相关论文: Extraterrestrial Photochemistry: Principles and Ap…
Photoluminescence from metal nanostructures following intense ultrashort illumination is a fundamental aspect of light-matter interactions. Surprisingly, many of its basic characteristics are under ongoing debate. Here, we resolve many of…
We calculate the thermochemical equilibrium of the diffuse interstellar medium, including ionization by a photon flux F_{nu} from neutrino decay. The main heating mechanism considered is photoelectrons from grains and PAHs. For the studied…
Our Galaxy is the largest nuclear interaction experiment which we know, because of the interaction between cosmic ray particles and the interstellar material. Cosmic rays are particles, which have been accelerated in the Galaxy or in…
Ice is a major component of astrophysical environment - from interstellar molecular clouds through protoplanetary disks to evolved solar systems. Ice and complex organic matter coexist in these environments as well, and it is thought…
Interstellar ice mantles on the surfaces of dust grains are thought to have a bi-layered structure, with a H2O-rich polar layer, covered by a CO-rich apolar layer that probably harbors H2 and other volatiles such as N2. In this work, we…
The chemical and mass evolution of exoplanet atmospheres is shaped by their specific X-ray through ultraviolet (5 - 3200 Angstroms) irradiance history. X-ray and EUV (5 - 911 Angstroms) radiation largely contributes to atmospheric heating…
We have designed an improved algorithm that enables us to simulate the chemistry of cold dense interstellar clouds with a full gas-grain reaction network. The chemistry is treated by a unified microscopic-macroscopic Monte Carlo approach…
In this chapter, we provide a review of radiative processes in cometary atmospheres spanning a broad range of wavelengths, from radio to X-rays. We focus on spectral modeling, observational opportunities, and anticipated challenges in the…
Motivated by the WMAP results indicating an early epoch of reionization, we consider alternative cosmic star formation models which are capable of reionizing the early intergalactic medium. We develop models which include an early burst of…
Protoplanetary disks undergo substantial mass-loss by photoevaporation, a mechanism which is crucial to their dynamical evolution. However, the processes regulating the gas energetics have not been well constrained by observations so far.…
In the laboratory, the photo-and thermochemical evolution of ices, made of simple molecules of astrophysical relevance, always leads to the formation of semi-refractory water-soluble organic residues. Targeted searches for specific…
Hydroxylamine (NH2OH) is one of the potential precursors of complex pre-biotic species in space. Here we present a detailed experimental study of hydroxylamine formation through nitric oxide (NO) surface hydrogenation for astronomically…
Photosynthesis offers a convenient means of sustaining biospheres. We quantify the constraints for photosynthesis to be functional on the permanent nightside of tidally locked rocky exoplanets via reflected light from their exomoons. We…
Context. Interstellar surface chemistry is a complex process that occurs in icy layers accumulated onto grains of different sizes. Efficiency of surface processes often depends on the immediate environment of adsorbed molecules. Aims. We…
We are now on a clear trajectory for improvements in exoplanet observations that will revolutionize our ability to characterize their atmospheric structure, composition, and circulation, from gas giants to rocky planets. However, exoplanet…
UV ice photodesorption is an important non-thermal desorption pathway in many interstellar environments that has been invoked to explain observations of cold molecules in disks, clouds and cloud cores. Systematic laboratory studies of the…
The development of molecular complexity during stellar and planetary formation owes much to the interaction of gas and dust. When the first astrochemical models including solid-state chemistry were developed more than forty years ago, data…
Cosmic rays of kinetic energies below ~1 GeV per nucleon are thought to play a key role in the chemistry and dynamics of the interstellar medium. They are also thought to be responsible for nucleosynthesis of the light elements Li, Be, and…
A new experimental set-up INterStellar Ice-Dust Experiment (INSIDE), was designed for studying cosmic grain analogues represented by ice-coated carbon- and silicate-based dust grains. In the new instrument, we can simulate physical and…
Laboratory astrochemistry aims at simulating in the laboratory some of the chemical and physical processes that operate in different regions of the Universe. Amongst the diverse astrochemical problems that can be addressed in the…