural properties of the spin chain and ladder compound Sr$_{14}$Cu$_{24}$O$_{41}$ have been studied using diffraction with hard x-rays. Strong incommensurate modulation reflections are observed due to the lattice mismatch of the chain…

强关联电子 · 物理学 2007-05-23 M. v. Zimmermann , J. Geck , S. Kiele , R. Klingeler , B. Büchner

We use variable-temperature x-ray thermal diffuse scattering and inelastic scattering to investigate the lattice dynamics in single crystals of multiferroic CaMn7O12 which undergo a series of orbital and magnetic transitions at low…

强关联电子 · 物理学 2016-11-24 S. M. Souliou , Y. Li , X. Du , M. Le Tacon , A. Bosak

The lack of inversion symmetry in the crystal lattice of magnetic materials gives rise to complex non-collinear spin orders through interactions of relativistic nature, resulting in interesting physical phenomena, such as emergent…

Noncollinear magnetic structures and multiple magnetic phase transitions in a sawtooth lattice antiferromagnet consisting of Cr$^{3+}$ are experimentally identified in this work, thereby proposing the scenario of magnetism-driven…

The mixed spinel, MgFe2O4 has been synthesized by ball-milling assisted sintering method. X-ray diffraction study confirms formation of cubic MgFe2O4 and the lattice parameter values calculated are a = b = c = 8.369(3) {\AA}. Vibrating…

材料科学 · 物理学 2018-10-01 B. Santhosh Kumar , N. Praveen Shankar , N. Aparna devi , C. Venkateswaran

We report the synthesis, and structural and physical properties of CaFe4As3 single crystals. Needle-like single crystals of CaFe4As3 were grown out of Sn flux and the compound adopts an orthorhombic structure as determined by X-ray…

超导电性 · 物理学 2015-05-27 A. B. Karki , G. T. McCandless , S. Stadler , Y. M. Xiong , J. Li , Julia Y. Chan , R. Jin

We report the path from the charge density wave (CDW)-bearing superconductor CuIr2Te4 to the metal insulator transition (MIT)-bearing compound CuIr2S4 by chemical alloying with the gradual substitution of S for Te. The evolution of…

Using elastic and inelastic neutron scattering we show that a cubic spinel, CdCr$_2$O$_4$, undergoes an elongation along the c-axis ($c > a = b$) at its spin-Peierls-like phase transition at $T_N$ = 7.8 K. The N\'{e}el phase ($T < T_N$) has…

强关联电子 · 物理学 2009-11-11 J. -H. Chung , M. Matsuda , S. -H. Lee , K. Kakurai , H. Ueda , T. J. Sato , H. Takagi , K. -P. Hong , S. Park

The structural and magnetic phase transitions of the ternary iron arsenides SrFe2As2 and EuFe2As2 were studied by temperature-dependent x-ray powder diffraction and 57-Fe Moessbauer spectroscopy. Both compounds crystallize in the tetragonal…

The magnetic and lattice properties of the $S$=1/2 quantum-spin-chain ferromagnet, CuAs$_2$O$_4$, mineral name trippkeite, were investigated. The crystal structure of CuAs$_2$O$_4$ is characterized by the presence of corrugated CuO$_2$…

材料科学 · 物理学 2015-06-18 K. Caslin , R. K. Kremer , F. S. Razavi , A. Schulz , A. Muñoz , F. Pertlik , J. Liu , M. -H. Whangbo , J. M. Law

We present an extensive powder and single-crystal neutron scattering investigation of the crystallographic structure and magnetic order of the frustrated metallic $f$-electron magnet UNi$_4$B. We carry out a full refinement of the…

Calcium vanadate CaV$_2$O$_4$ has a crystal structure of quasi-one-dimensional zigzag chains composed of orbital-active V$^{3+}$ ions and undergoes successive structural and antiferromagnetic phase transitions at $T_s\sim 140$ K and $T_N…

强关联电子 · 物理学 2020-06-17 T. Watanabe , S. Kobayashi , Y. Hara , J. Xu , B. Lake , J. -Q. Yan , A. Niazi , D. C. Johnston

Plate-like single crystals of SrFe2As2 as large as 3x3x0.5 mm3 have been grown out of Sn flux. The SrFe2As2 single crystals show a structural phase transition from a high temperature tetragonal phase to a low temperature orthorhombic phase…

The fluorine-doped rare-earth iron oxyarsenides, REFeAsO1-xFx (RE =rare earth) have recently emerged as a new family of high-temperature superconductors with transition temperatures (Tc) as high as 55 K (refs 1-4). Early work has provided…

GeCo$_2$O$_4$ is a unique system in the family of cobalt spinels ACo$_2$O$_4$ (A= Sn, Ti, Ru, Mn, Al, Zn, Fe, etc.) in which magnetic Co ions stabilize on the pyrochlore lattice exhibiting a large degree of orbital frustration. Due to the…