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The light-mediated interaction of fermionic and bosonic excitations governs the optoelectronic properties of condensed matter systems. In photoexcited semiconductors, the coupling of electron-hole pairs (excitons) to coherent optical…

The interaction of excitons with lattice vibrations underlies the scattering from bright to dark excitons as well as the coherent modulation of the exciton energy. Unlike the former mechanism, which involves phonons with finite momentum,…

介观与纳米尺度物理 · 物理学 2024-06-24 Enrico Perfetto , Kai Wu , Gianluca Stefanucci

Atomically thin semiconductors exhibit tunable exciton resonances that can be harnessed for dynamic manipulation of visible light in ultra-compact metadevices. However, the rapid nonradiative decay and dephasing of excitons at room…

光学 · 物理学 2025-02-18 Tom Hoekstra , Jorik van de Groep

We discuss how excitons can affect the generation of coherent radial breathing modes in ultrafast spectroscopy of single wall carbon nanotubes. Photoexcited excitons can be localized spatially and give rise to a spatially distributed…

Controlled non-local energy and coherence transfer enables light harvesting in photosynthesis and non-local logical operations in quantum computing. The most relevant mechanism of coherent coupling of distant qubits is coupling via the…

We study the dynamics of excitonic insulators coupled to phonons. Without phonon couplings, the linear response is given by the damped amplitude oscillations of the order parameter with frequency equal to the minimum band gap. A phonon…

强关联电子 · 物理学 2017-12-19 Yuta Murakami , Denis Golež , Martin Eckstein , Philipp Werner

We employ quasiparticle path integral molecular dynamics to study how the excitonic properties of model semiconductors are altered by electron-phonon coupling. We describe ways within a path integral representation of the system to evaluate…

材料科学 · 物理学 2022-09-28 Yoonjae Park , David T. Limmer

We investigate the excitation of phonons in photoexcited antimony and demonstrate that the entire electron-lattice interactions, in particular coherent and incoherent electron-phonon coupling, can be probed simultaneously. Using femtosecond…

We study theoretically the radiative recombination of excitons in double quantum dots in the presence of carrier-phonon coupling. We show that the phonon-induced pure dephasing effects and transitions between the exciton states strongly…

介观与纳米尺度物理 · 物理学 2012-01-20 Pawel Karwat , Anna Sitek , Pawel Machnikowski

Exciton-photon hybridization is typically realised in geometrically defined optical cavities, where tunability is achieved by modifying either the cavity or the excitonic medium. Here we investigate transition-radiation interferences in…

Coupling to phonon modes is a primary mechanism of excitonic dephasing and energy loss in semiconductors. However, low-energy phonons in colloidal quantum dots and their coupling to excitons are poorly understood, since their experimental…

介观与纳米尺度物理 · 物理学 2019-10-22 Albert Liu , Diogo B. Almeida , Wan-Ki Bae , Lazaro A. Padilha , Steven T. Cundiff

Metasurfaces enable flat optical elements by leveraging optical resonances in metallic or dielectric nanoparticles to obtain accurate control over the amplitude and phase of the scattered light. While highly efficient, these resonances are…

光学 · 物理学 2022-09-07 Jason Lynch , Ludovica Guarneri , Deep Jariwala , Jorik van de Groep

We provide a self-contained review of master equation approaches to modelling phonon effects in optically driven self-assembled quantum dots. Coupling of the (quasi) two-level excitonic system to phonons leads to dissipation and dephasing,…

介观与纳米尺度物理 · 物理学 2016-06-14 Ahsan Nazir , Dara P. S. McCutcheon

Optical excitation and control of excitonic wavepackets in organic molecules is the basis to energy conversion processes. To gain insights into such processes, it is essential to establish the relationship between the coherence timescales…

The way nuclear motion affects electronic responses has become a very hot topic in materials science. Coherent acoustic phonons can dynamically modify optical, magnetic and mechanical properties at ultrasonic frequencies, with promising…

介观与纳米尺度物理 · 物理学 2018-08-29 Edoardo Baldini , Tania Palmieri , Adriel Dominguez , Pascal Ruello , Angel Rubio , Majed Chergui

Here we show how time-resolved broadband optical spectroscopy can be used to quantify, with femtometer resolution, the oscillation amplitudes of coherent phonons through a displacive model without free tuning parameters, except an overall…

材料科学 · 物理学 2020-10-08 Davide Soranzio , Maria Peressi , Robert J. Cava , Fulvio Parmigiani , Federico Cilento

The strong confinement of semiconductor excitons in a quantum dot gives rise to atom-like behavior. The full benefit of such a structure is best observed in resonant excitation where the excited state can be deterministically populated and…

The effects of the electron-phonon interaction on optical excitations can be understood in terms of exciton-phonon coupling, and require a careful treatment in low-dimensional materials with strongly bound excitons or strong electron-hole…

材料科学 · 物理学 2022-02-17 Gabriel Antonius , Steven G. Louie

Actively tunable photonic devices are vital for next-generation optoelectronics requiring rapid switching and high bandwidth. Although organic optoelectronic devices have found wide application, their use as optical modulators has been…

The measurement and manipulation of the coherent dynamics of excitonic states constitute a forefront research challenge in semiconductor optics and in quantum coherence-based protocols for optoelectronic technologies. Layered semiconductors…

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