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We prepare mixtures of ultracold $^{39}$K atoms in various hyperfine spin states and $^{23}$Na$^{39}$K molecules in an optical dipole trap at a fixed magnetic field and study inelastic two-body atom-molecule collisions. We observe…

The realization of ultracold polar molecules in laboratories has pushed both physics and chemistry to new realms. In particular, these polar molecules offer scientists unprecedented opportunities to explore chemical reactions in the…

量子气体 · 物理学 2020-05-19 Mingyuan He , Chenwei Lv , Hai-Qing Lin , Qi Zhou

We study polar alkali dimer scattering in a quasi-1D geometry for both reactive and non-reactive species. Elastic and reactive rates are computed as a function of the amplitude of a static electric field within a purely long-range model…

原子物理 · 物理学 2019-09-19 Romain Vexiau , Jean-Michel Launay , Andrea Simoni

Magnetic Feshbach resonances have allowed great success in the production of ultracold diatomic molecules from bi-alkali mixtures, but have so far eluded observation in mixtures of alkali and alkaline-earth-like atoms. Inelastic collisional…

We study the electron-energy loss spectra of strongly correlated electronic systems doped away from half-filling using dynamical mean-field theory ($d=\infty$). The formalism can be used to study the loss spectra in the optical (${\bf…

强关联电子 · 物理学 2009-10-31 Luis Craco , Mukul S. Laad

We investigate collisions of polar molecules in quasi-2D traps in the presence of an external electric field perpendicular to the collision plane. We use the quantum-defect model characterized by two dimensionless parameters: $y$ and $s$.…

量子物理 · 物理学 2015-08-17 M. Krych , Z. Idziaszek

The recent experimental realization of cold polar molecules in the rotational and vibrational ground state opens the door to the study of a wealth of phenomena involving long-range interactions. By applying an optical lattice to a gas of…

量子气体 · 物理学 2015-03-13 J. R. Armstrong , N. T. Zinner , D. V. Fedorov , A. S. Jensen

We investigate entanglement in a linear chain of $N$ polar molecules coupled by dipole interaction. In our model, nearest neighbour interaction predominate, and we compute entanglement with the help of a two-party correlation entanglement…

量子物理 · 物理学 2008-10-01 Pérola Milman , Arne Keller

The effect of electric field, applied on systems in the nanoscale regime has attracted a lot of research in recent times. We highlight some of the recent results in the field of single molecule electronics and then move on to focus on some…

材料科学 · 物理学 2008-10-11 S. Lakshmi , Sudipta Dutta , Swapan K. Pati

Exploring inelastic and reactive collisions on the quantum level is a main goal of the developing field of ultracold chemistry. We present first experimental studies of inelastic collisions of metastable ultracold triplet molecules in the…

We briefly introduce the formalism for describing dipolar molecules in an ultracold gaseous environment. This treatment includes the quantum mechanical states of the dipoles, the electric fields they produce, and their interactions with one…

原子物理 · 物理学 2009-01-05 John L. Bohn

This paper reviews recent advances in the study of strongly interacting systems of dipolar molecules. Heteronuclear molecules feature large and tunable electric dipole moments, which give rise to long-range and anisotropic dipole-dipole…

量子气体 · 物理学 2016-07-14 Bryce Gadway , Bo Yan

It is demonstrated that elastic collisions of ultracold atoms forming a heteronuclear collision complex can be manipulated by laboratory practicable dc electric fields. The mechanism of electric field control is based on the interaction of…

原子物理 · 物理学 2007-05-23 R. V. Krems

We investigate the impact of an electric field on the structure of ultralong-range polar diatomic Rydberg molecules. Both the s-wave and p-wave interactions of the Rydberg electron and the neutral ground state atom are taken into account.…

原子物理 · 物理学 2015-06-15 Markus Kurz , Peter Schmelcher

We computed the long-range interactions between two identical polar bialkali molecules in their rovibronic ground level, for all ten species involving Li, Na, K, Rb and Cs, using accurate quantum chemistry results combined with available…

原子物理 · 物理学 2017-04-11 Maxence Lepers , Romain Vexiau , Mireille Aymar , Nadia Bouloufa-Maafa , Olivier Dulieu

The formation of ultracold molecules via stimulated emission followed by a radiative deexcitation cascade in the presence of a static electric field is investigated. By analyzing the corresponding cross sections, we demonstrate the…

量子物理 · 物理学 2007-06-06 Rosario González-Férez , Michael Mayle , Peter Schmelcher

We explore the external electric field control of a species of ultralong-range molecules that emerge from the interaction of a ground state polar molecule with a Rydberg atom. The external field mixes the Rydberg electronic states and…

原子物理 · 物理学 2012-06-01 M. Mayle , S. T. Rittenhouse , P. Schmelcher , H. R. Sadeghpour

The electric field dielectric polarization-based separations mechanism represents a novel method for separating solutions at small length scales. An electric field gradient with a maximum strength of $\mathrm{0.4~MV/m}$ applied across a…

化学物理 · 物理学 2023-11-29 Gaurav Anand , Samira Safaripour , Craig Snoeyink

We present an analytic model of thermal state-to-state rotationally inelastic collisions of polar molecules in electric fields. The model is based on the Fraunhofer scattering of matter waves and requires Legendre moments characterizing the…

化学物理 · 物理学 2008-07-09 Mikhail Lemeshko , Bretislav Friedrich

We present a unified formalism for describing chemical reaction rates of trapped, ultracold molecules. This formalism reduces the scattering to its essential features, namely, a propagation of the reactant molecules through a gauntlet of…

量子物理 · 物理学 2015-05-19 Zbigniew Idziaszek , Goulven Quéméner , John L. Bohn , Paul S. Julienne