相关论文: A custom-tailored multi-TW optical electric field …
A stable 50 mJ three-channel optical waveform synthesizer is demonstrated and used to reproducibly generate a high-order harmonics supercontinuum in the soft-x-ray region. This synthesizer is composed of pump pulses from a…
The generation of gigawatt-class isolated attosecond pulses (IAPs) is vital for attosecond pump-probe experiments. In such experiments, the temporal duration of IAPs must be determined quickly and accurately. In this study, we developed a…
Probing coherent quantum dynamics in light-matter interactions at the microscopic level requires high-repetition-rate isolated attosecond pulses (IAPs) in pump-probe experiments. To date, the generation of IAPs has been mainly limited to…
Isolated attosecond pulses (IAPs) produced through laser-driven high-harmonic generation (HHG) hold promise for unprecedented insight into biological processes via attosecond x-ray diffraction with tabletop sources. However, efficient…
We report theoretical calculations of high-order harmonic generation (HHG) of Xe with the inclusion of multi-electron effects and macroscopic propagation of the fundamental and harmonic fields in an ionizing medium. By using the…
Generation of ultrabroadband isolated attosecond pulses (IAPs) is essential for time-resolved applications in chemical and material sciences, as they have the potential to access the spectral water window region of chemical elements, which…
Attosecond pulse trains (APTs) are indispensable for probing electron dynamics at their intrinsic timescales. High harmonic generation (HHG) has long been a successful and widely used technique in producing extreme ultraviolet APTs. While…
High-order harmonic generation (HHG) arising from the non-perturbative interaction of intense light fields with matter constitutes a well-established tabletop source of coherent extreme-ultraviolet and soft X-ray radiation, which is…
Isolated attosecond pulses (IAP) generated by high-order harmonic generation are valuable tools that enable dynamics to be studied on the attosecond time scale. The applicability of these IAP would be widened drastically by increasing their…
High-order harmonic generation (HHG) provides a broad spectral bandwidth for synthesizing attosecond pulses. However, in the current HHG schemes, only part of the harmonics can be phase-locked, which limits the ability to achieve shorter…
An all-optical method for directly reconstructing the spectral phase of isolated attosecond pulse (IAP) has been proposed recently [New J. Phys. 25, 083003 (2023)]. This method is based on the high-harmonic generation (HHG) streaking…
The generation of attosecond pulses (1 as=10-18 s) has enabled real-time observation and manipulation of coherent electron dynamics, yet their low peak power has hindered the development of advanced attosecond pump-probe spectroscopy and…
Isolated attosecond pulses (IAPs) generated by few-cycle femtosecond lasers are essential for capturing ultrafast dynamics in atoms, molecules, and solids. Nonetheless, the advancement of attosecond science critically depends on achieving…
Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: higher photon flux (permitting…
We present experimental results showing the appearance of a near-continuum in the high-order harmonic generation (HHG) spectra of atomic and molecular species as the driving laser intensity of an infrared pulse increases. Detailed…
The mechanism underlying high harmonic generation (HHG) in gases has been well clarified, characterizing attosecond pulse trains (APT) in the time domain, significantly advances the synthesis of isolated attosecond pulse (IAP). However, the…
The generation of terawatt (TW) near-single-cycle laser pulses is of high interest for applications including attosecond science. Here we demonstrate a three-stage post-compression scheme in a non-guided geometry using He as the nonlinear…
We have produced a soft x-ray supercontinuum with a pulse energy of 0.24-$\mu$J using high-order harmonics from a multiterawatt, 10-Hz, stable, three-channel waveform synthesizer [Sci. Adv. eaay2802 (2020)]. We report here an attosecond…
We theoretically investigate high-order harmonic generation (HHG) and its ellipticity in gapped graphene, driven by a femtosecond short-pulse laser at various orientation angles, employing the two-band density-matrix equations within the…
The conventional way of generating optical waveforms relies on the in-phase and quadrature (IQ) modulation of a continuous wave (CW) laser tone. In this case, the bandwidth of the resulting optical waveform is limited by the underlying…