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Operando microscopy has unveiled key mechanistic insights in battery materials during early cycling, but long-term characterization to unveil material evolution, degradation, and failure remain limited. To address this gap, we develop a…

Nuclear magnetic resonance (NMR) investigations of electrochemical systems require gas-tight and non-metallic cell housings. This contribution reports on the development and evaluation of a cylindrical battery container in combination with…

The rapid pace of replacing fossil fuel propelled transport by electric vehicles is critically dependent on high-performing, high energy density and efficient batteries. Optimal and safe use of existing battery cells and development of…

Capacity degradation of lithium-ion batteries under long-term cyclic aging is modelled via a flexible sigmoidal-type regression set-up, where the regression parameters can be interpreted. Different approaches known from the literature are…

应用统计 · 统计学 2019-07-31 Marcus Johnen , Simon Pitzen , Udo Kamps , Maria Kateri , Dirk Uwe Sauer

The reliability and safety of Lithium-ion batteries (LiBs) are of great concern in the energy storage industry. Nevertheless, the real-time monitoring of their degradation remains challenging due to limited quantitative metrics available…

We present a refined Mn-Zn-H$_2$O Pourbaix diagram with the emphasis on parameters relevant for the Zn/MnO$_2$ rechargeable cells. It maps out boundaries of electrochemical stability for MnO$_2$, ZnMn$_2$O$_4$, ZnMn$_3$O$_7$, and MnOOH. The…

Herein, in-situ reduction of bismuth and graphene oxide was performed by a solvothermal method under a nitrogen atmosphere, and the resulting Bi on RGO nanocomposites were used as an anode material for Mg-ion batteries. The nanocomposite of…

As global energy demands escalate, and the use of non-renewable resources become untenable, renewable resources and electric vehicles require far better batteries to stabilize the new energy landscape. To maximize battery performance and…

Si-anodes have long been candidates thanks to an expected ten-fold increase in capacity compared to graphite. However, details of the mechanisms governing their degradation remain elusive, hindering science-guided development of long-lived…

Zinc-ion batteries are promising alternatives to lithium-ion batteries, offering advantages in safety, cost, and environmental impact. However, their performance is often limited by the functioning of the zinc anode. This study employs…

材料科学 · 物理学 2025-03-31 Xinxin Hu , Shivam Dangwal , Xucheng Wang , Fan Zhang , Haijuan Kong , Jun Li , Kaveh Edalati

Metal-air batteries are among the most promising next-generation energy storage devices. Relying on abundant materials and offering high energy densities, potential applications lie in the fields of electro-mobility, portable electronics,…

化学物理 · 物理学 2017-06-15 Johannes Stamm , Alberto Varzi , Arnulf Latz , Birger Horstmann

The properties of porous glasses and their field of application strongly depend on the characteristics of the void space. Understanding the relationship between their porous structure and failure behaviour can contribute to the development…

"Anode-free" lithium-metal batteries promise significantly higher energy density than conventional graphite-based lithium-ion batteries; however, lithium dendrite growth can lead to internal short circuits with associated safety risks.…

Reliable early detection of lithium-ion battery degradation requires health indicators that are physically interpretable and computable from routine cycler telemetry without access to the degradation region. We introduce…

材料科学 · 物理学 2026-05-19 Dieter W. Heermann , Hagen Heermann

Lithium-ion batteries are recognised as a key technology to power electric vehicles and integrate grid-connected renewable energy resources. The economic viability of these applications is affected by the battery degradation during its…

应用物理 · 物理学 2020-07-07 Ahmed Gailani , Rehab Mokidm , Moaath El-Dalahmeh , Maad El-Dalahmeh , Maher Al-Greer

Silicon is a promising anode material for next-generation lithium-ion batteries due to its exceptionally high specific capacity (3600 mAh g$^{-1}$), significantly exceeding that of conventional graphite. However, its practical application…

化学物理 · 物理学 2026-01-08 D Sugunan , Y Jiang , J Guo , H Wang , M Marinescu , G Offer

Accurate tracking of the internal electrochemical states of lithium-ion battery during cycling enables advanced battery management systems to operate the battery safely and maintain high performance while minimizing battery degradation. To…

系统与控制 · 电气工程与系统科学 2020-10-01 Sravan Pannala , Puneet Valecha , Peyman Mohtat , Jason B. Siegel , Anna G. Stefanopoulou

Next-generation lithium-ion batteries with silicon anodes have positive characteristics due to higher energy densities compared to state-of-the-art graphite anodes. However, the large volume expansion of silicon anodes can cause high…

数值分析 · 数学 2024-04-03 R. Schoof , G. F. Castelli , W. Dörfler

Accurately predicting the future health of batteries is necessary to ensure reliable operation, minimise maintenance costs, and calculate the value of energy storage investments. The complex nature of degradation renders data-driven…

应用统计 · 统计学 2020-06-05 Robert R. Richardson , Michael A. Osborne , David A. Howey

This work presents an effective state of health indicator to indicate lithium-ion battery degradation based on a long short-term memory (LSTM) recurrent neural network (RNN) coupled with a sliding-window. The developed LSTM RNN is able to…

系统与控制 · 电气工程与系统科学 2022-05-17 Kotub Uddin , James Schofield , W. Dhammika Widanage