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Symmetry breaking and the emergence of order is one of the most fascinating phenomena in condensed matter physics. It leads to a plethora of intriguing ground states found in antiferromagnets, Mott insulators, superconductors, and…

Photoexcitation is a powerful means in distinguishing different interactions and manipulating the states of matter, especially in complex quantum systems. As a well-known charge density wave (CDW) material, 1T-TaS2 has been widely studied…

强关联电子 · 物理学 2019-10-02 Jin Zhang , Chao Lian , Mengxue Guan , Wei Ma , Huixia Fu , Sheng Meng

We show the ferro-rotational nature of the commensurate charge density wave (CCDW) in $1T$-$\mathrm{TaS}_2$ and track its dynamic modulations by temperature-dependent and time-resolved electric quadrupole rotation anisotropy-second harmonic…

The self-energy of the photo-hole in 2H-TaSe2 is measured by angle-resolved photoemission spectroscopy (ARPES) as a function of binding energy and temperature. In the charge-density wave (CDW) state, a structure in the self- energy is…

强关联电子 · 物理学 2007-05-23 T. Valla , A. V. Fedorov , P. D. Johnson , J. Xue , K. E. Smith , F. J. Di Salvo

Utilizing ultrafast time-resolved pump-probe spectroscopy measurements, we investigate the photoinduced quasiparticle dynamics of the topological materials LaSbTe and CeSbTe. In LaSbTe, the relaxation of quasiparticles is dominated by two…

强关联电子 · 物理学 2025-04-23 Liye Cao , Cuiwei Zhang , Yi Yang , Lei Wang , BiXia Gao , Xinbo Wang , Youguo Shi , Rongyan Chen

Using time- and angle-resolved photoemission spectroscopy with selective near- and mid-infrared photon excitations, we investigate the femtosecond dynamics of the charge density wave (CDW) phase in 1$T$-TiSe$_2$, as well as the dynamics of…

The complex phase diagram of 1T-TiSe2 consists of a charge density wave (CDW) below 200 K, and CDW fluctuations of still unknown origin at higher temperatures. Here, we use time-resolved extreme ultraviolet momentum microscopy and density…

Charge density waves (CDW) are ubiquitous in the complex phase diagram of cuprate superconductors and exhibit both short- and long-range correlations. Using time-resolved resonant X-ray scattering, we investigate the photo-induced dynamics…

The intricate competition between coexisting charge density waves (CDWs) can lead to rich phenomena, offering unique opportunities for phase manipulation through electromagnetic stimuli. Leveraging time-resolved X-ray diffraction, we…

$1T$-TiSe$_2$ is believed to posses a soft electronic mode, i.e., plasmon or exciton, that might be responsible for the exciton condensation and charge-density-wave (CDW) transition. Here, we explore collective electronic excitations in…

材料科学 · 物理学 2024-05-24 Zahra Torbatian , Dino Novko

Here we perform angle and time-resolved photoelectron spectroscopy on the commensurate Charge Density Wave (CDW) phase of 1T-TaS$_2$. Data with different probe pulse polarization are employed to map the dispersion of electronic states below…

Charge-density-wave (CDW) materials having a strong electron-phonon coupling provide a powerful platform for investigating the intricate interplay between lattice fluctuations and a macroscopic quantum order. Using time- and angle-resolved…

Systematic measurements of auto- and cross-correlations of photons emitted from individual CdTe/ZnTe quantum dots under pulsed excitation were used to elucidate non-resonant excitation mechanisms in this self-assembled system. Memory…

A charge density wave (CDW) is a phase of matter characterized by a periodic modulation of the valence electron density accompanied by a distortion of the lattice structure. The microscopic details of CDW formation are closely tied to the…

We investigate the out-of-equilibrium dynamics of a photo-excited charge-density-wave (CDW) state in the square-lattice Holstein model, in a setup similar to a pump-probe experiment. At half-filling, the ground state of this system is…

强关联电子 · 物理学 2024-06-18 Lingyu Yang , Gia-Wei Chern

We investigate the nonequilibrium electronic structure of 1T-TaS2 by time- and angle-resolved photoemission spectroscopy. We observe that strong photoexcitation induces the collapse of the Mott gap, leading to the photo-induced metallic…

强关联电子 · 物理学 2023-06-08 Q. -H. Ren , T. Suzuki , T. Kanai , J. Itatani , S. Shin , K. Okazaki

Femtosecond time-resolved core-level photoemission spectroscopy with a free-electron laser is used to measure the atomic-site specific charge-order dynamics in the charge-density-wave/Mott insulator 1T-TaS2. After strong photoexcitation, a…

Charge density waves (CDWs) underpin the electronic properties of many complex materials. Near-equilibrium CDW order is linearly coupled to a periodic, atomic-structural distortion, and the dynamics is understood in terms of amplitude and…

The dynamics of the photoinduced commensurate to incommensurate charge density wave (CDW) phase transition in 4Hb-TaSe2 are investigated by femtosecond electron diffraction. In the perturbative regime the CDW reforms on a 150 ps timescale,…

强关联电子 · 物理学 2015-06-11 N. Erasmus , M. Eichberger , K. Haupt , I. Boshoff , G. Kassier , R. Birmurske , H. Berger , J. Demsar , H. Schwoerer

We formulate a dynamical model to describe a photo-induced charge density wave (CDW) quench transition and apply it to recent multi-probe experiments on LaTe$_3$ [A. Zong et al., Nat. Phys. 15, 27 (2019)]. Our approach relies on coupled…

介观与纳米尺度物理 · 物理学 2020-02-20 Pavel E. Dolgirev , A. V. Rozhkov , Alfred Zong , Anshul Kogar , Nuh Gedik , Boris V. Fine
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