相关论文: Triple-$q$ quadrupole-octupole order scenario for …

We report the results of 27Al-NMR measurements on a single crystal of PrTi2Al20. This compound shows a phase transition near 2 K associated with the quadrupole degree of freedom of Pr ions, for which the ground state of the crystalline…

Ferro-quadrupole (FQ) order in the non-Kramers $\Gamma_3$ doublet system PrTi$_2$Al$_{20}$ has been investigated via angle-resolved measurements of the specific heat, rotational magnetocaloric effect, and entropy, under a rotating magnetic…

We investigate antiferro quadrupole orders in systems with non-Kramers doublet ground state with total angular momentum J=4 in T_d point group symmetry. We demonstrate that a pure O_2^2 antiferro quadrupole order is impossible in general…

We report magnetic-field-induced first-order phase transitions in the ferro-quadrupole (FQ) ordered state of PrTi2Al20, in which non-Kramers Pr3+ ions with two 4f electrons have a non-magnetic Gamma3 doublet ground state in the cubic Td…

We study $\Gamma_3$ quadrupole orders in a face-centered cubic lattice. The $\Gamma_3$ quadrupole moments under cubic symmetry possess a unique cubic invariant in their free energy in the uniform ($q=0$) sector and the triple-q sector for…

We performed field-angle-resolved magnetostriction and thermal-expansion measurements on PrIr$_2$Zn$_{20}$, a cubic non-Kramers compound exhibiting antiferroquadrupolar order below $T_{\rm Q}=0.125$ K. Thermal expansion exhibits two…

We theoretically investigate possible symmetry-broken states in ${\rm UNi_4B}$, constructing a localized pseudo triplet crystalline-electric field model. For a long time, its low-temperature symmetry-broken phase in ${\rm UNi_4B}$ has been…

Detecting symmetry-breaking hidden orders with conventional probes has been a long-standing challenge in the field of magnetism. Higher-rank multipolar ordering $-$ anisotropic charge and magnetization distributions arising from a…

A series of Pr(TM)$_2$X$_{20}$ (with TM=Ti,V,Rh,Ir and X=Al,Zn) Kondo materials, containing non-Kramers Pr$^{3+}$ $4f^2$ moments on a diamond lattice, have been shown to exhibit intertwined orders such as quadrupolar order and…

Our single crystal study reveals that PrTr2Al20 (Tr = Ti and V) provides the first examples of a cubic {\Gamma}3 nonmagnetic ground doublet system that shows the Kondo effect including a -ln T dependent resistivity. The {\Gamma}3…

Quadrupole ordering with the ordering wavevector at the L points in PrIr$_2$Zn$_{20}$ under magnetic fields is analyzed using classical Monte Carlo simulations based on an effective $\Gamma_3$ quadrupole model on the diamond structure. We…

We study quadrupole orders in heavy-fermion compound PrIr$_2$Zn$_{20}$ under magnetic fields on the basis of the Landau theory. Assuming $E_g$ electric quadrupolar orders in the cubic symmetry with the ordering wavenumber at the L points in…

Motivated by the time-reversal symmetry breaking signal in muon spin relaxation below a transition temperature without accompanying noticeable magnetic Bragg peaks in $5d^2$ Os double perovskites, a rare ferro-octupolar order was proposed…

We theoretically study electric quadrupole orders in f-electron systems on the fcc lattice. Qudrupole degrees of freedom $O_{20}$ and $O_{22}$ originate in the non-Kramers doublet ground state $\Gamma_3$ of ion with $f^2$ electron…

Neutron diffraction measurements have been performed on the cubic compound PrPb3 in a [001] magnetic field to examine the quadrupolar ordering. Antiferromagnetic components with q=(1/2+-d 1/2 0), (1/2 1/2+-d 0) (d~1/8) are observed below…

Among heavy fermion materials, there is a set of rare-earth intermetallics with non-Kramers Pr$^{3+}$ $4f^2$ moments which exhibit a rich phase diagram with intertwined quadrupolar orders, superconductivity, and non-Fermi liquid behavior.…

Higher-rank electric/magnetic multipole moments are attracting attention these days as candidate order parameters for exotic material phases. However, quantum-mechanical formulation of those multipole moments is still an ongoing issue. In…

The nature of multiple electronic orders in skutterudite PrFe_4P_{12} is discussed on the basis of a model with antiferro-quadrupole (AFQ) interaction of \Gamma_3 symmetry. The high-field phase can be reproduced qualitatively provided (i)…

We investigate effects of multipole moments in f-electron systems both from phenomenological and microscopic viewpoints. First, we discuss significant effects of octupole moment on the magnetic susceptibility in a paramagnetic phase. It is…

In the electromagnetic multipole expansion, magnetic octupoles are the subsequent order of magnetic multipoles allowed in centrosymmetric systems, following the more commonly observed magnetic dipoles. As order parameters in condensed…