相关论文: Attosecond correlated electron dynamics at C$_{60}…
We demonstrate the role played by the fullerene shell in the photoionization and vacancy decay of endohedral atoms A@C60. It is shown, partly in the frame of a rather simple model that describes the fullerene shell, partly using only the…
We develop an analytical model for ultraintense attosecond pulse emission in the highly relativistic laser-plasma interaction. In this model, the attosecond pulse is emitted by a strongly compressed electron layer around the instant when…
Plasmons produce large confinement and enhancement of light that enable applications as varied as cancer therapy and catalysis. Adding to these appealing properties, graphene has emerged as a robust, electrically tunable material exhibiting…
In polymeric semiconductors, charge carriers are polarons, which means that the excess charge deforms the molecular structure of the polymer chain that hosts it. This effect results in distinctive signatures in the vibrational modes of the…
Tracking the coupled motion of electrons and nuclei on their intrinsic timescales is essential to understanding and controlling photochemical transformations. While attosecond techniques have provided unprecedented insight into electronic…
The photoelectric effect has a sister process relevant in optoelectronics called internal photoemission. Here an electron is photoemitted from a metal into a semiconductor. While the photoelectric effect takes place within less than 100…
Time delays in photoemission are on the order of attoseconds and have been experimentally determined in atoms, molecules and solids. Their magnitude and energy dependence are expected to yield fundamental insights into the properties of the…
Photoelectric properties of metamaterials containing non-centrosymmetric, similarly oriented metallic nanoparticles embedded in a homogeneous semiconductor matrix are theoretically studied. Due to the asymmetric shape of the nanoparticle…
The generation of ultra-strong attosecond pulses through laser-plasma interactions offers the opportunity to surpass the intensity of any known laboratory radiation source, giving rise to new experimental possibilities, such as quantum…
We point out that plasmons in doped graphene simultaneously enable low-losses and significant wave localization for frequencies below that of the optical phonon branch $\hbar\omega_{Oph}\approx 0.2$ eV. Large plasmon losses occur in the…
In recent years nanoscale coherent imaging has emerged as an indispensable imaging modality allowing to surpass the resolution limit given by classical imaging optics. At the same time, attosecond science has experienced enormous progress…
Recently, the implementation of plasmonic nanoantennas has opened new possibilities to investigate the nanoscale dynamics of individual biomolecules in living cell. However, studies have yet been restricted to single molecular species as…
When intense laser fields interact with nanoscale targets, strong-field physics meets plasmonic near-field enhancement and sub-wavelength localization of light. Photoemission spectra reflect the associated attosecond optical and electronic…
We concentrate here on photon absorption as well as electron and positron scattering upon endohedrals that consist of a fullerenes shell and an inner atom A. The aim is to understand the effect of fullerene electron shell in formation of…
In quantum systems, coherent superpositions of electronic states evolve on ultrafast timescales (few femtosecond to attosecond, 1 as = 0.001 fs = 10^{-18} s), leading to a time dependent charge density. Here we exploit the first attosecond…
Plasmonic metal nanostructures are an integral part of nanophotonic device applications owing to their ability to generate strong localized electromagnetic fields when illuminated from the far-field. These nanostructures can be prepared in…
Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…
Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: higher photon flux (permitting…
Time-resolved electron microscopy aims at tracking nanoscale excitations and dynamic states of matter with a temporal resolution ultimately reaching the attosecond regime. Periodically time-varying fields in an illuminated specimen cause…
Plasmonic superradiance originates from the plasmon mediated strong correlation that builds up between dipolar emitters coupled to a metal nanoparticle. This leads to a fast burst of emission so that plasmonic superradiance constitutes…