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We describe numerically the ionization process induced by linearly and circularly polarized XUV attosecond laser pulses on an aligned atomic target, specifically, the excited state…

原子物理 · 物理学 2021-05-26 Juan J. Omiste , Lars Bojer Madsen

We study the breakup of $\text{H}_2^+$ exposed to super-intense, femtosecond laser pulses with frequencies greater than that corresponding to the ionization potential. By solving the time-dependent Schr\"odinger equation in an extensive…

原子物理 · 物理学 2016-04-12 Lun Yue , Lars Bojer Madsen

The dipolar dissociation of molecular oxygen due to 21-35 eV energy electron collision has been studied using the time sliced velocity map imaging technique. A rough estimation about the threshold of the process and the kinetic energy and…

原子与分子团簇 · 物理学 2016-08-31 Pamir Nag , Dhananjay Nandi

The dynamics of molecular electron excitation and ionisation is studied in real-time for ultra-short IR laser pulses of intensity I>10^{13} W/cm^{2}. The multi-electron molecule is modeled by a system of two active electrons moving in a…

光学 · 物理学 2015-06-26 A. I. Pegarkov

A theoretical investigation of electron-D2 resonant collisions - via the low lying and the Rydberg states of D2- - is presented for vibrational excitation, dissociative electron attachment and dissociative excitation processes by using the…

原子物理 · 物理学 2024-11-15 V Laporta , R Agnello , G Fubiani , I Furno , C Hill , D Reiter , F Taccogna

The ionization energy of D$_2$ has been determined experimentally from measurements involving two-photon Doppler-free vacuum-ultraviolet pulsed laser excitation and near-infrared continuous-wave laser excitation to yield…

We investigate theoretically the dissociative ionization of a H2+ molecule using two ultrashort laser (pump-probe) pulses. The pump pulse prepares a dissociating nuclear wave packet on an ungerade surface of H2+. Next, an UV (or XUV) probe…

量子物理 · 物理学 2013-05-29 Szczepan Chelkowski , André D. Bandrauk

We have studied the ionization and fragmentation of $SO_2$ molecular target in collision with 1 MeV proton beam using the technique of recoil ion momentum spectroscopy. Fragmentation dynamics of doubly charged $SO_2^{2+}$ molecular ion has…

原子物理 · 物理学 2025-04-08 Sandeep Bajrangi Bari , Ranojit Das , Rohit Tyagi , Aditya H. Kelkar

We describe the results of experiments and simulations performed with the aim of extending photoelectron spectroscopy with intense laser pulses to the case of molecular compounds. Dimer frame photoelectron angular distributions generated by…

The ultrafast electronic and nuclear dynamics of H2 laser-induced double ionization is studied using a time-dependent wave packet approach that goes beyond the fixed nuclei approximation. The double ionization pathways are analyzed by…

量子物理 · 物理学 2011-11-09 Sebastien Saugout , Christian Cornaggia , Annick Suzor-Weiner , Eric Charron

We study the dissociation of H$_2$$^+$ in uv laser pulses by solving the non-Born-Oppenheimer time-dependent Schr\"{o}dinger equation as a function of the photon energy $\omega$ of the pulse. Significant enhancements of the dissociation…

原子与分子团簇 · 物理学 2014-07-22 Kunlong Liu , Qianguang Li , Pengfei Lan , Peixiang Lu

An ab initio simulation of strong-field photodissociation of diatomic molecules was developed, inspired by recent dissociation experiments of F2-. The transition between electronic states was modeled, including the laser pulse and…

原子物理 · 物理学 2020-06-26 Bar Ezra , Shimshon Kallush , Ronnie Kosloff

We investigate K-shell ionization of N$_2$ at 40 keV photon energy. Using a COLTRIMS reaction microscope we determine the vector momenta of the photoelectron, the Auger electron and both N$^+$ fragments. These fully differential data show…

We analyze the photoelectron angular distribution in two-pathway interference between non\-resonant one-photon and resonant two-photon ionization of neon. We consider a bichromatic femtosecond XUV pulse whose fundamental frequency is tuned…

We report measurements on the H$^{+}$ + H$^{+}$ fragmentation channel following direct single-photon double ionization of neutral NH$_{3}$ at 61.5 eV, where the two photoelectrons and two protons are measured in coincidence using 3-D…

We formulate a general hybrid quantum-classical technique to describe the interaction of diatomic molecules with XUV pulses. We demonstrate the accuracy of our model in the context of the interaction of the O$_2$ molecule with an XUV pulse…

We show the details of the pathway for dissociative ionization process of ground electronic state of aligned D$^{+}_{2}$ due to first ionization of D$_2$ in short ($\thicksim$100 fs) and intense ($4.0\times10^{14}$ W cm$^{-2}$) 480 nm laser…

原子物理 · 物理学 2010-11-23 Mohsen Vafaee , Babak Shokri

We report a joint experimental and theoretical study using a combination of polarization-controlled free-electron-laser (FEL) and near-infra\-red (NIR) pulses in a synchronized two-color photo\-ionization scheme. Excited He$^+$ ions,…

Double ionization of diatomic molecules by short linearly polarized laser pulses is analyzed. We consider the final stage of the ionization process, that is the decay of a highly excited two electron molecule, which is formed after…

原子物理 · 物理学 2016-09-08 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt , Jakub Zakrzewski

We present a combined experimental and theoretical study on the photodissociation dynamics of ion-pair formation in O$_2$ following resonant two-photon absorption of a 9.3 eV femtosecond pulse, where the resulting O$^+$ ions are detected…

化学物理 · 物理学 2020-08-28 Kirk A. Larsen , Robert R. Lucchese , Daniel S. Slaughter , Thorsten Weber
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