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We demonstrate coherent control of multiphoton and above-threshold photoemission from a single solid-state nanoemitter driven by a fundamental and a weak second harmonic laser pulse. Depending on the relative phase of the two pulses,…

When two-color femtosecond laser pulses interact with matter, electrons can be emitted through various multiphoton excitation pathways. Quantum interference between these pathways gives rise to a strong oscillation of the photoemitted…

光学 · 物理学 2022-05-24 Ang Li , Yiming Pan , Philip Dienstbier , Peter Hommelhoff

We report on a quantitative measurement of the spatial coherence of electrons emitted from a sharp metal needle tip. We investigate the coherence in photoemission using near-ultraviolet laser triggering with a photon energy of 3.1 eV and…

In this article we present coherent control of above-threshold photoemission from a tungsten nanotip achieving nearly perfect modulation. Depending on the pulse delay between fundamental (1560 nm) and second harmonic (780 nm) pulses of a…

We investigate the process of phase-controlled high-order above-threshold photoemission from sharp metallic nanotips under bichromatic laser fields. Experimental photoelectron spectra resulting from two-color excitation with a moderately…

原子物理 · 物理学 2018-07-04 Lennart Seiffert , Timo Paschen , Peter Hommelhoff , Thomas Fennel

Coherent control of interfering one- and two-photon processes has for decades been the subject of research to achieve the redirection of photocurrent. The present study develops two-pathway coherent control of ground state helium atom…

原子物理 · 物理学 2021-06-02 Yimeng Wang , Chris H. Greene

Two-color multiphoton emission from polycrystalline tungsten nanotips has been demonstrated using two-color laser fields. The two-color photoemission is assisted by a three-photon multicolor quantum channel, which leads to a twofold…

量子物理 · 物理学 2021-05-18 Wayne Cheng-Wei Huang , Maria Becker , Joshua Beck , Herman Batelaan

Irradiation of sharp silver tips with femtosecond laser pulses leads to photoassisted coherent field emission without a static field. We reconstruct the time profile of the emission, and show that the process is entirely governed by the…

We comprehensively investigate two-color-laser-driven photocurrent and high harmonic generation (HHG) in graphene models. By numerically solving the quantum master equation, we uniformly explore a broad parameter regime including both the…

介观与纳米尺度物理 · 物理学 2025-07-10 Minoru Kanega , Masahiro Sato

We report a new method of two-pathway coherent control using three narrow-band cw laser sources, phase locked in an optical phase-lock loop, to maintain the high degree of optical coherence required for the coherent control process. In…

原子物理 · 物理学 2026-01-16 Jonah A. Quirk , Carol E. Tanner , D. S. Elliott

We demonstrate a left-right asymmetry control of the photo\-electron angular distribution in multi\-photon ionization of Li atoms by a bichromatic laser field. By delaying the fundamental (780 nm) and its second harmonic relative to each…

原子物理 · 物理学 2024-05-20 Silva Mezinska , Alexander Dorn , Thomas Pfeifer , Klaus Bartschat

We demonstrate optical coherent control of the emission direction of THz radiation. Femtosecond laser pulses are used to excite different types of ultrafast photocurrents along different directions in a bulk GaAs sample. The overall…

光学 · 物理学 2013-08-06 Heiko Füser , Mark Bieler

We experimentally demonstrate the coherent control, i.e., phase-dependent enhancement and suppression, of the optical absorption in an array of metallic nanoantennas covered by a thin lu- minescent layer. The coherent control is achieved by…

In this work, we investigate the generation of second harmonic light by gold nanorods and demonstrate that the collected nonlinear intensity depends upon a phase interplay between different modes available in the nanostructure. By recording…

Though interference from different emission channels enabled a deeper understanding of strong-field photoemission in atoms and molecules, it remained out of reach for solids. Here, we explore metal needle tips under single-cycle pulses via…

By studying the fluorescence and optical properties of a three-level system, we propose a new point of view on the coherent control of these spectra. With the definite phase difference between the fields of the air band and dielectric band…

材料科学 · 物理学 2009-11-13 Szu-Cheng Cheng , Jing-Nuo Wu , Tzong-Jer Yang , Wen-Feng Hsieh

Strong-field photoemission from nanostructures and the associated temporally modulated currents play a key role in the development of ultrafast vacuum optoelectronics. Optical light fields could push their operation bandwidth into the…

We present a new technique based on two-pathway optical coherent control for the sensitive detection and precise measurement of highly-forbidden transitions in atomic systems. Specifically, we show that ($\omega$, 2$\omega$) coherent…

原子物理 · 物理学 2010-01-15 D. Antypas , D. S. Elliott

We describe optimized coherent control methods for two-photon transitions in atoms of a ladder-type three-state energy configuration. Our approach is based on the spatial coherent control scheme which utilizes counter-propagating ultrashort…

原子物理 · 物理学 2015-10-28 Woojun Lee , Hyosub Kim , Kyungtae Kim , Jaewook Ahn

We propose and demonstrate a technique to control the balance between the two amplitudes of a dual-wavelength laser based on a phase-controlled optical feedback. The feedback cavity length is adjusted to achieve a relative phase shift…

光学 · 物理学 2022-07-04 Robert Pawlus , Stefan Breuer , Martin Virte
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