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Understanding the interplay between illumination and the electron distribution in metallic nanostructures is a crucial step towards developing applications such as plasmonic photo-catalysis for green fuels, nano-scale photo-detection and…

光学 · 物理学 2019-07-23 Yonatan Dubi , Yonatan Sivan

Light absorption and scattering of plasmonic metal nanoparticles can lead to non-equilibrium charge carriers, intense electromagnetic near-fields, and heat generation, with promising applications in a vast range of fields, from chemical and…

光学 · 物理学 2020-08-27 Guillaume Baffou , Ivan Bordacchini , Andrea Baldi , Romain Quidant

One of the goals of pump/probe spectroscopies is to determine how electrons relax after they have been driven out of equilibrium. It is challenging to determine how close electrons are to a thermal state solely by fitting their distribution…

强关联电子 · 物理学 2019-06-26 O. P. Matveev , A. M. Shvaika , T. P. Devereaux , J. K. Freericks

Recent experiments claimed that the enhancement of catalytic reaction rates occurs via the reduction of activation barriers driven by non-equilibrium (``hot'') electrons in plasmonic metal nanoparticles. These experiments place plasmonic…

化学物理 · 物理学 2020-04-22 Yonatan Sivan , Ieng Wai Un , Yonatan Dubi

We report the experimental realization of a non-galvanic, primary thermometer capable of measuring the electron temperature of a two-dimensional electron gas with negligible thermal load. Such a thermometer consists of a quantum dot whose…

介观与纳米尺度物理 · 物理学 2013-12-13 P. Torresani , M. J. Martínez-Pérez , S. Gasparinetti , J. Renard , G. Biasiol , L. Sorba , F. Giazotto , S. De Franceschi

Photoluminescence from metal nanostructures following intense ultrashort illumination is a fundamental aspect of light-matter interactions. Surprisingly, many of its basic characteristics are under ongoing debate. Here, we resolve many of…

光学 · 物理学 2023-04-20 Y. Sivan , I. W. Un , I. Kalyan , K. -Q. Lin , J. M. Lupton , S. Bange

We solve the Maxwell and heat equations self-consistently for metal nanoparticles under intense continuous wave (CW) illumination. Unlike previous studies, we rely on {\em experimentally}-measured data for the metal permittivity for…

光学 · 物理学 2016-07-13 Yonatan Sivan , Shi-Wei Chu

Energy and charge transfer across metal-semiconductor interfaces are the fundamental driving forces for a broad range of applications, such as computing, energy harvesting, and photodetection. However, the exact roles and physical…

We couple a proximity Josephson junction to a Joule-heated normal metal film and measure its electron temperature under steady state and nonequilibrium conditions. With a timed sequence of heating and temperature probing pulses, we are able…

介观与纳米尺度物理 · 物理学 2019-03-26 Libin Wang , Olli-Pentti Saira , Jukka Pekola

We use simultaneous electronic transport and optical characterization measurements to reveal new information about electronic and optical processes in nanoscale junctions fabricated by electromigration. Comparing electronic tunneling and…

介观与纳米尺度物理 · 物理学 2015-05-28 Douglas Natelson , Daniel R. Ward , Falco Hüser , Fabian Pauly , Juan Carlos Cuevas , David A. Corley , James M. Tour

Models for characterization of laser-accelerated electron via its produced bremsstrahlung are provided for both thin and thick targets. An effective temperature functional is proposed to overcome the so-called cold and hot "temperatures" in…

仪器与探测器 · 物理学 2018-08-01 Guillermo Hernández , Francisco Fernández

Understanding the intricate relation between illumination and temperature in metallic nano-particles is crucial for elucidating the role of illumination in various physical processes which rely on plasmonic enhancement but are also…

化学物理 · 物理学 2023-03-31 Ieng-Wai Un , Yonatan Dubi , Yonatan Sivan

We present a method for the measurement of a temperature differential across a single quantum dot that has transmission resonances that are separated in energy by much more than the thermal energy. We determine numerically that the method…

材料科学 · 物理学 2011-11-10 E. A. Hoffmann , N. Nakpathomkun , A. I. Persson , H. A. Nilsson , L. Samuelson , H. Linke

The thermal Casimir effect, arising from fluctuating electromagnetic fields of thermally agitated charges, induces thermosensitive forces and presents a novel approach to detecting nanoscale hot electrons, elusive yet ubiquitous in modern…

When a quantum dot is subjected to a thermal gradient, the temperature of electrons entering the dot can be determined from the dot's thermocurrent if the conductance spectrum and background temperature are known. We demonstrate this…

Measuring the temperature of a two-dimensional electron gas at temperatures of a few mK is a challenging issue, which standard thermometry schemes may fail to tackle. We propose and analyze a nongalvanic thermometer, based on a quantum…

介观与纳米尺度物理 · 物理学 2012-06-20 S. Gasparinetti , M. J. Martínez-Pérez , S. de Franceschi , J. P. Pekola , F. Giazotto

The possibility of studying non-thermal electron energization in laser-driven plasma experiments of magnetic reconnection is studied using two- and three-dimensional particle-in-cell simulations. It is demonstrated that non-thermal…

等离子体物理 · 物理学 2016-03-23 Samuel Totorica , Tom Abel , Frederico Fiuza

We present a detailed study of the non-linear thermoelectric properties of a molecular junction, represented by a dissipative Anderson-Holstein model. A single orbital level with strong Coulomb interaction is coupled to a localized…

介观与纳米尺度物理 · 物理学 2013-01-10 M. Leijnse , M. R. Wegewijs , K. Flensberg

In the domain of Fermi energy, the hot nucleus temperature can be determined by using the energy spectra of evaporated light charged particles. But this method of measurement is not without difficulties both theoretical and experimental.…

The non-thermal acceleration of electrons and ions at an oblique, non-relativistic shock is studied using large scale particle-in-cell (PIC) simulations in one spatial dimension. Physical parameters are selected to highlight the role of…

等离子体物理 · 物理学 2021-11-01 Naveen Kumar , Brian Reville
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