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We report the single-crystal X-ray analysis and magnetic properties of a new double-layered perovskite antiferromagnet, Cs$_3$Cu$_2$Cl$_4$Br$_3$. This structure is composed of Cu$_2$Cl$_4$Br$_3$ double layers with elongated CuCl$_4$Br$_2$…

强关联电子 · 物理学 2015-06-25 F. Yamada , T. Ono , H. Tanaka , J. Yamaura

The magnetic structure of (La${}_{1.8}$Eu${}_{0.2}$)CuO${}_4$ has been studied by magnetization measurements of single crystals, which show antiferromagnetic long-range order below $T_N$ = 265 K and a structural phase transition at $T_s$ =…

超导电性 · 物理学 2009-11-07 I. Tsukada , X. F. Sun , Seiki Komiya , A. N. Lavrov , Yoichi Ando

Materials with strongly correlated electrons exhibit physical properties that are often difficult to predict as they result from the interactions of large numbers of electrons combined with several quantum degrees of freedom. The layered…

A quantum spin liquid state has long been predicted to arise in spin-1/2 Heisenberg square-lattice antiferromagnets at the boundary region between N\'eel (nearest-neighbor interaction dominates) and columnar (next-nearest-neighbor…

In strongly correlated electron materials, the electronic, spin, and charge degrees of freedom are closely intertwined. This often leads to the stabilization of emergent orders that are highly sensitive to external physical stimuli…

In contrast to the previous reports that the divalent perovskite SrCrO$_3$ was believed to be cubic structure and nonmagnetic metal, recent measurements suggest coexistence of majority tetragonally distorted weak antiferromagnetic phase and…

强关联电子 · 物理学 2009-10-01 K. -W. Lee , W. E. Pickett

Double-perovskite oxides that contain both 3d and 5d transition metal elements have attracted growing interest as they provide a model system to study the interplay of strong electron interaction and large spin-orbit coupling (SOC). Here,…

A ferroelectric transition occurring simultaneously with helical spin order has been found in both the polycrystalline and single crystal samples of LiCuVO4. The system has Cu2+ spins (s=1/2) of the CuO2 chains formed of edge-sharing CuO4…

强关联电子 · 物理学 2015-06-25 Yutaka Naito , Kenji Sato , Yukio Yasui , Yusuke Kobayashi , Yoshiaki Kobayashi , Masatoshi Sato

We report the structural, magnetic and thermodynamic properties of the double perovskite compound La2CuIrO6 from X-ray, neutron diffraction, neutron depolarization, dc magnetization, ac susceptibility, specific heat, muon-spin-relaxation…

Using high-pressure single-crystal x-ray diffraction combined with thermodynamic measurements and density-functional calculations, we uncover the microscopic magnetic model of the mineral brochantite, Cu$_4$SO$_4$(OH)$_6$, and its evolution…

强关联电子 · 物理学 2025-11-25 Victoria A. Ginga , Bin Shen , Ece Uykur , Nico Giordano , Philipp Gegenwart , Alexander A. Tsirlin

We systematically synthesized perovskite-type oxides Sr1-xCaxCoO3 containing unusually high valence Co4+ ions by a high pressure technique, and investigated the effect of systematic lattice change on the magnetic and electronic properties.…

First principles density functional calculations for Fe$_{2}$O$_{3}$ has been performed over a wide range of pressures. The ground state is corundum-type hematite and is an antiferromagnetic insulator. This is in good agreement with…

材料科学 · 物理学 2009-03-13 Dipta Bhanu Ghosh , Stefano de Gironcoli

We report a first-order phase transition at T_M=357 K in single crystal Ca_2RuO_4, an isomorph to the superconductor Sr_2RuO_4. The discontinuous decrease in electrical resistivity signals the near destruction of the Mott insulating phase…

强关联电子 · 物理学 2009-10-31 C. S. Alexander , G. Cao , V. Dobrosavljevic , E. Lochner , S. McCall , J. E. Crow , R. P. Guertin

We theoretically investigate magnetic properties of Sr$_2$TcO$_4$, a 4d transition-metal layered perovskite of the K$_2$NiF$_4$-type with half-filled t$_{2g}$ states. The effect of local Coulomb repulsion between the t$_{2g}$ orbitals is…

强关联电子 · 物理学 2017-05-17 Alen Horvat , Leonid Pourovskii , Markus Aichhorn , Jernej Mravlje

We report the systematic synthesis, crystal structure, magnetization, and powder neutron diffraction of single crystalline and polycrystalline CaCo$_2$TeO$_6$ samples. CaCo$_2$TeO$_6$ crystallizes in an orthorhombic structure with $Pnma$…

Antiferromagnetic insulators on the diamond lattice are candidate materials to host exotic magnetic phenomena ranging from spin-orbital entanglement to degenerate spiral ground-states and topological paramagnetism. Compared to other…

强关联电子 · 物理学 2017-08-16 L. Ge , J. Flynn , J. A. M. Paddison , M. B. Stone , S. Calder , M. A. Subramanian , A. P. Ramirez , M. Mourigal

\SCWO is a tetragonal ($I4/m$) double perovskite with diamagnetic W$^{6+}$ (5d$^0$) and (Jahn-Teller-active) Cu$^{2+}$ (3$d^9$) in a rocksalt-ordered arrangement on the B sites, modelling an anisotropic fcc-lattice antiferromagnet with…

Recent experiments [J. Guo et al., Phys. Rev. Lett.124,206602 (2020)] on thermodynamic properties of the frustrated layered quantum magnet SrCu$_2$(BO$_3$)$_2$ -- the Shastry-Sutherland material -- have provided strong evidence for a…

强关联电子 · 物理学 2021-06-18 Guangyu Sun , Nvsen Ma , Bowen Zhao , Anders W. Sandvik , Zi Yang Meng

In half-doped Pr0.50A0.50CoO3 metallic perovskites, the spin-lattice coupling brings about distinct magnetostructural transitions for A=Ca and A=Sr at temperatures close to 100 K. However, the ground magnetic properties of Pr0.50Sr0.50CoO3…

Magnetometry, electrical transport, and neutron scattering measurements were performed on single crystals of the Fe^{4+}-containing perovskite-related phase Sr_3Fe_2O_7-x as a function of oxygen content. Although both the crystal structure…

强关联电子 · 物理学 2013-06-12 D. C. Peets , J. -H. Kim , P. Dosanjh , M. Reehuis , A. Maljuk , N. Aliouane , C. Ulrich , B. Keimer
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