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Motivated by recent reports of superconductivity in Sr-doped NdNiO$_2$ films on SrTiO$_3$(001) [Nature (London) 572, 624 (2019)], we explore the role of the polar interface on the structural and electronic properties of…

超导电性 · 物理学 2020-07-15 Benjamin Geisler , Rossitza Pentcheva

The recent discovery of superconductivity in Sr-doped NdNiO$_2$ films grown on SrTiO$_3$ started a novel field within unconventional superconductivity. To understand the similarities and differences between nickelate and cuprate layers on…

强关联电子 · 物理学 2020-11-13 Yang Zhang , Ling-Fang Lin , Wenjun Hu , Adriana Moreo , Shuai Dong , Elbio Dagotto

Nickel-based superconductors provide a long-awaited experimental platform to explore possible cuprate-like superconductivity. Despite similar crystal structure and $d$ electron filling, these systems exhibit several differences. Nickelates…

The search for oxide materials with physical properties similar to the cuprate high Tc superconductors, but based on alternative transition metals such as nickel, has grown and evolved over time. The recent discovery of superconductivity in…

To understand the superconductivity recently discovered in Nd$_{0.8}$Sr$_{0.2}$NiO$_2$, we carried out LDA+DMFT (local density approximation plus dynamical mean-field theory) and magnetic force response calculations. The on-site correlation…

超导电性 · 物理学 2020-02-25 Siheon Ryee , Hongkee Yoon , Taek Jung Kim , Min Yong Jeong , Myung Joon Han

Infinite-layer nickelate thin films materialize an intriguing new platform for high-temperature unconventional superconductivity, with LaNiO$_2$/SrTiO$_3$ as reference setup. We discuss the relative stability of the elementary interfaces of…

超导电性 · 物理学 2020-08-03 F. Bernardini , A. Cano

The correlated electronic structure of the infinite-layer compounds NdNiO$_2$ and SrCuO$_2$ at stoichiometry and with finite hole doping is compared. Key differences are elucidated from an advanced first-principles many-body perspective.…

强关联电子 · 物理学 2020-03-06 Frank Lechermann

In complex transition metal oxide heterostructures of physically dissimilar perovskite compounds, interface phenomena can lead to novel physical properties not observed in either of their constituents. This remarkable feature opens new…

强关联电子 · 物理学 2011-12-30 Natalia Pavlenko , Thilo Kopp

The discovery of infinite-layer nickelate superconductors has spurred enormous interest. While the Ni$^{1+}$ cations possess nominally the same 3$d^9$ configuration as Cu$^{2+}$ in cuprates, the electronic structure variances remain…

Several reports about infinite-layer nickelate thin films suggest that the superconducting critical temperature versus chemical doping phase diagram has a dome-like shape, similar to cuprates. Here, we demonstrate a highly reproducible…

The 2019 discovery of high temperature superconductivity in layered nickelate films, Nd$_{1-x}$SrNiO$_2$, has galvanized a community that has been studying nickelates for more than 30 years both as cuprate analogs and in their own right. On…

超导电性 · 物理学 2021-12-24 J. F. Mitchell

The impact of spin-orbit interactions in NdNiO2/SrTiO3(001) and NdNiO2/KTaO3(001) is explored by performing density functional theory simulations including a Coulomb repulsion term. Polarity mismatch drives the emergence of an interfacial…

超导电性 · 物理学 2024-01-10 Benjamin Geisler

Superconductivity in infinite-layer nickelates holds exciting analogies with that of cuprates, with similar structures and $3d$-electron count. Using resonant inelastic x-ray scattering (RIXS) we studied electronic and magnetic excitations…

The recent observation of superconductivity in infinite-layer Nd$_{1-x}$Sr$_x$NiO$_2$ thin films has attracted a lot of attention, since this compound is electronically and structurally analogous to the superconducting cuprates. Due to the…

We report the phase diagram of Nd$_{1-x}$Sr$_x$NiO$_2$ infinite layer thin films grown on SrTiO$_3$. A superconducting dome spanning $0.125 < x < 0.25$ is found, remarkably similar to cuprates, albeit over a narrower doping window. However,…

Recently superconductivity at 9 - 15 K was discovered in an infinite-layer nickelate (Nd$_{0.8}$Sr$_{0.2}$NiO$_2$ films), which has received enormous attention. Since the $Ni^{1+}$ ionic state in NdNiO$_2$ may have the $3d^9$ outer-shell…

超导电性 · 物理学 2020-04-06 Qing Li , Chengping He , Jin Si , Xiyu Zhu , Yue Zhang , Hai-Hu Wen

Rare-earth infinite-layer nickelates represent an emerging class of unconventional superconductors, with materials synthesis largely limited to early lanthanide compounds. Here, we report the synthesis and characterization of phase-pure…

The large antiferromagnetic exchange coupling in the parent high-$T_{\rm c}$ cuprate superconductors is believed to play a crucial role in pairing the superconducting carriers. The recent observation of superconductivity in hole-doped…

强关联电子 · 物理学 2020-12-22 Vamshi M. Katukuri , Nikolay A. Bogdanov , Oskar Weser , Jeroen van den Brink , Ali Alavi

A variety of nickel oxide compounds have long been studied for their manifestation of various correlated electron phenomena. Recently, superconductivity was observed in nanoscale infinite layer nickelate thin films of…

The recent discovery of superconductivity in hole-doped planar nickelates R1-xSrNiO2 (R=Pr,Nd) raises the foundational question of how the electronic structure and electronic correlations of these Ni1+ compounds compare to those of the Cu2+…

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