相关论文: Isolating Polaritonic 2D-IR Transmission Spectra
The spectral and dispersive emission properties are analytically determined for the two-dimensional system of exciton-polaritons in microcavities excited by a resonant and coherent optical pump. New collective excitations result from the…
There is growing interest in using strongly coupled organic microcavities to tune molecular dynamics, including the electronic and vibrational properties of molecules. However, very little attention has been paid to the utility of cavity…
The polariton, a quasiparticle formed by strong coupling of a photon to a matter excitation, is a fundamental ingredient of emergent photonic quantum systems ranging from semiconductor nanophotonics to circuit quantum electrodynamics.…
In this article, we show that the collective light-matter strong coupling regime, where $N$ molecular emitters couple to the photon mode of an optical cavity, can be mapped to a quantum impurity model where the photon is the impurity that…
Optical two-dimensional Fourier-transformed (2DFT) spectroscopy is used to study the coherent optical response of potassium vapor in a thin transmission cell. Rephasing and non-rephasing spectra of the D1 and D2 transitions are obtained and…
We visualized negative refraction of phonon polaritons, which occurs at the interface between two natural crystals. The polaritons - hybrids of infrared photons and lattice vibrations - form collimated rays that display negative refraction…
Semiconductor microcavity polaritons, formed via strong exciton-photon coupling, provide a quantum many-body system on a chip, featuring rich physics phenomena for better photonic technology. However, conventional polariton cavities are…
Polaritonic modes in low-dimensional materials enable strong light-matter interactions and provide a platform for light manipulation at nanoscale. Very recently, a new class of polaritons has attracted considerable interest in…
Strong coupling (SC) between light and matter excitations such as excitons and molecular vibrations bear intriguing potential for controlling chemical reactivity, conductivity or photoluminescence. So far, SC has been typically achieved…
Over the past decade, exciton-polaritons in semiconductor microcavities have attracted a great deal of interest as a driven-dissipative quantum fluid. These systems offer themselves as a versatile platform for performing Hamiltonian…
Synthetic materials are obtained by assembling atoms or artificial atoms into regular arrays, thereby forming artificial crystals that offer powerful platforms to emulate and explore condensed-matter phenomena in highly controlled settings.…
Entanglement generation in polariton systems is fundamentally constrained by high losses and decoherence, which typically outweigh polariton nonlinearities. Here, we propose a conceptually different approach that uses optomechanical…
We demonstrate how the transport properties of molecular polaritons in optical cavities can be extracted from a microscopic modeling of pump-probe spectroscopy. Our approach combines a mean-field treatment of the light-matter Hamiltonian…
Hybrid excitations, called polaritons, emerge in systems with strong light-matter coupling. Usually, they dominate the linear and nonlinear optical properties with applications in quantum optics. Here, we show the crucial role of the…
Surface polaritons display short wavelengths compared to propagating light, thus enabling large spatial concentration and enhancement of electromagnetic energy. However, this wavelength mismatch is generally accompanied by poor…
Accurate rovibrational molecular models are employed to gain insight in high-resolution into the collective effects and intermolecular processes arising when molecules in the gas phase are interacting with a resonant infrared (IR) radiation…
Polaritons are compositional light-matter quasiparticles that arise as a result of strong coupling between a vacuum field of a resonant optical cavity and electronic excitations in quantum emitters. Reaching such a regime is often hard, as…
Plasmonic nanocavities enable the confinement of molecules and electromagnetic fields within nano-metric volumes. As a consequence, the molecules experience a remarkably strong interaction with the electromagnetic field, to such an extent…
Two-dimensional (2D) materials are able to strongly confine light hybridized with collective excitations of atoms, enabling electric-field enhancements and novel spectroscopic applications. Recently, freestanding monolayers of oxide…
We construct a model describing the response of a hybrid system where the electromagnetic field - in particular, surface plasmon polaritons - couples strongly with electronic excitations of atoms or molecules. Our approach is based on the…