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The 4503 rovibronic term values belonging to the mutually perturbed $A^1\Sigma^+_u$ and $b^3\Pi_u$ states of Cs$_2$ were extracted from laser induced fluorescence (LIF) $A\sim b\rightarrow X^1\Sigma^+_g$ Fourier transform spectra with the…

原子物理 · 物理学 2019-10-23 A. Znotins , A. Kruzins , M. Tamanis , R. Ferber , E. A. Pazyuk , A. V. Stolyarov , A. Zaitsevskii

Rotationally-resolved Fourier-transform spectra of laser-induced fluorescence (LIF) $A^1\Sigma^+_u\sim b^3\Pi_u \rightarrow X^1\Sigma^+_g$ of K$_2$ molecules were recorded and analyzed yielding 4053 term values of spin-orbit (SO) coupled $A…

原子物理 · 物理学 2023-12-29 I. Klincare , A. Lapins , M. Tamanis , R. Ferber , A. Zaitsevskii , E. A. Pazyuk , A. V. Stolyarov

The laser induced fluorescence (LIF) spectra A1Sigma ~ b3Pi --> X1Sigma+ of KCs dimer were recorded in near infrared region by Fourier Transform Spectrometer with a resolution of 0.03 cm-1. Overall more than 200 LIF spectra were…

原子物理 · 物理学 2015-05-14 A. Kruzins , I. Klincare , O. Nikolayeva , M. Tamanis , R. Ferber , E. A. Pazyuk , A. V. Stolyarov

Laser-induced fluorescence spectra of the $c^3\Sigma^+(v_{c},J_{c}=N_{c})\rightarrow a^3\Sigma^+(v_{a},N_{a} = J_{c} \pm 1)$ transitions excited from the ground $X^1\Sigma^+$ state of $^{39}$K$^{133}$Cs molecule were recorded with…

We combined high-resolution Fourier-transform spectroscopy and large-scale electronic structure calculation to study energy and radiative properties of the high-lying (3)1{\Pi} and (5)1{\Sigma}+ states of the RbCs molecule. The…

原子物理 · 物理学 2019-05-22 K. Alps , A. Kruzins , O. Nikolayeva , M. Tamanis , R. Ferber , E. A. Pazyuk , A. V. Stolyarov

The oscillation continuum in laser-induced fluorescence spectra of bound-free $c^3\Sigma^+ \to a^3\Sigma^+$ and (4)$^1\Sigma^+ \to X^1\Sigma^+$ transitions of the KCs molecule were recorded by Fourier-transform spectrometer and modelled…

We observed the $A^1\Sigma^+\sim b^3\Pi\to a^3\Sigma^+/X^1\Sigma^+$ laser-induced fluorescence (LIF) spectra of the RbCs molecule excited from the ground $X^1\Sigma^+$ state by the Ti:Sapphire laser. The LIF radiation from the common…

We present the first high-resolution spectroscopic study of LiCs. LiCs is formed in a heat pipe oven and studied via laser-induced fluorescence Fourier-transform spectroscopy. By exciting molecules through the X$^1\Sigma^+$-B$^1\Pi$ and…

原子物理 · 物理学 2007-05-23 Peter Staanum , Asen Pashov , Horst Knoeckel , Eberhard Tiemann

LiSr was produced in a heat-pipe oven and its thermal emission spectrum around 9300 cm$^{-1}$ was recorded by a high resolution Fourier transform spectrometer. In addition, selected lines of the spectrum of deeply bound vibrational levels…

KCa was produced in a heatpipe oven and its thermal emission spectrum around 8900 cm$^{-1}$ was recorded by a high resolution Fourier transform spectrometer. In addition, many selected transitions of this spectrum between deeply bound…

The relative intensity distribution in the rotationally resolved laser-induced fluorescence spectra belonging to the $E(4)^1\Sigma^+\to (a^3\Sigma^+_1,X^1\Sigma^+)$ band systems of the KCs molecule was analyzed. The experimental intensities…

原子物理 · 物理学 2022-09-14 I. Klincare , M. Tamanis , R. Ferber , E. A. Pazyuk , A. V. Stolyarov , I. Havalyova , A. Pashov

We report on high resolution Fourier-transform spectroscopy of fluorescence to the a^3\Sigma_u^+ state excited by two-photon or two-step excitation from the X^1\Sigma_g^+ state to the 2^3\Pi_g state in the molecule K_2. These spectroscopic…

原子物理 · 物理学 2009-11-13 A. Pashov , P. Popov , H. Knöckel , E. Tiemann

The high-resolution B$^1\Sigma^+$ - A$^1\Pi$ (0, 0) and (0, 3) emission bands of the less-abundant $^{13}$C$^{17}$O isotopologue have been investigated by Fourier-transform spectroscopy in the visible region using a Bruker IFS 125HR…

The rotational and hyperfine spectrum of the $X^1\Sigma^+ \rightarrow B^3\Pi_1$ transition in TlF molecules was measured using laser-induced fluorescence from both a thermal and a cryogenic molecular beam. Rotational and hyperfine constants…

An experimental study of the long range behavior of the ground state X^1\Sigma^+_g of Sr_2 is performed by high resolution spectroscopy of asymptotic vibrational levels and the use of available photoassociation data. Ground state levels as…

化学物理 · 物理学 2010-04-19 A. Stein , H. Knöckel , E. Tiemann

A high resolution study of the electronic states 1^1\Sigma^+_u and 1^1\Pi_u which belong to the asymptote 4^1D + 5^1S and of the state 2(A)^1\Sigma^+_u, which correlates to the asymptote 5^1P + 5^1S, is performed by Fourier-transform…

化学物理 · 物理学 2015-03-19 Alexander Stein , Horst Knöckel , Eberhard Tiemann

Recently, we determined the detailed energy level structure of the $X^1\Sigma^+$, $A^1\Pi$ and $a^3\Pi$ states of AlF that are relevant to laser cooling and trapping experiments. Here, we investigate the $b^3\Sigma^+, v=0$ state of the AlF…

We have reinvestigated the A$^1\Pi$$(v=0)$ level of $^{13}$C$^{18}$O\ using new high-resolution spectra obtained via multi-photon laser excitation as well as with synchrotron-based Fourier-transform absorption spectroscopy of the A$^1\Pi…

State-of-the-art ab initio techniques have been applied to compute the potential energy curves for the electronic states in the A^1\Sigma_u^+, c^3\Pi_u, and a^3\Sigma_u^+ manifold of the strontium dimer, the spin-orbit and nonadiabatic…

化学物理 · 物理学 2012-05-30 Wojciech Skomorowski , Filip Pawlowski , Christiane P. Koch , Robert Moszynski

With four electrons, He$_2$ is one of very few molecules for which first-principles quantum-chemical calculations that include the treatment of nonadiabatic, relativistic and quantum-electrodynamics corrections are possible. Precise…

原子物理 · 物理学 2025-08-25 V. Wirth , M. Holdener , F. Merkt
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