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We present experimental data on the strong-field ionization of the argon dimer in a co-rotating two-color (CoRTC) laser field. We observe a sub-cycle interference pattern in the photoelectron momentum distribution and infer the Wigner time…

We use the non-relativistic random phase approximation with exchange to perform calculations of valence shell photoionization of Ne, Ar, Kr and Xe from their respective thresholds to photon energy of 200 eV. The energy derivative of the…

原子物理 · 物理学 2026-03-03 A. S. Kheifets

We investigate signatures of anisotropy on the dynamics of time-resolved near-threshold molecular photoemission, through simulations on a one-dimension asymmetric model molecule. More precisely, we study the relationship between the…

量子物理 · 物理学 2024-01-10 Berkane M. , Desrier A. , Lévêque C. , Taïeb R. , Caillat J

Attosecond ionization time-delays at photoelectron energies above typically 10 eV are usually interpreted using the so called asymptotic approximation as a sum of the atomic or molecular delays with a universal laser-induced contribution.…

We describe in detail how attosecond delays in laser-assisted photoionization can be computed using perturbation theory based on two-photon matrix elements. Special emphasis is laid on above-threshold ionization, where the electron…

原子物理 · 物理学 2015-06-19 J. M. Dahlström , E. Lindroth

Measured photoionization time delays may exhibit large variations as a function of the emission angles, even for spherically symmetric targets, as shown in recent RABBITT (reconstruction of attosecond beating by interference of two-photon…

原子物理 · 物理学 2022-12-29 D. I. R. Boll , L. Martini , A. Palacios , O. A. Fojón

The effects of confinement resonances on photoelectron group delay (Wigner time delay) following ionization of an atom encapsulated inside a C$_{60}$ cage have been studied theoretically using both relativistic and non-relativistic random…

原子物理 · 物理学 2014-06-11 P. C. Deshmukh , A. Mandal , S. Saha , A. S. Kheifets , V. K. Dolmatov , S T Manson

Focused laser fields with textured polarization on a sub-wavelength scale allow extracting information on electronic processes which are not directly accessible by homogeneous fields. Here, we consider photoionization in radially and…

原子物理 · 物理学 2021-06-30 Jonas Wätzel , Jamal Berakdar

We present a combined numerical and theoretical study of atomic photoionization in the time domain. We show how a photoelectron wave packet rapidly changes its shape after being emitted, from a complex multi-peak structure to eventually a…

原子物理 · 物理学 2018-04-03 Ruihua Xu , Zhaoyan Zhou , Xu Wang

A Fano resonance arises from the pathway interference between discrete and continuum states, playing a fundamental role in many branches of physics, chemistry and material science. Here, we introduce the concept of a laser-assisted Fano…

In a seminal article, Fano predicts that absorption of light occurs preferably with increase of angular momentum. Here we generalize Fano's propensity rule to laser-assisted photoionization, consisting of absorption of an…

Photoionization from energetically distinct electronic states may have a relative time delay of tens of attoseconds. Here we demonstrate that pulses of optical vortices allow measuring such attoseconds delays from magnetic sublevels, even…

原子物理 · 物理学 2016-10-03 Jonas Wätzel , Jamal Berakdar

Upon absorbing a photon, the ionized electron sails through the target force field in attoseconds to reach free space. This navigation probes details of the potential landscape that get imprinted into the phase of the ionization amplitude.…

原子物理 · 物理学 2024-12-12 Sajad Azizi , Mohamed El-Amine Madjet , Zheng Li , Jan M. Rost , Himadri S. Chakraborty

Photoionization as a half-scattering process is not instantaneous. Usually, time delays in photoionization are of the order of few tens of attoseconds (1 as = 10$^{-18}$ s). While going from a single atom to a nano-object, one can expect…

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

Ji \etal [New J. Phys. {\bf 26}, 093014 (2024)] established a direct link between the photoionization cross section and the attosecond time delay near Cooper minima (CM) in the valence shells of noble-gas atoms. This link is based on the…

原子物理 · 物理学 2026-03-03 Adam J. C. Singor , Dmitry V. Fursa , Igor Bray , Anatoli S. Kheifets

Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalization of valence electron wave functions set fundamental limits…

If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort…

The photoelectric effect, explained by Einstein in 1905, is often regarded as a one-electron phenomenon. However, in multi-electron systems, the interaction of the escaping electron with other electrons, referred to as electron correlation,…

We present analytical expressions of momentum-resolved core-level photoemission time delay in a molecular frame of a heteronuclear diatomic molecule upon photoionization by a linearly polarized soft x-rays attosecond pulse. For this…

化学物理 · 物理学 2022-05-31 Y. Tamura , K. Yamazaki , K. Ueda , K. Hatada