相关论文: Fluorescence quenching in plasmonic dimers due to …
We develop a microscopic model for fluorescence of a molecule (or semiconductor quantum dot) near a small metal nanoparticle. When a molecule is situated close to metal surface, its fluorescence is quenched due to energy transfer to the…
The optical response of a coupled nanowire dimer is studied using a fully quantum mechanical approach. The translational invariance of the system allows to apply the time--dependent density functional theory for the plasmonic dimer with the…
The coupling of nanostructures with emitters opens ways for the realization of man-made subwavelength light emitting elements. In this article, we investigate the modification of fluorescence when an emitter is placed close to a…
Quantum aspects, such as electron tunneling between closely separated metallic nanoparticles, are crucial for understanding the plasmonic response of nanoscale systems. We explore quantum effects on the response of the conductively coupled…
An emitter in the vicinity of a metal nanostructure is quenched by its decay through non-radiative channels, leading to the belief in a zone of inactivity for emitters placed within $<$10nm of a plasmonic nanostructure. Here we demonstrate…
We investigate the dynamics of a plasmonic oscillation over a metal nanoparticle when it is strongly coupled to a quantum emitter (e.g. quantum dot, molecule). We simulate the density matrix evolution for a simple model; coupled…
The spontaneous emission rate of dipole emitters close to plasmonic dimers are theoretically studied within a nonlocal hydrodynamic model. A nonlocal model has to be used since quantum emitters in the immediate environment of a metallic…
Understanding and controlling the interaction between the excitonic states of a quantum emitter and the plasmonic modes of a nanocavity is one of the most relevant current scientific challenges, key for the development of many applications,…
A surrounding electromagnetic environment can engineer spontaneous emissions from quantum emitters through the Purcell effect. For instance, a plasmonic antenna can efficiently confine an electromagnetic field and enhance the fluorescent…
We demonstrate that the fluorescent emitters can increase light emission from the plasmonic nanostructures in turn. With the help of atomic force microscopy, a hybrid system consisting of a fluorescent nanodiamond and a gold nanoparticle…
We describe the process of Foerster transfer between semiconductor nanoparticles in the presence of a metal subsystem (metal nanocrystals). In the presence of metal nanocrystals, the Foerster process can become faster and more long-range.…
The electroluminescence of molecules confined inside a nanocavity in the scanning tunneling microscopy possesses many intriguing but unexplained features. We present here a general theoretical approach based on the density matrix formalism…
A rigorous theory of photon emission accompanied inelastic tunnelling inside the gap of plasmonic nanoantennas has been developed. The disappointingly low efficiency of the electrical excitation of surface plasmon polaritons in these…
We demonstrate that the emission of light by fluorescent molecules in the proximity of periodic arrays of nanoantennas or plasmonic crystals can be strongly modified when the arrays are covered by a dielectric film. The coupling between…
We analytically study the spontaneous emission of a single optical dipole emitter in the vicinity of a plasmonic nanoshell, based on the Lorenz-Mie theory. We show that the fluorescence enhancement due to the coupling between optical…
The rate of spontaneous emission is known to depend on the environment of a light source, and the enhancement of one-photon emission in a resonant cavity is known as the Purcell effect. Here we develop a theory of spontaneous two-photon…
The nonclassical modification of plasmon-assisted fluorescence enhancement is theoretically explored by placing two-level dipole emitters at the narrow gaps encountered in canonical plasmonic architectures, namely dimers and trimers of…
We develop a theory for spontaneous decay of a quantum emitter (QE) situated near metal-dielectric structure supporting localized surface plasmons. If plasmon resonance is tuned close to the QE emission frequency, the emission is enhanced…
Very large spontaneous-emission-rate enhancements (~1000) are obtained for quantum emitters coupled with tiny plasmonic resonance, especially when emitters are placed in the mouth of nanogaps formed by metal nanoparticles that are nearly in…
The combination of single photon emitters (quantum dots) and tailored metal nanoparticles with defined size and shape allows a detailed study of the interaction between light and matter. The enhanced optical near-field of the nanoparticles…