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Coulomb bound electron-hole pairs, excitons, govern the optical properties of semi-conducting transition metal dichalcogenides like MoS$_2$ and WSe$_2$. We study optical transitions at the K-point for 2H homobilayer MoS$_2$ in Density…

We investigate the strong coupling between the excitons and quasi-bound states in the continuum (BIC) resonance in a bulk WS$_2$ metasurface. Here we employ the bulk WS$_2$ to construct an ultrathin nanodisk metasurface, supporting the…

Polariton-based devices require materials where light-matter coupling under ambient conditions exceeds losses, but our current selection of such materials is limited. Here we measured the dispersion of polaritons formed by the $A$ and $B$…

材料科学 · 物理学 2021-06-16 Patryk Kusch , Niclas S. Mueller , Martin T. Hartmann , Stephanie Reich

Hybrid systems of excitons strongly coupled to localized surface plasmons supported by metallic nanoparticles define a new approach to control light-matter interactions. Here, we report exciton-plasmon coupling in two-dimensional (2D)…

The two-dimensional transition-metal dichalcogenides (2D TMDCs) are an intriguing platform for studying light-matter interactions because they combine the electronic properties of conventional semiconductors with the optical resonances…

介观与纳米尺度物理 · 物理学 2022-05-02 Aaron H. Rose , Taylor J. Aubry , Hanyu Zhang , Jao van de Lagemaat

Enhancing the light-matter interactions in two-dimensional materials via optical metasurfaces has attracted much attention due to its potential to enable breakthrough in advanced compact photonic and quantum information devices. Here, we…

Nanoscale light-matter interaction in the weak-coupling regime has been achieved with unique hyperbolic metamaterial modes possessing a high density of states. Here, we show strong coupling between intersubband transitions (ISBTs) of a…

光学 · 物理学 2014-08-01 Prashant Shekhar , Zubin Jacob

Excitons are vital in the photophysics of materials, especially in low-dimensional systems. The conceptual and quantitative understanding of excitonic effects in nonlinear optical (NLO) processes is more challenging compared to linear ones.…

材料科学 · 物理学 2026-02-26 Jiawei Ruan , Y. -H. Chan , Steven G. Louie

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

Monolayer (ML) transition metal dichalcogenides (TMDs) integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter coupling regime. Analogous concepts for hybrid light-matter systems employing…

Strong interactions between surface plasmons in ultra-compact nanocavities and excitons in two dimensional materials have attracted wide interests for its prospective realization of polariton devices at room temperature. Here, we propose a…

We report a new dark exciton in monolayer MoS$_2$ using second harmonic generation spectroscopy. Hereby, the spectrally dependent second harmonic generation intensity splits into two branches, and an anticrossing is observed at $\sim$ 25…

介观与纳米尺度物理 · 物理学 2024-08-22 Chenjiang Qian , Viviana Villafañe , Pedro Soubelet , Peirui Ji , Andreas V. Stier , Jonathan J. Finley

Strong light matter coupling between excitons and microcavity photons, as described in the framework of cavity quantum electrodynamics, leads to the hybridization of light and matter excitations. The regime of collective strong coupling…

We demonstrate the strong coupling of direct transition excitons in tungsten disulfide (WS2) with collective plasmonic resonances at room temperature. We use open plasmonic cavities formed by periodic arrays of metallic nanoparticles. We…

Spectral control of closely spaced excitonic transitions is central to valleytronic photonics, nanoscale light sources, and wavelength-encoded sensing. In monolayer molybdenum disulfide (MoS2), the A and B excitons are separated by only…

光学 · 物理学 2026-05-21 Abdullah Efe Yildiz , Emre Ozan Polat

Tailoring the photoluminescence (PL) properties in two-dimensional (2D) molybdenum disulfide (MoS2) crystals using external factors is critical for its use in valleytronic, nanophotonic and optoelectronic applications. Although significant…

We present an analytical investigation of the optical absorption spectrum of monolayer molybdenumdisulfide. Based on the density matrix formalism, our approach gives insights into the microscopic origin of excitonic transitions, their…

材料科学 · 物理学 2014-03-24 Gunnar Berghäuser , Ermin Malic

Excitons, Coulomb bound electron-hole pairs, are composite bosons and their interactions in traditional semiconductors lead to condensation and light amplification. The much stronger Coulomb interaction in transition metal dichalcogenides…

介观与纳米尺度物理 · 物理学 2017-04-05 M. Manca , M. M. Glazov , C. Robert , F. Cadiz , T. Taniguchi , K. Watanabe , E. Courtade , T. Amand , P. Renucci , X. Marie , G. Wang , B. Urbaszek

Monolayer transition-metal dichalcogenide (TMD) semiconductors exhibit strong excitonic effects and hold promise for optical and optoelectronic applications. Yet, electron doping of TMDs leads to the conversion of neutral excitons into…

The discovery of two-dimensional transition metal dichalcogenides (2D TMDs) has promised next-generation photonics and optoelectronics applications, particularly in the realm of nanophotonics. Arguably, the most crucial fundamental…

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