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We demonstrate microwave dressing on ultracold, fermionic ${}^{23}$Na${}^{40}$K ground-state molecules and observe resonant dipolar collisions with cross sections exceeding three times the $s$-wave unitarity limit. The origin of these…

量子气体 · 物理学 2020-08-06 Zoe Z. Yan , Jee Woo Park , Yiqi Ni , Huanqian Loh , Sebastian Will , Tijs Karman , Martin Zwierlein

We report the investigation on dipolar collisions in rotational state mixtures of ultracold bosonic $^{23}$Na$^{87}$Rb molecules. The large resonant dipole-dipole interaction between molecules in rotational states of opposite parities…

原子物理 · 物理学 2021-01-13 Junyu He , Xin Ye , Junyu Lin , Mingyang Guo , Goulven Quéméner , Dajun Wang

The dipolar collision between ultracold polar molecules is an important topic both by its own right from the fundamental point of view and for the successful exploration of many-body physics with strong and long-range dipolar interactions.…

Full control of molecular interactions, including reactive losses, would open new frontiers in quantum science. Here, we demonstrate extreme tunability of chemical reaction rates by using an external electric field to shift excited…

We show that the electric dipole-dipole interaction between a pair of polar molecules undergoes an all-out transformation when superimposed by a far-off resonant optical field. The combined interaction potential becomes tunable by variation…

原子物理 · 物理学 2015-05-30 Mikhail Lemeshko , Bretislav Friedrich

Microscopic control over polar molecules with tunable interactions would enable realization of novel quantum phenomena. Using an applied electric field gradient, we demonstrate layer-resolved state preparation and imaging of ultracold…

Scattering resonances due to the dipole-dipole interaction between ultracold molecules, induced by static or microwave fields, are studied theoretically. We develop a method for coupled-channel calculations that can efficiently impose many…

量子气体 · 物理学 2023-07-11 Tijs Karman

We propose a one-channel, simple model to describe the dynamics of ultracold dipolar molecules around a F\"orster resonance. Slightly above a specific electric field, a collisional shielding can take place, suppressing the molecular losses…

量子气体 · 物理学 2024-06-21 Lucas Lassablière , Goulven Quéméner

We discuss the influence of collisions on the dynamics of an ultracold gas whose constituents interact via dipolar forces. This dynamics is governed by the elastic scattering cross section of the molecules, which is to some extent under the…

量子气体 · 物理学 2025-12-02 Reuben R. W. Wang , John L. Bohn

Ultracold polar molecules offer the possibility of exploring quantum gases with interparticle interactions that are strong, long-range, and spatially anisotropic. This is in stark contrast to the dilute gases of ultracold atoms, which have…

原子物理 · 物理学 2015-05-18 K. -K. Ni , S. Ospelkaus , D. Wang , G. Quemener , B. Neyenhuis , M. H. G. de Miranda , J. L. Bohn , J. Ye , D. S. Jin

The long-range electrostatic interactions between molecules depend strongly on their relative orientation, which manifests as a rotational state dependence. Interactions between molecules in the same rotational quantum state are well-known…

原子物理 · 物理学 2024-05-16 Etienne F. Walraven , Tijs Karman

We consider collisions of electric and magnetic polar molecules, taking the OH radical as an example, subject to combined electric and magnetic static fields. We show that the relative orientation of the fields has an important effect on…

原子物理 · 物理学 2013-07-16 Goulven Quéméner , John L. Bohn

Collisions of polar $^{1}\Sigma$ state molecules at ultralow energies are considered, within a model that accounts for long-range dipole-dipole interactions, plus rotation of the molecules. We predict a substantial suppression of…

原子物理 · 物理学 2016-09-08 Alexander V. Avdeenkov , Masatoshi Kajita , John L. Bohn

The ability to tune interparticle interactions is one of the main advantages of using ultracold quantum gases for quantum simulation of many-body physics. Current experiments with ultracold polar molecules employ shielding with microwave or…

量子气体 · 物理学 2026-03-24 Christopher J. Ho , Joy Dutta , Bijit Mukherjee , Jeremy M. Hutson , Michael R. Tarbutt

We show that a ferro-electric quantum phase transition can be driven by the dipolar interaction of polar molecules in the presence a micro-wave field. The obtained ferro-electricity crucially depends on the harmonic confinement potential,…

量子气体 · 物理学 2015-05-13 Chien-Hung Lin , Yi-Ting Hsu , Hao Li , Daw-Wei Wang

We investigate the ultracold collisions of rotationally excited dipolar molecules in free-space, taking the hetero-nuclear bi-alkali molecule of KRb as an example. We show that we can sharply tune the elastic, inelastic and reactive rate…

原子物理 · 物理学 2015-03-31 Gaoren Wang , Goulven Quéméner

We examine the potential-energy curves and polarization of the dipole moments of two static polar molecules under the influence of an external dc electric field and their anisotropic dipole-dipole interaction. We model the molecules as…

量子物理 · 物理学 2024-09-24 Felipe Isaule , Robert Bennett , Jörg B. Götte

The collisions between linear polar molecules, trapped in a microwave field with circular polarization, are theoretically analyzed. The microwave trap suggested by DeMille \cite{DeMille} seems to be rather advantageous in comparison with…

原子物理 · 物理学 2015-05-13 Alexander V. Avdeenkov

Elastic scattering resonances occurring in ultracold collisions of either bosonic or fermionic polar molecules are investigated. The Born-Oppenheimer adiabatic representation of the two-bodydynamics provides both a qualitative…

原子与分子团簇 · 物理学 2009-11-13 V. Roudnev , M. Cavagnero

We calculate the microwave spectra of ultracold KRb alkali metal dimers, including hyperfine interactions and in the presence of electric and magnetic fields. We show that microwave transitions may be used to transfer molecules between…

化学物理 · 物理学 2015-05-13 J. Aldegunde , Hong Ran , Jeremy M. Hutson
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