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This review outlines several linear optical effects featured by molecular polaritons arising in the collective strong light-matter coupling regime. Under weak laser irradiation and when the single-molecule light-matter coupling can be…

We demonstrate that exciton conductance in organic materials can be enhanced by several orders of magnitude when the molecules are strongly coupled to an electromagnetic mode. Using a 1D model system, we show how the formation of a…

介观与纳米尺度物理 · 物理学 2015-05-26 Johannes Feist , Francisco J. Garcia-Vidal

Singlet fission, the molecular process through which photons are effectively converted into pairs of lower energy triplet excitons, holds promise as a means of boosting photovoltaic device efficiencies. In the preceding article of this…

材料科学 · 物理学 2017-05-12 Roel Tempelaar , David R. Reichman

Very efficient amplification of light-matter waves (polaritons), that are a superposition of cavity photons and excitons [1] has recently been reported[2-11]. The optical gain curve versus the pump power shows a threshold and then saturates…

材料科学 · 物理学 2007-05-23 S. Savasta , O. Di Stefano , R. Girlanda

Exciton-polaritons are hybrid elementary excitations of light and matter that, thanks to their nonlinear properties, enable a plethora of physical phenomena ranging from room temperature condensation to superfluidity. While polaritons are…

介观与纳米尺度物理 · 物理学 2022-03-23 Davide Nigro , Vincenzo D'Ambrosio , Daniele Sanvitto , Dario Gerace

Molecular strong coupling offers exciting prospects in physics, chemistry and materials science. Whilst attention has been focused on developing realistic models for the molecular systems, the important role played by the entire photonic…

Exciton polaritons, arising from the interaction of electronic transitions with confined electromagnetic fields, have emerged as a powerful tool to manipulate the properties of organic materials. However, standard experimental and…

Light-matter interaction not only plays an instrumental role in characterizing materials' properties via various spectroscopic techniques but also provides a general strategy to manipulate material properties via the design of novel…

化学物理 · 物理学 2023-08-30 Braden M. Weight , Xinyang Li , Yu Zhang

Strong optical nonlinearities play a central role in realizing quantum photonic technologies. In solid state systems, exciton-polaritons, which result from the hybridization of material excitations and cavity photons, are an attractive…

Lead halide perovskites have emerged as platforms for exciton-polaritonic studies at room temperature thanks to their excellent photoluminescence efficiency and synthetic versatility. In this work we find proof of strong exciton-photon…

The interaction between light and matter can give rise to novel topological states. This principle was recently exemplified in Floquet topological insulators, where \emph{classical} light was used to induce a topological electronic band…

量子气体 · 物理学 2015-07-08 Torsten Karzig , Charles-Edouard Bardyn , Netanel Lindner , Gil Refael

Strong coupling between light and matter generates hybrid polariton modes. We present a continuum formalism that expresses the polariton modes in terms of light and matter densities of states (DOS). We derive exact expressions for the light…

材料科学 · 物理学 2024-12-03 Suman Gunasekaran , Ryan F. Pinard , Andrew J. Musser

Chemical manifestations of strong light-matter coupling have been recently subject of intense experimental and theoretical studies. Here we review the present status of this field. Section 1 is an introduction to molecular polaritonics and…

化学物理 · 物理学 2021-12-15 Tao E. Li , Bingyu Cui , Joseph E. Subotnik , Abraham Nitzan

Molecular polaritons, hybrid light-matter states formed from the strong coupling of molecular transitions and discrete photonic modes, are a compelling platform for optical control of chemical reactivity. Despite the origins of the field of…

化学物理 · 物理学 2026-02-11 Jane C. Nelson , Trevor H. Wright , Neo Lin , Madeline Rohde , Marissa L. Weichman

The elementary optical excitations of a two-dimensional electron system strongly coupled to a microcavity are trion-polaritons. Using a variational approach, we demonstrate that the competition between Coulomb interaction and light-matter…

介观与纳米尺度物理 · 物理学 2016-03-15 Ch. Grenier , C. Ciuti , A. Imamoglu

Understanding the radiative decay of exciton-polaritons is essential for achieving long-lived polaritons - a key prerequisite for enhancing nonlinear and quantum polaritonic effects. However, conventional wisdom - the coupled oscillator…

光学 · 物理学 2025-09-01 Jiaxun Song , Li He , Bo Zhen

Exciton polaritons are hybrid particles of excitons (bound electron-hole pairs) and cavity photons, which are renowned for displaying Bose Einstein condensation and other coherent phenomena at elevated temperatures. However, their formation…

介观与纳米尺度物理 · 物理学 2024-08-29 Kenneth Choo , Olivier Bleu , Jesper Levinsen , Meera M. Parish

Exciton-polaritons in semiconductor microcavities have advanced to become a model system for studying dynamical Bose-Einstein condensation, macroscopic coherence, many-body effects, nonclassical states of light and matter, and possibly…

量子气体 · 物理学 2017-03-21 C. Schneider , K. Winkler , M. D. Fraser , M. Kamp , Y. Yamamoto , E. A. Ostrovskaya , S. Hoefling

Polaritonic states arise when a bright optical transition of a molecular ensemble is resonantly matched to an optical cavity mode frequency. Here, we lay the groundwork to study the behavior of polaritons in clean, isolated systems by…

化学物理 · 物理学 2023-10-20 Adam D. Wright , Jane C. Nelson , Marissa L. Weichman

Strong light-matter interactions in both the single-emitter and collective strong coupling regimes attract significant attention due to emerging quantum and nonlinear optics applications, as well as opportunities for modifying…

介观与纳米尺度物理 · 物理学 2019-09-11 Tuomas P. Rossi , Timur Shegai , Paul Erhart , Tomasz J. Antosiewicz