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The transient Pauli blocking effect offers a promising route for achieving ultrafast optical switching in semiconductors, enabling a rapid switching from an initially opaque state to a relatively transparent state upon photoexcitation.…

The ultrafast dynamics of surface electromagnetic waves photogenerated on aluminum film perforated with subwavelength holes array was studied in the visible spectral range by the technique of transient photomodulation with 100 fs time…

材料科学 · 物理学 2008-08-27 M. Tong , A. S. Kirakosyan , T. V. Shahbazyan , Z. V. Vardeny

Ultrafast optical pump-probe spectroscopy measurement on monolayer graphene observes significant optical nonlinearities. We show that strongly photoexcited graphene monolayers with 35 fs pulses quasi-instantaneously build up a broadband,…

介观与纳米尺度物理 · 物理学 2015-06-15 Junhua Zhang , Joerg Schmalian , Tianqi Li , Jigang Wang

The photoexcited state in superconducting metals and alloys was studied via pump-probe spectroscopy. A pulsed Ti:sapphire laser was used to create the non-equilibrium state and the far-infrared pulses of a synchrotron storage ring, to which…

Approaching energy coupling in laser-irradiated metals, we point out the role of electron-electron collision as an efficient control factor for ultrafast optical absorption. The high degree of laser-induced electron-ion nonequilibrium…

光学 · 物理学 2008-12-18 Jean-Philippe Colombier , Patrick Combis , Eric Audouard , Razvan Stoian

Many linked processes occur concurrently in strongly excited semiconductors, such as interband and intraband absorption, scattering of electrons and holes by the heated lattice, Pauli blocking, bandgap renormalization and the formation of…

We study the ultrafast dynamics of surface electromagnetic waves photogenerated on aluminum film perforated with subwavelength holes array by means of transient photomodulation with 100 fs time resolution. We observed a pronounced blueshift…

材料科学 · 物理学 2009-11-13 A. S. Kirakosyan , M. Tong , T. V. Shahbazyan , Z. V. Vardeny

Transient reflectivity (TR) from thin films (6 - 40 nm thick) of the topological insulator Bi2Se3 reveal ultrafast carrier dynamics, which suggest the existence of both radiative and non-radiative recombination between electrons residing in…

介观与纳米尺度物理 · 物理学 2015-06-23 Yuri D. Glinka , Sercan Babakiray , Trent A. Johnson , Mikel B. Holcomb , David Lederman

The optical conductivity of freely suspended graphene was examined under non-equilibrium conditions using femtosecond pump-probe spectroscopy. We observed a conductivity transient that varied strongly with the electronic temperature,…

介观与纳米尺度物理 · 物理学 2013-06-20 Leandro M. Malard , Kin Fai Mak , A. H. Castro Neto , N. M. R. Peres , Tony F. Heinz

We demonstrate, by femtosecond time- and angle-resolved photoemission spectroscopy, that photoinduced interlayer charge transfer in a heterostructure consisting of Bernal-stacked bilayer graphene and a single atomic layer of silver on…

介观与纳米尺度物理 · 物理学 2026-02-23 Eduard Moos , Zhi-Yuan Deng , Hauke Beyer , Arpit Jain , Chengye Dong , Li-Syuan Lu , Joshua A. Robinson , Kai Rossnagel , Michael Bauer

The coherent reflectivity of a dense, relativistic, ultra-thin electron layer is derived analytically for an obliquely incident probe beam. Results are obtained by two-fold Lorentz transformation. For the analytical treatment, a plane…

等离子体物理 · 物理学 2009-11-13 Hui-Chun Wu , Jürgen Meyer-ter-Vehn

Metals exhibit nonequilibrium electron and lattice subsystems at transient times following femtosecond laser excitation. In the past four decades, various optical spectroscopy and time-resolved diffraction methods have been used to study…

化学物理 · 物理学 2024-05-17 Xing He , Mithun Ghosh , Ding-Shyue Yang

Transient reflectivity (TR) measured at laser photon energy 1.51 eV from the indirectly intersurface coupled topological insulator Bi2-xMnxSe3 films (12 nm thick) revealed a strong dependence of the rise-time and initial decay-time…

介观与纳米尺度物理 · 物理学 2016-04-20 Yuri D. Glinka , Sercan Babakiray , Mikel B. Holcomb , David Lederman

We theoretically investigate ultrafast and nonlinear optical properties of graphite thin films based on first-principles time-dependent density functional theory. We first calculate electron dynamics in a unit cell of graphite under a…

Complex materials encompassing different phases of matter can display new photoinduced metastable states differing from those attainable under equilibrium conditions. These states can be realized when energy is injected in the material…

Ultrafast degenerate pump-probe experiments performed on a free standing film of double walled carbon nanotubes near the first metallic transition energy of outer tube show ultrafast ($97 fs$) photobleaching followed by a photo-induced…

其他凝聚态物理 · 物理学 2009-11-13 N. Kamaraju , Sunil Kumar , B. Karthikeyan , Alexander Moravsky , R. O. Loutfy , A. K. Sood

Out-of-equilibrium effects provide an elegant pathway to probing and understanding the underlying physics of topological materials. Creating exotic states of matter using ultrafast optical pulses in particular has shown promise towards…

Using time-domain Terahertz spectroscopy we performed direct studies of the photoinduced suppression and recovery of the superconducting gap in a conventional BCS superconductor NbN. Both processes are found to be strongly temperature and…

超导电性 · 物理学 2015-05-27 M. Beck , M. Klammer , S. Lang , P. Leiderer , V. V. Kabanov , G. N. Gol'tsman , J. Demsar

Transition metal nitrides have recently gained attention in the fields of plasmonics, plasmon-enhanced photocatalysis, photothermal applications, and nonlinear optics because of their suitable optical properties, refractory nature, and…

We have recorded the coherent diffraction images of individual xenon clusters with intense extreme ultraviolet pulses to elucidate the influence of light-induced electronic changes on the diffraction pattern. Using the FLASH free-electron…

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