相关论文: Cavity-Modulated Proton Transfer Reactions
Manipulation of chemical reactivity often involves changing reagents or environmental conditions. Alternatively, strong coupling between light and matter offers a way to tunably hybridize their physicochemical properties and thereby change…
We demonstrate the manipulation of transmitted light through an optical Fabry-Perot cavity, built around a spectroscopy cell containing enriched rubidium vapor. Light resonant with the $^{87}$Rb D$_{2}$ ($F=2/F=1$) $\leftrightarrow F'$…
We experimentally study the interaction between a cold atom cloud and many longitudinal modes of a high quality Fabry-Perot cavity, by measuring signatures of collective light shifts in the cavity transmission spectrum of an optical…
Cavity quantum electrodynamics provides an ideal platform to engineer and control light-matter interactions with polariton quasiparticles. In this work, we investigate collective phenomena in a system of many particles in a harmonic trap…
We show that a pair of quantized cavity modes interacting with a spectrally broadened ensemble of Lambda-type atoms is analogous to an ensemble of two level systems coupled to a bosonic reservoir. This provides the possibility for an…
The rate of energy transfer in donor-acceptor systems can be manipulated via the common interaction with the confined electromagnetic modes of a micro-cavity. We analyze the competition between the near-field short range dipole-dipole…
We show that by manipulating quantum interference in a multi-atom cavity QED system, the nonlinear excitation of the cavity-atom polariton can be resonantly enhanced while the linear excitation is suppressed. Under appropriate conditions,…
Cavity quantum electrodynamics offers the possibility to observe and control the motion of few or individual atoms, enabling the realization of various quantum technological tasks such as quantum-enhanced metrology or quantum simulation of…
Quantum proton tunneling (QPT) in the two representative multi-electron/-proton transfer electrode processes, i.e. hydrogen evolution reaction (HER) and oxygen reduction reaction (ORR), was investigated by using polycrystalline platinum…
Molecular polaritons arise when molecules interact so strongly with light that they become entangled with each other. This light-matter hybridization alters the chemical and physical properties of the molecular system and allows chemical…
We demonstrate the effects of cavity quantum electrodynamics for a quantum dot coupled to a photonic molecule, consisting of a pair of coupled photonic crystal cavities. We show anti-crossing between the quantum dot and the two super-modes…
We investigate the conditions yielding plasmon-exciton strong coupling at the single emitter level in the gap between two metal nanoparticles. A quasi-analytical transformation optics approach is developed that makes possible a thorough…
Achieving control over chemical reaction's rate and stereoselectivity realizes one of the Holy Grails in chemistry that can revolutionize chemical and pharmaceutical industries. Strong light-matter interaction in optical or nanoplasmonic…
Cavity quantum electrodynamics (QED) studies the interaction between light and matter at the single quantum level and has played a central role in quantum science and technology. Combining the idea of cavity QED with moir\'e materials, we…
A major trend within the field of cavity QED is to boost the interaction strength between the cavity field and the atomic internal degrees of freedom of the trapped atom by decreasing the mode volume of the cavity. In such systems, it is…
Dressing quantum states of matter with virtual photons can create exotic effects ranging from vacuum-field modified transport to polaritonic chemistry, and may drive strong squeezing or entanglement of light and matter modes. The…
The coherent energy transfer between a quantum charger and a quantum battery is analyzed. In particular, we study how to improve the direct energy transfer by adding a photonic cavity as a mediator. We show that the additional degree of…
We have studied the electron hopping in a two-CdSe quantum dot system linked by an azobenzene-derived light-switching molecule. This system can be considered as a prototype of a QD supercrystal. Following the computational strategies given…
From fundamental studies of light-matter interaction to applications in quantum networking and sensing, cavity quantum electrodynamics (QED) provides a platform-crossing toolbox to control interactions between atoms and photons. The…
Polaritonic chemistry exploits strong light-matter coupling between molecules and confined electromagnetic field modes to enable new chemical reactivities. In systems displaying this functionality, the choice of the cavity determines both…