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Recently, several putative quantum spin liquid (QSL) states were discovered in ${\tilde S} = 1/2$ rare-earth based triangular-lattice antiferromagnets (TLAF) with the delafossite structure. A way to clarify the origin of the QSL state in…

The Yb based triangular lattice delafossites $A$Yb$X_2$ ($A$ = alkali metal, $X$ = O, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of CuYbSe$_2$ with a perfect…

强关联电子 · 物理学 2025-09-23 Barkha Khattar , Anzar Ali , Masahiko Isobe , Yogesh Singh

Rare-earth delafossites were recently proposed as promising candidates for the realization of an effective $S$=1/2 quantum spin liquid (QSL) on the triangular lattice. In contrast to the most actively studied triangular-lattice…

强关联电子 · 物理学 2020-01-08 R. Sarkar , Ph. Schlender , V. Grinenko , E. Haeussler , Peter J. Baker , Th. Doert , H. -H. Klauss

Layered rare-earth delafossites $ARX_2$ with $R$ = Yb(III) or Ce(III) have received a lot of interest as potential hosts for a quantum spin-liquid ground state. Some systems of this family that show no long-range order down to the lowest…

强关联电子 · 物理学 2022-12-26 S. M. Avdoshenko , A. A. Kulbakov , E. Häußler , P. Schlender , Th. Doert , J. Ollivier , D. S. Inosov

The delafossite-like compound NaYbO$_2$ hosts a triangular lattice of Yb$^{3+}$ moments and is a promising candidate for the realization of a quantum spin liquid ground state -- an exotic, quantum-disordered magnetic phase featuring…

Rare earth triangular lattice materials have been proposed as a good platform for the investigation of frustrated magnetic ground states. KErSe$_2$ with the delafossite structure, contains perfect two-dimensional Er$^{3+}$ triangular layers…

Here, we report the synthesis and magnetic properties of a Yb-based triangular-lattice compound LiYbS$_2$. At low temperatures, it features an effective spin-$\frac{1}{2}$ state due to the combined effect of crystal electric field and spin…

强关联电子 · 物理学 2020-04-22 K. M. Ranjith , Ph. Schlender , Th. Doert , M. Baenitz

We investigated the spin dynamics by electron spin resonance (ESR) of the Yb-based, effective spin-1/2 delafossites NaYbO$_{2}$, AgYbO$_{2}$, LiYbS$_{2}$, NaYbS$_{2}$, and NaYbSe$_{2}$ which all show an absence of magnetic order down to…

A quantum spin liquid (QSL) is a state of matter characterized by fractionalized quasiparticle excitations, quantum entanglement, and a lack of long-range magnetic order. However, QSLs have evaded definitive experimental observation.…

Antiferromagnetically coupled S=1/2 spins on an isotropic triangular lattice is the paradigm of frustrated quantum magnetism, but structurally ideal realizations are rare. Here we investigate NaYbO$_2$, which hosts an ideal triangular…

Triangular lattice of rare-earth ions with interacting effective spin-$1/2$ local moments is an ideal platform to explore the physics of quantum spin liquids (QSLs) in the presence of strong spin-orbit coupling, crystal electric fields, and…

The two-dimensional triangular-lattice antiferromagnet (TLAF) is a textbook example of frustrated magnetic systems. Despite its simplicity, the TLAF model exhibits a highly rich and complex magnetic phase diagram, featuring numerous…

The delafossite structure of NaYbS2 contains a planar spin-1/2 triangular lattice of Yb3+ ions and features a possible realisation of a quantum spin-liquid state. We investigated the Yb3+ spin dynamics by Electron Spin Resonance (ESR) in…

强关联电子 · 物理学 2019-03-11 Jörg Sichelschmidt , Philipp Schlender , Burkhard Schmidt , Michael Baenitz , Thomas Doert

High-quality single crystals of NaYbSe$_2$, which resembles a perfect triangular-lattice antiferromagnet without the intrinsic disorder, are investigated by magnetization and specific heat, as well as the local probe techniques nuclear…

We present the structural characterization and low-temperature magnetism of the triangular-lattice delafossite NaYbO$_2$. Synchrotron x-ray diffraction and neutron scattering exclude both structural disorder and crystal-electric-field…

The ytterbium-based delafossite NaYbSe$_2$ is discussed as a prototype for a spin-orbit entangled, effective spin-1/2 triangular spin lattice with emerging antiferromagnetic correlations and a quantum-spin-liquid (QSL) ground state. We…

强关联电子 · 物理学 2025-01-08 S. Luther , K. M. Ranjith , Th. Doert , J. Wosnitza , H. Kühne , M. Baenitz

Two-dimensional triangular-lattice materials with spin-1/2 are perfect platforms for investigating quantum frustrated physics with spin fluctuations. Here we report the structure, magnetization, heat capacity and inelastic neutron…

强关联电子 · 物理学 2019-12-17 Jie Xing , Liurukara D. Sanjeewa , Jungsoo Kim , G. R. Stewart , Andrey Podlesnyak , Athena S. Sefat

We introduce the rare-earth delafossite compound TlYbSe$_2$ -- extending the search for quantum spin liquids in frustrated triangular lattice magnets. While the DC magnetisation suggests magnetic exchange interactions in the order of…

强关联电子 · 物理学 2025-09-16 Bishnu P. Belbase , Arjun Unnikrishnan , Shi Feng , Eun Sang Choi , Johannes Knolle , Arnab Banerjee

Platelike high-quality NaYbS$_{2}$ rhombohedral single crystals with lateral dimensions of a few mm have been grown and investigated in great detail by bulk methods like magnetization and specific heat, but also by local probes like nuclear…

The electronic and magnetic properties of the delafossite CuFeO2 are investigated by means of electronic structure calculations. They are performed using density functional theory in the generalized gradient approximation as well as the new…

强关联电子 · 物理学 2008-08-24 Volker Eyert , Raymond Fresard , Antoine Maignan
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