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In the 1970s a new paradigm was introduced that interacting quenched systems, such as a spin-glass, have a phase transition in which long time memory of spatial patterns is realized without spatial correlations. The principal methods to…

Understanding and interpreting dynamics of functional materials \textit{in situ} is a grand challenge in physics and materials science due to the difficulty of experimentally probing materials at varied length and time scales. X-ray photon…

Analysis of X-ray Photon Correlation Spectroscopy (XPCS) data for non-equilibrium dynamics often requires manual binning of age regions of an intensity-intensity correlation function. This leads to a loss of temporal resolution and…

信号处理 · 电气工程与系统科学 2022-01-21 Tatiana Konstantinova , Lutz Wiegart , Maksim Rakitin , Anthony M DeGennaro , Andi M Barbour

Around a glass transition, the dynamics of a supercooled liquid dramatically slow down, exhibited by caging of particles, while the structural changes remain subtle. In alternative to recent machine learning studies searching for structural…

无序系统与神经网络 · 物理学 2022-09-07 Kaihua Zhang , Xinyang Li , Yuliang Jin , Ying Jiang

Understanding solution-phase aggregation and dynamics in complex fluids is critical for material processing, yet widely used dynamic light scattering (DLS) fails for strongly attenuating systems such as conjugated polymers. We use X-ray…

Fast multi-phase processes in methane hydrate-bearing samples are challenging for micro-CT quantitative study because of complex tomographic data analysis involving time-consuming segmentation procedures. This is due to the sample…

地球物理 · 物理学 2022-09-12 Mikhail I. Fokin , Viktor V. Nikitin , Anton A. Duchkov

X-ray photon correlation spectroscopy (XPCS) allows for the resolution of dynamic processes within a material across a wide range of length and time scales. X-ray speckle visibility spectroscopy (XSVS) is a related method that uses a single…

数值分析 · 数学 2023-01-09 Shaswat Mohanty , Christopher B. Cooper , Hui Wang , Mengning Liang , Wei Cai

Behavior of two-time autocorrelation during the phase separation in solid binary mixtures are studied via numerical solutions of the Cahn-Hilliard equation as well as Monte Carlo simulations of the Ising model. Results are analyzed via…

统计力学 · 物理学 2015-09-02 Jiarul Midya , Suman Majumder , Subir K. Das

X-ray free electron laser (XFEL) experiments have brought unique capabilities and opened new directions in research, such as creating new states of matter or directly measuring atomic motion. One such area is the ability to use finely…

This paper describes a novel system for automatic classification of images obtained from Anti-Nuclear Antibody (ANA) pathology tests on Human Epithelial type 2 (HEp-2) cells using the Indirect Immunofluorescence (IIF) protocol. The IIF…

细胞行为 · 定量生物学 2014-04-15 Arnold Wiliem , Conrad Sanderson , Yongkang Wong , Peter Hobson , Rodney F. Minchin , Brian C. Lovell

We investigate the behaviour of randomly cross-linked (co)polymer blends using a combination of replica theory and large-scale molecular dynamics simulations. In particular, we derive the analogue of the random phase approximation for…

软凝聚态物质 · 物理学 2009-11-13 A. V. Klopper , Carsten Svaneborg , Ralf Everaers

The calculation of thermodynamic properties of biochemical systems typically requires the use of resource-intensive molecular simulation methods. One example thereof is the thermodynamic profiling of hydration sites, i.e. high-probability…

生物大分子 · 定量生物学 2020-01-08 Ahmadreza Ghanbarpour , Amr H. Mahmoud , Markus A. Lill

We report X-ray Photon Correlation Spectroscopy (XPCS) results on a bidimensional (2D) gel formed by a Langmuir monolayer of gold nanoparticles. The system allows an experimental determination of the fourth order time correlation function…

软凝聚态物质 · 物理学 2012-03-29 D. Orsi , L. Cristofolini , G. Baldi , A. Madsen

X-ray Photon Correlation Spectroscopy (XPCS) enables direct access to atomic-scale dynamics in disordered materials, revealing both spontaneous and X-ray-induced relaxation processes. Here, we study two compositionally similar alloy glasses…

We study a possibility of measuring the time-resolved second-order autocorrelation function of one of two beams generated in type-II parametric downconversion by means of temporal magnification of this beam, bringing its correlation time…

Glass forming liquids exhibit structural relaxation behaviors, reflecting underlying atomic rearrangements on a wide range of timescales. These behaviors play a crucial role in determining many material properties. However, the relaxation…

A MATLAB program has been developed for simulation of polymer blend self-assembly with nano-scaled features. The Cahn-Hilliard equation is implemented to calculate the free energy profile of the polymer blends. The Flory-Huggins type of…

材料科学 · 物理学 2010-07-09 Yingrui Shang , David Kazmer

The Cahn-Hilliard system has been used to describe a wide number of phase separation processes, from co-polymer systems to lipid membranes. In this work the convergence properties of a closest-point based scheme is investigated. In place of…

数值分析 · 数学 2017-02-28 Prerna Gera , David Salac

We present an adaptive scheme for isogeometric phase-field modeling, to perform suitably graded hierarchical refinement and coarsening on both single- and multi-patch geometries by considering truncated hierarchical spline constructions…

We present a phase-field model based on the Cahn-Hilliard equation to investigate the properties of phase separation in DNA nanostar systems. Leveraging a realistic free-energy functional derived from Wertheim theory, our model captures the…

软凝聚态物质 · 物理学 2025-04-23 Marco Cappa , Francesco Sciortino , Lorenzo Rovigatti
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