相关论文: Enantio-detection via cavity-assisted three-photon…
We find that two-color fields can induce field-free permanent dipoles in initially isotropic samples of chiral molecules via resonant electronic excitation in a one-$3\omega$-photon vs. three-$\omega$-photons scheme. These permanent dipoles…
Synthetic chiral light enables ultrafast and highly efficient imaging of molecular chirality. Unlike standard circularly polarized light, the handedness of synthetic chiral light does not rely on the spatial structure of the light field: it…
Ultracold ground-state molecules can be formed from ultracold atoms via photoassociation followed by a spontaneous emission process. Typically, the molecular products are distributed over a range of final states. Here, we propose to use an…
The spontaneous emission spectrum of a multi-level atom or molecule with nonreciprocal transition is investigated. It is shown that the nonreciprocal transition can lead to the elimination of a spectral line in the spontaneous emission…
We inspect different quantum optical setups from the viewpoint of entanglement generation and detection. As a first step we consider a planar semiconductor microcavity and optimize the Bell-type correlations and their robustness against…
Molecular matter-wave interferometry enables novel strategies for manipulating the internal mechanical motion of complex molecules. Here, we show how chiral molecules can be prepared in a quantum superposition of two enantiomers by…
We propose a predictive building-up of tetrahedral molecules, based on a previously derived chirality index, which characterizes a tetrahedral molecule, with n chiral centers, as achiral, diastereoisomer, or enantiomer as a function of the…
Ultracold atoms coupled to optical cavities offer a powerful platform for studying strongly correlated many-body physics. Here, we propose an experimental scheme for creating biatomic molecules via cavity-enhanced photoassociation from an…
With a microwave-regime cyclic three-state configuration, an enantiomer-selective state transfer~(ESST) is carried out through the two-path interference between a direct one-photon coupling and an effective two-photon coupling. The…
Numerous inequalities involving moments of integrated intensities and revealing nonclassicality and entanglement in bipartite optical fields are derived using the majorization theory, non-negative polynomials, the matrix approach, as well…
Chiral molecules show differences in their chemical and optical properties due to different spatial arrangements of the atoms in the two enantiomers. A common way to optically differentiate them is to detect the disparity in the absorption…
We present a scheme for the fast generation of entangled photons from a single quantum dot coupled to a planar photonic crystal that support two orthogonally polarized cavity modes. We discuss ``within generation'' and ``across generation''…
We isolate the two-step mechanism involving a real intermediate photon from the one-step mechanism involving a virtual photon for the trident process in a constant crossed field. The two-step process is shown to agree with an integration…
A novel approach for the state-specific enantiomeric enrichment and the spatial separation of enantiomers is presented. Our scheme utilizes techniques from strong-field laser physics, specifically an optical centrifuge in conjunction with a…
We propose an optical cavity-QED scheme for the deterministic generation of polarization entangled photon pairs that operates with high fidelity even in the bad cavity limit. The scheme is based on the interaction of an excited four-level…
We explore a pure optical method for enantioselective orientation of chiral molecules by means of laser fields with twisted polarization. Several field implementations are considered, including a pair of delayed cross-polarized laser…
Chirality is a pervasive form of symmetry that is intimately connected to the physical properties of solids, as well as the chemical and biological activity of molecular systems. However, its control with light is challenging, because…
This review is based on the talk in the conference of "Spectroscopic Studies on Molecular Chirality" held on Dec 20-21 2013. The objects of the present paper are to (1) derive the energy difference between Laevorotatory, or left-handed,…
Strong coupling with circularly polarized vacuum fluctuations offers a viable route to manipulate molecular chirality. While experiments are advancing toward the realization of chiral cavities, a mean-field theoretical framework for…
We develop a mathematical formalism underlying the emergence of enantio-sensitive molecular orientation due to photoionization or photoexitation of chiral molecules. We consider geometric quantities such as the Berry connection and Berry…