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相关论文: Enantiosensitive steering of free-induction decay

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Exploring the photoinduced dynamics of chiral states offers promising avenues for advanced control of condensed matter systems. Photoinduced or photoenhanced chirality in 1T-TiSe$_{2}$ has been suggested as a fascinating platform for…

Chirality describes the asymmetry between an object and its mirror image and manifests itself in diverse functionalities across all scales of matter - from molecules and aggregates to thin films and bulk chiral materials. A particularly…

Chiral molecules exhibit enantiosensitive light-matter interactions, with photoelectron circular dichroism (PECD) serving as a sensitive probe of molecular chirality through the asymmetry in the photoelectron wavepacket amplitude. Here, we…

原子物理 · 物理学 2025-05-07 Zheming Zhou , Yang Li , Xu Zhang , Yueming Zhou , Peixiang Lu

Molecular chirality detection and enantiomer discrimination are very important issues for many areas of science and technology, prompting intensive investigations via optical methods. However, these methods are hindered by the intrinsically…

We predict a discriminatory interaction between a chiral molecule and an achiral molecule which is mediated by a chiral body. To achieve this, we generalize the van der Waals interaction potential between two ground-state molecules with…

量子物理 · 物理学 2017-05-19 Pablo Barcellona , Hassan Safari , A. Salam , Stefan Yoshi Buhmann

Separation of the two mirror images of a chiral molecule, the enantiomers, is a historically complicated problem of major relevance for biological systems. Since chiral molecules are optically active, it has been speculated that strong…

化学物理 · 物理学 2024-10-23 Rosario R. Riso , Matteo Castagnola , Enrico Ronca , Henrik Koch

Mirror symmetry is among the most fundamental concepts of physics and its spontaneous breaking at the molecular level allows chiral molecules to exist in two enantiomers that are mirror images of each other. The majority of chiro-optical…

光学 · 物理学 2021-09-29 Alessandro Ciattoni

Three-wave mixing spectroscopy of chiral molecules, which exist in left-handed and right-handed conformations, allows for enantio-selective population transfer despite random orientation of the molecules. This is based on constructive…

量子物理 · 物理学 2019-07-09 Monika Leibscher , Thomas F. Giesen , Christiane P. Koch

Recently developed circularly polarized X-ray light sources can probe ultrafast chiral electronic and nuclear dynamics through spatially localized resonant core transitions. We present simulations of time-resolved circular dichroism (TRCD)…

化学物理 · 物理学 2017-02-08 Jérémy R. Rouxel , Markus Kowalewski , Shaul Mukamel

Transverse spin angular momentum (SAM) of light and associated transverse chiral optical forces have received tremendous attention recently as the latter may lead to an optical separation of chiral biomolecules. In this context, the…

光学 · 物理学 2016-11-03 M. H. Alizadeh , B. M. Reinhard

Chiral nanophotonic platforms provide a means of creating near fields with both enhanced asymmetric properties and intensities. They can be exploited for optical measurements that allow enantiomeric discrimination at detection levels…

The circular dichroism (ICD) induced from interaction of chiral molecules with achiral plasmonic metal nanostructures has improved sensitivity of molecular chirality detection. Although experimental results have presented several orders…

Simultaneous scattering invisibility and free-space field enhancement have been achieved based on multipolar interferences among all-dielectric nanoparticles. The scattering properties of all-dielectric nanowire quadrumers are investigated…

光学 · 物理学 2017-10-05 Wei Liu , Andrey E. Miroshnichenko

Determination of enantiomeric excess is important and remains challenges. We theoretically propose a new spectroscopic method for this issue based on the chirality-dependent AC Stark effects in cyclic three-level models under the…

光学 · 物理学 2019-09-17 Chong Ye , Quansheng Zhang , Yu-Yuan Chen , Yong Li

Enantiomers are chiral molecules that exist in right-handed and left-handed conformations. Optical techniques of enantiomers detection are widely employed to discriminate between left- and right-handed molecules. However, identical spectra…

量子物理 · 物理学 2023-05-10 Mohsen Izadyari , M. Tahir Naseem , Özgür E. Müstecaplıouglu

Four-dimensional imaging of charge migration is crucial to the understanding of several ubiquitous processes in nature. The present work focuses on imaging of charge migration in an oriented epoxypropane: a chiral molecule. A linearly…

化学物理 · 物理学 2021-11-24 Sucharita Giri , Jean Christophe Tremblay , Gopal Dixit

Measuring and controlling the ionization dynamics by intense laser fields has recently led to important breakthroughs, from the investigation of tunneling time delays to attosecond molecular imaging by electron holography. In these…

Recently, two related three wave mixing experiments have been demonstrated that use allowed rotational transitions to produce a free induction decay signal with an amplitude linearly proportional to the enantiomeric excess of a chiral…

化学物理 · 物理学 2015-01-22 Kevin K. Lehmann

Ultrafast laser pulses provide unique tools to manipulate magnetization dynamics at femtosecond timescales, where the interaction of the electric field -- such as excitation of spin carriers to non-equilibrium states, generation of…

The frictionless, directional propagation of particles at the boundary of topological materials is one of the most striking phenomena in transport. These chiral edge modes lie at the heart of the integer and fractional quantum Hall effects,…