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Over the past two decades, the magnetic ground states of all rare earth titanate pyrochlores have been extensively studied, with the exception of Sm$_2$Ti$_2$O$_7$. This is, in large part, due to the very high absorption cross-section of…

Gd2GaSbO7 and Gd2InSbO7 pyrochlore compounds exhibit quantum fluctuations in a spin ice-like state. These compounds have not been adequately studied based on the concept of magnetic frustration. Here, we have synthesised and characterised…

The pyrochlore material Nd$_2$Zr$_2$O$_7$ with an "all-in-all-out" (AIAO) magnetic order shows novel quantum moment fragmentation with gapped flat dynamical spin ice modes. The parameterized spin Hamiltonian with a dominant frustrated…

材料科学 · 物理学 2020-03-11 J. Xu , Owen Benton , A. T. M. N. Islam , T. Guidi , G. Ehlers , B. Lake

We report on the study of unusual spin glass properties in the geometrically frustrated pyrochlore Tb$_{2}$Mo$_{2}$O$_{7}$, $T$$_{g}$$\simeq$24 K. The analysis of the nonlinear part of dc and complex susceptibilities, near the glass…

强关联电子 · 物理学 2013-09-17 D. K. Singh , Y. S. Lee

Using Raman scattering spectroscopy, we uncover a complex magnetic behavior of Nd$_2$Ir$_2$O$_7$ , which stands out among magnetic pyrochlores by the lowest temperature of the all-in-all-out (AIAO) Ir moments ordering…

Polycrystalline Nd2Ru2O7 samples have been prepared and examined using a combination of structural, magnetic, and electrical and thermal transport studies. Analysis of synchrotron X-ray and neutron diffraction patterns suggests some site…

We report neutron scattering studies of the spin correlations of the geometrically frustrated pyrochlore Tb2Mo2O7 using single crystal samples. This material undergoes a spin-freezing transition below Tg~24 K, similar to Y2Mo2O7, and has…

强关联电子 · 物理学 2009-11-13 D. K. Singh , J. S. Helton , S. Chu , T. H. Han , C. J. Bonnoit , S. Chang , H. J. Kang , J. W. Lynn , Y. S. Lee

The insulating pyrochlore compound Nd2Sn2O7 has been shown to undergo a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in--all-out magnetic structure of the Nd3+ magnetic moments. An anomalously slow paramagnetic…

强关联电子 · 物理学 2017-05-04 P. Dalmas de Reotier , A. Yaouanc , A. Maisuradze , A. Bertin , P. J. Baker , A. D. Hillier , A. Forget

We investigate the magnetic ground state of CuNdO$_2$, which is a delafossite with a triangular lattice of magnetic Nd$^{3+}$ ions that are well separated by non-magnetic Cu spacer layers. From inelastic neutron scattering measurements of…

In this study, we performed powder neutron diffraction and inelastic scattering measurements of frustrated pyrochlore Nd$_2$Ir$_2$O$_7$, which exhibits a metal-insulator transition at a temperature $T_{\rm MI}$ of 33 K. The diffraction…

强关联电子 · 物理学 2012-02-29 K. Tomiyasu , K. Matsuhira , K. Iwasa , M. Watahiki , S. Takagi , M. Wakeshima , Y. Hinatsu , M. Yokoyama , K. Ohoyama , K. Yamada

Pyrochlore oxides $A_2B_2$O$_7$ have been a fruitful playground for condensed matter physics because of the unique geometry in the crystal structure. Especially focusing on the $A$-site tetrahedral sub-lattice, in particular, pyrochlore…

材料科学 · 物理学 2022-07-04 T. C. Fujita , H. Ito , M. Kawasaki

In a recent letter [Phys. Rev. Lett. {\bf 82}, 1012 (1999)] it was found that the Tb$^{3+}$ magnetic moments in the Tb$_2$Ti$_2$O$_7$ pyrochlore lattice of corner-sharing tetrahedra remain in a {\it collective paramagnetic} state down to…

无序系统与神经网络 · 物理学 2009-10-31 M. J. P. Gingras , B. C. den Hertog , M. Faucher , J. S. Gardner , L. J. Chang , B. D. Gaulin , N. P. Raju , J. E. Greedan

We present present a quantitative experimental investigation of the scalar chiral magnetic order with in $\rm{Nd_3Sb_3Mg_2O_{14}}$. Static magnetization reveals a net ferromagnetic ground state, and inelastic neutron scattering from the…

强关联电子 · 物理学 2019-07-17 A. Scheie , S. Dasgupta , M. Sanders , A. Sakai , Y. Matsumoto , T. R. Prisk , S. Nakatsuji , R. J. Cava , C. Broholm

We report neutron diffraction measurements of the magnetic structures in two pyrochlore iridates, Yb2Ir2O7 and Lu2Ir2O7. Both samples exhibit the all-in-all-out magnetic structure on the Ir4+ sites below TN~ 150,K, with a low temperature…

Motivated by the variation in reported lattice parameters of floating-zone-grown Nd$_{2}$Zr$_{2}$O$_{7}$ crystals, we have performed a detailed study of the relationship between synthesis environment, structural disorder, and magnetic…

Within the past 20 years or so, there has occurred an explosion of interest in the magnetic behavior of pyrochlore oxides of the type $A_{2}^{3+}$$B_{2}^{4+}$O$_{7}$ where $A$ is a rare-earth ion and $B$ is usually a transition metal. Both…

无序系统与神经网络 · 物理学 2010-01-26 Jason S. Gardner , Michel J. P. Gingras , John E. Greedan

We report the synthesis and structural study of mixed oxides in the Ln2ScNbO7 series. New phases with Ln = Pr, Eu, Gd and Dy are obtained. All crystallize in the cubic pyrochlore structure type, space group F-d3m, with no Sc-Nb ordering on…

材料科学 · 物理学 2008-12-16 Siwar Zouari , Rafik Ballou , Abdelwaheb Cheikh-Rouhou , Pierre Strobel

The consecutive magnetic ordering of the Ho and Ru ions in the pyrochlore Ho2Ru2O7 and their interplay are investigated by neutron scattering, magnetic and specific heat measurements. The Ru moments order at 95 K into a $\Gamma_5$…

The results of magnetic investigations on a new series of compounds, Mn2R3Sb3O14, containing 2-dimensional Kagome lattice of R ions and belonging to pyrochlore series, are presented. Crystallographic features of light R members (R= La, Pr…

强关联电子 · 物理学 2016-05-18 Venkatesh Chandragiri , Kartik K Iyer , K. Maiti , E. V. Sampathkumaran

In the pyrochlore compounds, Tb$_2$Ti$_2$O$_7$ and Tb$_2$Sn$_2$O$_7$, only the Tb$^{3+}$ ions are magnetic. They exhibit quite abnormal -- and, in view of their chemical similarity, strikingly different -- magnetic behaviour, as probed by…

强关联电子 · 物理学 2009-11-11 I. Mirebeau , A. Apetrei , I. N. Goncharenko , R. Moessner