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The delafossite-like compound NaYbO$_2$ hosts a triangular lattice of Yb$^{3+}$ moments and is a promising candidate for the realization of a quantum spin liquid ground state -- an exotic, quantum-disordered magnetic phase featuring…

We present the low-temperature magnetic properties of two Yb$^{3+}$-based triangular lattice compounds NaSrYb(BO$_3$)$_2$ and K$_3$YbSi$_2$O$_7$ via thermodynamic measurements followed by crystal electric field (CEF) calculations.…

材料科学 · 物理学 2025-01-27 S. Guchhait , R. Kolay , A. Magar , R. Nath

We present the structural characterization and low-temperature magnetism of the triangular-lattice delafossite NaYbO$_2$. Synchrotron x-ray diffraction and neutron scattering exclude both structural disorder and crystal-electric-field…

The magnetic properties of $\alpha$-NaFeO$_2$ are studied by neutron diffraction and magnetization measurements. An ordered phase with spins aligned along the b$_hex$ axis exists at low temperatures (T < 4 K). At intermediate temperatures…

强关联电子 · 物理学 2009-02-02 T. M. McQueen , Q. Huang , J. W. Lynn , R. F. Berger , T. Klimczuk , B. G. Ueland , P. Schiffer , R. J. Cava

In this paper we report low-temperature magnetic properties of the rare-earth perovskite material YbAlO$_3$. Results of elastic and inelastic neutron scattering experiment, magnetization measurements along with the crystalline electrical…

Yb- and Ce-based delafossites were recently identified as effective spin-1/2 antiferromagnets on the triangular lattice. Several Yb-based systems, such as NaYbO2, NaYbS2, and NaYbSe2, exhibit no long-range order down to the lowest measured…

In this comprehensive study, we present results of bulk measurements (magnetization, specific heat, ac susceptibility, thermal expansion, and magnetostriction) combined with local methods such as nuclear magnetic resonance (^23Na NMR) and…

The interplay of magnetic correlations, crystal electric field interactions, and spin-orbit coupling in low-dimensional frustrated magnets fosters novel ground states with unusual excitations. Here, we report the magnetic properties and…

材料科学 · 物理学 2024-09-02 S. Guchhait , A. Painganoor , S. S. Islam , J. Sichelschmidt , M. D. Le , N. B. Christensen , R. Nath

Rare-earth chalcogenide compounds $\mathrm{ARECh_2}$ (A = alkali or monovalent metal, RE = rare earth, Ch = O, S, Se, Te) are a large family of quantum spin liquid (QSL) candidate materials. $\mathrm{NaYbS_2}$ is a representative member of…

强关联电子 · 物理学 2024-09-25 Weizhen Zhuo , Zheng Zhang , Mingtai Xie , Anmin Zhang , Jianting Ji , Feng Jin , Qingming Zhang

The subtle interplay between competing degrees of freedom, crystal electric fields, and spin correlations can lead to exotic quantum states in 4f ion-based frustrated triangular lattice antiferromagnets. We present the crystal structure,…

We report crystal structure and magnetic behavior of the triangular antiferromagnet KYbO$_2$, the A-site substituted version of the quantum spin liquid candidate NaYbO$_2$. The replacement of Na by K introduces an anisotropic tensile strain…

While the Heisenberg model for magnetic Mott insulators on planar lattice structures is comparatively well understood in the case of transition metal ions, the intrinsic spin-orbit entanglement of 4f magnetic ions on such lattices shows…

强关联电子 · 物理学 2021-06-29 B. Schmidt , J. Sichelschmidt , K. M. Ranjith , Th. Doert , M. Baenitz

The magnetocaloric effect in the quantum dipolar magnet Yb$_3$Ga$_5$O$_{12}$ is studied both for pure material and with non-magnetic substitution: (Yb$_{1-x}$Y$_x$)$_3$Ga$_5$O$_{12}$. Magnetization measurements have been performed on a…

材料科学 · 物理学 2026-03-24 E. Riordan , E. Lhotel , N. -R. Camara , C. Marin , M. E. Zhitomirsky

In this article, the Curie-Weiss type behavior and the appearance of an "interaction" or "ordering" temperature for a collection of magnetic nanoparticles is explored theoretically. We show that some systems where an interaction temperature…

材料科学 · 物理学 2024-10-25 Robert E Camley , Rair Macêdo , Karen L Livesey

We calculate the Curie temperature of layered ferromagnets, chromium tri-iodide (CrI3), chromium tri-bromide (CrBr3), chromium germanium tri-telluride (CrGeTe3), and the Neel temperature of a layered anti-ferromagnet iron di-chloride…

介观与纳米尺度物理 · 物理学 2021-01-27 Sabyasachi Tiwari , Maarten L Van de Put , Bart Soree , William G. Vandenberghe

Antiferromagnetically coupled S=1/2 spins on an isotropic triangular lattice is the paradigm of frustrated quantum magnetism, but structurally ideal realizations are rare. Here we investigate NaYbO$_2$, which hosts an ideal triangular…

Perovskite structure SrMnO$_3$ is a rare example of a multiferroic material where strain-tuning and/or cation substitution could lead to coinciding magnetic and ferroelectric ordering temperatures, which would then promise strong…

材料科学 · 物理学 2018-10-24 Alexander Edström , Claude Ederer

Layered rare-earth delafossites $ARX_2$ with $R$ = Yb(III) or Ce(III) have received a lot of interest as potential hosts for a quantum spin-liquid ground state. Some systems of this family that show no long-range order down to the lowest…

强关联电子 · 物理学 2022-12-26 S. M. Avdoshenko , A. A. Kulbakov , E. Häußler , P. Schlender , Th. Doert , J. Ollivier , D. S. Inosov

We present a neutron diffraction study of NaYbO$_2$, a candidate quantum spin liquid compound hosting a geometrically frustrated triangular lattice of magnetic Yb$^{3+}$ ions. We observe diffuse magnetic scattering that persists to at least…

Crystal and magnetic structures of $R_2$Ni$_2$In ($R$ = Tb and Ho) have been studied by powder neutron diffraction at low temperatures. The compounds crystallize in an orthorhombic crystal structure of the Mn$_2$AlB$_2$-type. At low…

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