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Cubic gauche polynitrogen (cg-N) is an attractive high-energy density material. However, high-pressure synthesized cg-N will decompose at low-pressure and cannot exist at ambient conditions. Here, the stabilities of cg-N surfaces with and…

材料科学 · 物理学 2024-12-02 Guo Chen , Caoping Niu , Wenming Xia , Jie Zhang , Zhi Zeng , Xianlong Wang

We theoretically investigate the temperature dependence of the reversible structural relaxation time and diffusion constant of metallic glasses under pressure. The compression not only changes the glassy dynamics, but also generates a…

材料科学 · 物理学 2021-05-28 Nguyen K. Ngan , Anh D. Phan , Alessio Zaccone

Sought-after ordered structures of mixtures of hard anisotropic nanoparticles can often be thermodynamically unfavorable due to the components' geometric incompatibility to densely pack into regular lattices. A simple compatibilization rule…

软凝聚态物质 · 物理学 2014-10-22 Mihir R. Khadilkar , Fernando A. Escobedo

The manipulation of microparticles using optical forces has led to many applications in the life and physical sciences. To extend optical trapping towards the nano-regime, in this work we demonstrate trapping of single nanoparticles in…

Solid-state nanofoaming experiments are conducted on two PMMA grades of markedly different molecular weight using CO$_2$ as the blowing agent. The sensitivity of porosity to foaming time and foaming temperature is measured. Also, the…

The impact of shear deformation in $(1\,0\,1)[1\,0\,\bar{1}]$ system of non-modulated (NM) martensite in Ni$_2$MnGa ferromagnetic shape memory alloy is investigated by means of ab initio atomistic simulations. The shear system is associated…

材料科学 · 物理学 2024-11-11 Martin Heczko , Petr Šesták , Hanuš Seiner , Martin Zelený

In this paper, a micro-mechanical model is introduce to characterize the stress softening phenomenon in double network hydrogels. Damage in polymer matrices under deformation, which appears as the rupture of cross-linking, is assumed to…

应用物理 · 物理学 2017-12-22 İsmail Doğan Külcü , Roozbeh Dargazany

Applying pressure around megabar is indispensable in the synthesis of high-temperature superconducting hydrides, such as SH$_3$ and LaH$_{10}$. Stabilizing the high-pressure phase of hydride around ambient condition is a severe challenge.…

超导电性 · 物理学 2023-05-17 Miao Gao , Peng-Jie Guo , Huan-Cheng Yang , Xun-Wang Yan , Fengjie Ma , Zhong-Yi Lu , Tao Xiang , Hai-Qing Lin

Carbon monoxide and nitrogen are among the potentially interesting high-energy density materials. However, in spite of the physical similarities of the molecules, they behave very differently at high pressures. Using density functional…

材料科学 · 物理学 2013-12-06 Zamaan Raza , Chris J. Pickard , Carlos Pinilla , A. Marco Saitta

Optical and synchrotron x-ray diffraction diamond anvil cell experiments have been combined with first principles theoretical structure predictions to investigate mixed N2 and H2 up to 55 GPa. We found the formation of oligomeric NxH (x>1)…

Self-assembling novel ordered structures with nanoparticles has recently received much attention. Here we use computer simulations to study a two-dimensional model system characterized by a simple isotropic interaction that could be…

软凝聚态物质 · 物理学 2015-03-18 Michael Engel

Dynamic nuclear polarization (DNP) of molecules in a solution at room temperature has potential to revolutionize nuclear magnetic resonance spectroscopy and imaging. The prevalent methods for achieving DNP in solutions are typically most…

化学物理 · 物理学 2016-03-02 Qiong Chen , Ilai Schwarz , Fedor Jelezko , Alex Retzker , Martin B Plenio

Germanium is an extremely important material used for numerous functional applications in many fields of nanotechnology. In this paper, we study the crystallization of amorphous Ge using atomistic simulations of critical nano-metric nuclei…

材料科学 · 物理学 2015-07-15 Luis A. Sandoval , Celia Reina , Jaime Marian

We analyze the transport properties of a low density ensemble of identical macroscopic particles immersed in an active fluid. The particles are modeled as inelastic hard spheres (granular gas). The non-homogeneous active fluid is modeled by…

软凝聚态物质 · 物理学 2017-10-17 Francisco Vega Reyes , Antonio Lasanta

We investigate the collective behavior of suspended thermoresponsive microgels, that expel solvent and subsequently decrease in size upon heating. Using a binary mixture of differently thermoresponsive microgels, we demonstrate how…

A physical mechanism has been proposed to describe the formation of a stable state of a nonwetting liquid after filling of a porous medium at an increased pressure with the subsequent reduction of the overpressure to zero. It has been shown…

统计力学 · 物理学 2016-03-04 V. D. Borman , A. A. Belogorlov , V. A. Byrkin , V. N. Tronin , V. I. Troyan

The study of materials behavior under extreme conditions is fundamental to science and modern technology. Fast ramp compression is a unique method for exploring materials behavior and phase transformations under extreme conditions. One…

材料科学 · 物理学 2026-03-04 Daria A. Komkova , Alexey Yu. Volkov , Evgeny F. Talantsev

While largely studied on the macroscopic scale, the dynamics leading to nucleation and fission processes in atmospheric aerosols are still poorly understood at the molecular level. Here, we present a joint experimental-theoretical study of…

The reformulation of the mode-coupling theory (MCT) of the liquid-glass transition which incorporates the element of metastability is applied to the hard-sphere system. It is shown that the glass transition in this system is not a sharp one…

凝聚态物理 · 物理学 2016-08-31 Joonhyun Yeo

Understanding the crystallization pathways of water-rich ammonia-water (NH3-H2O) solutions and the stability of ammonia hydrates is key to unraveling the behavior of complex hydrogen-bonding networks as well as for planetary interior…