相关论文: Engineering long-lived vibrational states for an o…
Molecules constitute compact hybrid quantum optical systems that can interface photons, electronic degrees of freedom, localized mechanical vibrations and phonons. In particular, the strong vibronic interaction between electrons and nuclear…
We have investigated the phonon dynamics of a single-molecule embedded in a mechanical resonator made of an organic crystal. The whole system is placed in an optical resonator within the bad cavity limit. We have found that the optical…
We propose an optomechanical scheme for reaching quantum entanglement in vibration polaritons. The system involves $N$ molecules, whose vibrations can be fairly entangled with plasmonic cavities. We find that the vibration-photon…
The conventional explanation of plasmon-enhanced Raman scattering attributes the enhancement to the antenna effect focusing the electromagnetic field into sub-wavelength volumes. Here we introduce a new model that additionally accounts for…
Cavity optomechanics aims to establish optical control over vibrations of mechanical systems, to heat, cool or to drive them toward coherent, or nonclassical states. This field was recently extended to include molecular optomechanics, which…
This chapter reviews the fundamental optical properties and applications of pho-tonic molecules (PMs) - photonic structures formed by electromagnetic coupling of two or more optical microcavities (photonic atoms). Controllable interaction…
Molecular optomechanics stems from the description of Raman scattering in the presence of an optical resonator using a cavity optomechanics formalism. We extend the molecular optomechanics formalism to the case of hybrid…
We describe how strong resonant interactions in multimode optomechanical systems can be used to induce controlled nonlinear couplings between single photons and phonons. Combined with linear mapping schemes between photons and phonons,…
We propose a molecular optomechanical platform to generate robust entanglement among bosonic modes-photons, phonons, and plasmons-under ambient conditions. The system integrates an ultrahigh-Q whispering-gallery-mode (WGM) optical resonator…
Radio-frequency communication systems have long used bulk- and surface-acoustic-wave devices supporting ultrasonic mechanical waves to manipulate and sense signals. These devices have greatly improved our ability to process microwaves by…
The optical properties of defects in solids produce rich physics, from gemstone coloration to single-photon emission for quantum networks. Essential to describing optical transitions is electron-phonon coupling, which can be predicted from…
Phonon nonlinearities play an important role in hybrid quantum networks and on-chip quantum devices. We investigate the phonon statistics of a mechanical oscillator in hybrid systems composed of an atom and one or two standard…
Molecular cavity optomechanical systems, featuring ultrahigh vibrational frequencies and strong light-matter interactions, hold significant promise for advancing applications in quantum science and technology. Specifically, by introducing…
Determining the vibrational structure of a molecule is central to fundamental applications in several areas, from atmospheric science to catalysis, fuel combustion modeling, biochemical imaging, and astrochemistry. However, when significant…
High-fidelity quantum optomechanical control of a mechanical oscillator requires the ability to perform efficient, low-noise operations on long-lived phononic excitations. Microfabricated high-overtone bulk acoustic wave resonators…
Molecules are ubiquitous in natural phenomena and man-made products, but their use in quantum optical applications has been hampered by incoherent internal vibrations and other phononic interactions with their environment. We have now…
To date, micro- and nano-scale optomechanical systems have enabled many proof-of-principle quantum operations through access to high-frequency (GHz) phonon modes that are readily cooled to their thermal ground state. However, minuscule…
Atomic force spectroscopy and microscopy (AFM) are invaluable tools to characterize nanostructures and biological systems. Most experiments, including state-of-the-art images of molecular bonds, are achieved by driving probes at their…
In cavity optomechanics, nanomechanical motion couples to a localized optical mode. The regime of single-photon strong coupling is reached when the optical shift induced by a single phonon becomes comparable to the cavity linewidth. We…
The mechanical properties of light have found widespread use in the manipulation of gas-phase atoms and ions, helping create new states of matter and realize complex quantum interactions. The field of cavity-optomechanics strives to scale…