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BaCo$_2$(AsO$_4$)$_2$ (BCAO), a honeycomb cobaltate, is considered a promising candidate for materials displaying the Kitaev quantum spin liquid state. This assumption is based on the distinctive characteristics of Co$^{2+}$ ions (3$d^7$)…

The insulating honeycomb magnet $\alpha$-RuCl$_{3}$ exhibits fractionalized excitiations that signal its proximity to a Kitaev quantum spin liquid (QSL) state, however, at $T=0$, fragile long-range magnetic order arises from non-Kitaev…

$\alpha$-RuCl$_{3}$ is a major candidate for the realization of the Kitaev quantum spin liquid, but its zigzag antiferromagnetic order at low temperatures indicates deviations from the Kitaev model. We have quantified the spin Hamiltonian…

Co-based honeycomb magnets have been actively studied recently for the potential realization of emergent quantum magnetism therein such as the Kitaev spin liquid. Here we employ density functional and dynamical mean-field theory methods to…

强关联电子 · 物理学 2025-08-11 Subhasis Samanta , Fabrizio Cossu , Heung-Sik Kim

Inelastic neutron scattering experiments with a large set of comounted Na$_2$IrO$_3$ crystals reveal the low-energy magnon dispersion in this candidate material for Kitaev physics. The magnon gap amounts to 1.7(1) meV and can be interpreted…

In this study, we reanalyze the magnetic interactions in the Kitaev spin liquid candidate materials Na$_2$IrO$_3$, $\alpha$-RuCl$_3$, and $\alpha$-Li$_2$IrO$_3$ using nonperturbative exact diagonalization methods. These methods are more…

强关联电子 · 物理学 2016-07-06 Stephen M. Winter , Ying Li , Harald O. Jeschke , Roser Valenti

In the search for realizations of Quantum Spin Liquids (QSL), it is essential to understand the interplay between inherent disorder and the correlated fluctuating spin ground state. H$_3$LiIr$_2$O$_6$ is regarded as a spin liquid proximate…

强关联电子 · 物理学 2024-07-11 A. de la Torre , B. Zager , F. Bahrami , M. H. Upton , J. Kim , G. Fabbris , G. -H. Lee , W. Yang , D. Haskel , F. Tafti , K. W. Plumb

Most of the searches for Kitaev materials deal with $4d/5d$ magnets with spin-orbit-coupled ${J=1/2}$ local moments such as iridates and $\alpha$-RuCl$_3$. Here we propose the monoclinic YbCl$_3$ with a Yb$^{3+}$ honeycomb lattice for the…

The magnetic orders in Na$_2$IrO$_3$ and $\alpha-$RuCl$_3$, honeycomb systems with strong spin-orbit coupling and correlations, have been recently described by models with the dominant Kitaev interactions. In this work we discuss how the…

强关联电子 · 物理学 2017-02-10 Yuriy Sizyuk , Peter Woelfle , Natalia B. Perkins

The magnetism in Mn$_3$Si$_2$Te$_6$ has been investigated using thermodynamic measurements, first principles calculations, neutron diffraction and diffuse neutron scattering on single crystals. These data confirm that Mn$_3$Si$_2$Te$_6$ is…

The structural and magnetic properties of a new series of iridium-based honeycomb lattices with the formula Na3-delta(Na1-xMgx)Ir2O6 (x = 0 to 1) are reported. As x and delta are increased, the honeycomb lattice contracts and the strength…

强关联电子 · 物理学 2014-04-18 D. C. Wallace , C. M. Brown , T. M. McQueen

We performed inelastic neutron scattering experiments on Cu$_2$$^{114}$Cd$^{11}$B$_2$O$_6$ powder. The magnetic excitations at low temperatures are similar to those of the interacting spin-1/2 tetramers in the ordered state. The weak…

Kitaev quantum spin liquids (KSLs) in layered honeycomb magnets are known to host Majorana quasiparticles, whose excitations depend strongly on the direction of the applied magnetic field. In the high-field phase of $\alpha$-RuCl$_3$,…

We study the phonon behavior of a Co-based honeycomb frustrated magnet Na$_2$Co$_2$TeO$_6$ under magnetic field applied perpendicular to the honeycomb plane. The temperature and field dependence of the sound velocity and sound attenuation…

We report on band structure calculations and a microscopic model of the low-dimensional magnet beta-Cu2V2O7. Magnetic properties of this compound can be described by a spin-1/2 anisotropic honeycomb lattice model with the averaged coupling…

强关联电子 · 物理学 2010-10-12 Alexander A. Tsirlin , Oleg Janson , Helge Rosner

We discuss magnetically ordered states, arising in Heisenberg-Kitaev and related spin models, on three-dimensional (3D) harmonic honeycomb lattices. For large classes of ordered states, we show that they can be mapped onto two-dimensional…

强关联电子 · 物理学 2020-01-29 Wilhelm G. F. Krüger , Matthias Vojta , Lukas Janssen

The honeycomb antiferromagnet BaCo2(AsO4)2, in which small in-plane magnetic fields (H1 = 0.26 T and H2 = 0.52 T at T = 1.8 K < TN = 5.4 K) induce two magnetic phase transitions, has attracted attention as a possible candidate material for…

Kitaev materials often order magnetically at low temperatures due to the presence of non-Kitaev interactions. Torque magnetometry is a very sensitive technique for probing the magnetic anisotropy, which is critical in understanding the…

Through a combination of crystal symmetry analysis and density functional theory calculations we unveil a possible microscopic origin of the unexpected insulating behavior reported in the honeycomb Kitaev material Cu$_2$IrO$_3$. Our study…

强关联电子 · 物理学 2024-12-03 Ying Li , Roger D. Johnson , Yogesh Singh , Radu Coldea , Roser Valentí

We report a muon spin rotation/relaxation ($\mu$SR) study of single-crystalline samples of the $\alpha$-RuCl$_3$ honeycomb magnet, which is presumed to be a model compound for the Kitaev-Heisenberg interaction. It is inferred from magnetic…