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Collective behavior of spins, frustration-induced strong quantum fluctuations, and subtle interplay between competing degrees of freedom in quantum materials can lead to correlated quantum states with exotic excitations that are essential…

The spin dynamics of geometrically frustrated pyrochlore antiferromagnets Y2Mo2O7 and Tb2Mo2O7 have been investigated using muon spin relaxation. A dramatic slowing down of the moment fluctuations occurs as one approaches the spin freezing…

The synergistic interplay between spin correlations, spin-orbit coupling, and competing exchange interactions provides a promising route to realize exotic quantum states with nontrivial excitations in rare-earth based frustrated magnets.…

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Muon spin rotation (muSR) experiments reveal unconventional spin freezing and dynamics in the two-dimensional (2D) triangular lattice antiferromagnet NiGa2S4. Long-lived disordered Ni-spin freezing (correlation time > 10-6 s at 2 K) sets in…

强关联电子 · 物理学 2009-11-13 D. E. MacLaughlin , Y. Nambu , S. Nakatsuji , R. H. Heffner , Lei Shu , O. O. Bernal , K. Ishida

PbCuTe2O6 is a rare example of a spin liquid candidate featuring a three dimensional magnetic lattice. Strong geometric frustration arises from the dominant antiferromagnetic interaction which generates a hyperkagome network of Cu2+ ions…

强关联电子 · 物理学 2016-03-14 P. Khuntia , F. Bert , P. Mendels , B. Koteswararao , A. V. Mahajan , M. Baenitz , F. C. Chou , C. Baines , A. Amato , Y. Furukawa

Muon spin relaxation experiments have been performed in the pyrochlore iridate Pr_2Ir_2O_7 for temperatures in the range 0.025-250 K. Kubo-Toyabe relaxation functions are observed up to > 200 K, indicating static magnetism over this…

强关联电子 · 物理学 2009-11-13 D. E. MacLaughlin , Y. Ohta , Y. Machida , S. Nakatsuji , G. M. Luke , K. Ishida , R. H. Heffner , Lei Shu , O. O. Bernal

The description and detection of unconventional magnetic states such as spin liquids is a recurring topic in condensed matter physics. While much of the efforts have traditionally been directed at geometrically frustrated antiferromagnets,…

强关联电子 · 物理学 2018-05-25 L. Bovo , M. Twengström , O. A. Petrenko , T. Fennell , M. J. P. Gingras , S. T. Bramwell , P. Henelius

The emergent behavior of spin liquids that are born out of geometrical frustration makes them an intriguing state of matter. We show that in the quantum kagome antiferromagnet ZnCu$_3$(OH)$_6$SO$_4$ several different correlated, yet…

强关联电子 · 物理学 2016-03-02 M. Gomilsek , M. Klanjsek , M. Pregelj , F. C. Coomer , H. Luetkens , O. Zaharko , T. Fennell , Y. Li , Q. M. Zhang , A. Zorko

The magnetic ground state of oxynitride pyrochlore Lu$_2$Mo$_2$O$_{5-y}$N$_2$, a candidate compound for the quantum spin liquid ($S=1/2$, Mo$^{5+}$), was studied by muon spin rotation/relaxation experiment. In contrast to Lu$_2$Mo$_2$O$_7$…

强关联电子 · 物理学 2023-01-11 S. K. Dey , K. Ishida , H. Okabe , M. Hiraishi , A. Koda , T. Honda , J. Yamaura , H. Kageyama , R. Kadono

Muon spin relaxation on Nd$_2$Ti$_2$O$_7$ (NTO) and NdLaTi$_2$O$_7$ (NLTO) compounds are presented. The time spectra for both compounds are as expected for the paramagnetic state at high temperatures, but deviate from the exponential…

强关联电子 · 物理学 2014-10-21 Hanjie Guo , Hui Xing , Jun Tong , Qian Tao , Isao Watanabe , Zhu-an Xu

We present the results of a muon-spin relaxation study of GeNi2O4. We provide further clarification of the two transitions to the antiferromagnetic state and measure the magnetic field dependence of the heat capacity up to 14 T. Both…

强关联电子 · 物理学 2007-11-14 T. Lancaster , S. J. Blundell , D. Prabhakaran , P. J. Baker , W. Hayes , F. L. Pratt

We report the magnetic and calorimetric measurements in single crystal samples of the square lattice $J_{1}-J_{2}$ quantum antiferromagnet BaCdVO(PO$_4$)$_2$. An investigation of the scaling of magnetization reveals a "dimensionality…

强关联电子 · 物理学 2019-01-14 K. Yu. Povarov , V. K. Bhartiya , Z. Yan , A. Zheludev

We carried out AC magnetic susceptibility measurements and muon spin relaxation spectroscopy on the cubic double perovskite Ba2YMoO6, down to 50 mK. Below ~1 K the muon relaxation is typical of a magnetic insulator with a spin-liquid type…

强关联电子 · 物理学 2013-06-03 M. A. de Vries , J. O. Piatek , M. Misek , J. S. Lord , H. M. Ronnow , J. -W. G. Bos

We report on thermodynamic, magnetization, and muon spin relaxation measurements of the strong spin-orbit coupled iridate Ba$_3$IrTi$_2$O$_9$, which constitutes a new frustration motif made up a mixture of edge- and corner-sharing…

强关联电子 · 物理学 2017-09-13 W. -J. Lee , S. -H. Do , Sungwon Yoon , S. Lee , Y. S. Choi , D. J. Jang , M. Brando , M. Lee , E. S. Choi , S. Ji , Z. H. Jang , B. J. Suh , K. -Y. Choi

We present microscopic magnetic properties of a two dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. A Curie-Weiss temperature theta_CW = --44 K and an antiferromagnetic (AFM) exchange…

强关联电子 · 物理学 2017-12-06 P. Khuntia , R. Kumar , A. V. Mahajan , M. Baenitz , Y. Furukawa

Inelastic neutron scattering is used to characterize spin fluctuations in the $d$-electron heavy fermion spinel $\rm LiV_2O_4$. The spin relaxation rate, $\Gamma_Q$, for $Q=0.6$ \AA$^{-1}$ is 1.5(1) meV at low temperatures and increases…

强关联电子 · 物理学 2009-11-07 S. -H. Lee , Y. Qiu , C. Broholm , Y. Ueda , J. J. Rush

Frustrated pyrochlore lattices in transition-metal oxides provide an ideal platform for realizing exotic quantum states, including spin liquids with unconventional low-energy excitations arising from the macroscopic ground-state degeneracy…

强关联电子 · 物理学 2026-05-26 Satish Kumar , U. Jena , A. Bandhopadhay , G. B. G. Stenning , D. T. Adroja , S. Petit , P. Khuntia

Using muon-spin-relaxation measurements we show that the pyrochlore compound Gd2Ti2O7, in its magnetically orderered phase below ~ 1 K, displays persistent spin dynamics down to temperatures as low as 20 mK. The characteristics of the…

Magnetic properties of a one-dimensional frustrated quantum spin system Rb2Cu2Mo3O12 is investigated by the muon spin relaxation (muSR) technique. Although this system shows an incommensurate spin correlation in neutron scattering, it has…

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