相关论文: Complexes formed in collisions between ultracold a…
We investigate theoretically the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom taking into account its fine-structure. The interaction involves the combination…
Understanding the sources of losses and chemical reactions of ultracold alkali-metal molecules is among the critical elements needed for their application in precision measurements and quantum technologies. Recent experiments with…
It has recently become possible to form molecules in ultracold gases of trapped alkali metal atoms. Once formed, the molecules may undergo elastic, inelastic and reactive collisions. Inelastic and reactive collisions are particularly…
Ultracold molecules undergo "sticky collisions" that result in loss even for chemically nonreactive molecules. Sticking times can be enhanced by orders of magnitude by interactions that lead to non-conservation of nuclear spin or total…
Ultracold gases of three distinguishable particles with large scattering lengths are expected to show rich few-body physics related to the Efimov effect. We have created three different mixtures of ultracold 6Li atoms and weakly bound 6Li2…
Collisions with chemically inert atoms or molecules change the hyperfine coupling of an alkali-metal atom through the hyperfine-shift interaction. This interaction is responsible for the pressure shifts of the microwave resonances of…
Spin-exchange collisions in alkali vapors have been at the basis of several fundamental and applied investigations, like nuclear structure studies and tests of fundamental symmetries, ultra-sensitive atomic magnetometers, magnetic resonance…
Ultracold collisions of neutral atoms and molecules have been of great interest since experimental advances enabled the cooling and trapping of such species. This study is a theoretical investigation of a low-energy collision between an…
We consider collisional properties of weakly bound heteronuclear molecules (dimers) formed in a two-species mixture of atoms with a large mass difference. We focus on dimers containing light fermionic atoms as they manifest collisional…
Elastic and inelastic properties of weakly bound s- and p-wave molecules of fermionic atoms that collide with a third atom are investigated. Analysis of calculated collisional properties of s-wave dimers of fermions in different spin states…
Ultracold collisions between spin-polarized Na atoms and vibrationally excited Na_2 molecules are investigated theoretically, using both an inelastic formalism (neglecting atom exchange channels) and a reactive formalism (including atom…
Angular momentum changing collisions can be suppressed in atoms whose valence electrons are submerged beneath filled shells of higher principle quantum number. To determine whether spin-exchange collisions are suppressed in these "submerged…
We consider the long-range states expected for complexes formed from an alkali-metal diatomic molecule in a singlet state and an alkali-metal atom. We explore the structure of the Hamiltonian for such systems, and the couplings between the…
We prepare mixtures of ultracold CaF molecules and Rb atoms in a magnetic trap and study their inelastic collisions. When the atoms are prepared in the spin-stretched state and the molecules in the spin-stretched component of the first…
We report numerically exact quantum scattering calculations on magnetic Feshbach resonances in ultracold, strongly anisotropic atom-molecule [Rb($^2$S) + SrF($^2\Sigma^+$)] collisions based on state-of-the-art ab initio potential energy…
We study the energetics of chemical reactions between ultracold ground-state alkaline-earth-metal diatomic molecules. We show that the atom-exchange reactions forming homonuclear dimers are energetically allowed for all heteronuclear…
We have carried out the first quantum dynamics calculations on ultracold atom-diatom collisions in isotopic mixtures. The systems studied are spin-polarized 7Li + 6Li7Li, 7Li + 6Li2, 6Li + 6Li7Li and 6Li + 7Li2. Reactive scattering can…
The spins of gaseous alkali atoms are commonly assumed to oscillate at a constant hyperfine frequency, which for many years has been used to define the Second. Indeed, under standard experimental conditions, the spins oscillate…
Atomic and molecular samples reduced to temperatures below 1 microkelvin, yet still in the gas phase, afford unprecedented energy resolution in probing and manipulating how their constituent particles interact with one another. For simple…
The study of state-to-state spin-exchange collisions in the vicinity of $p$-wave Feshbach resonances offer great opportunities to explore many-body interactions and novel quantum phases. Here, we report the observation of a spin-exchange…