相关论文: Nonlinear terahertz electro-optical responses in c…
Dynamic Kerr effect measurements provide a simple realization of a nonlinear experiment. We propose a field-off experiment where an electric field of one or several sinusoidal cycles is applied to a sample in thermal equilibrium.…
We have investigated both inter-band and intra-band second order nonlinear optical conductivity based on the velocity correlation formalism and the spectral expansion technique. We propose a scenario in which the second order intra-band…
Kernel-based methods have been recently introduced for linear system identification as an alternative to parametric prediction error methods. Adopting the Bayesian perspective, the impulse response is modeled as a non-stationary Gaussian…
Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…
We report on the nonlinear spectroscopy of water vapor at THz frequencies. Atmospheric water vapor has a rich spectrum with several strong resonances at frequencies below 3 THz, falling within the range of operation of most existing THz…
Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…
We resolve the real-time electric field of a femtosecond third-order nonlinear optical signal in the molecular frame. The electric field emitted by the induced third-order polarization from impulsively pre-aligned gas-phase molecules at…
We develop a systematic projector-based Feynman diagram framework that intrinsically encodes quantum geometry for nonlinear optical responses. By explicitly incorporating geometric quantities such as the quantum geometric tensor, quantum…
We study the non-linear electromagnetic response of graphene taking into account the self-consistent-field effects. Response of the system to a strong pulse excitation is calculated. It is shown that radiative decay in graphene differs from…
The invariance principle, through which the steady-state behavior of nonlinear systems was introduced by Isidori and Byrnes, is leveraged in this article to bring forth a unifying characterization of the frequency response of nonlinear…
Third harmonic generation of terahertz radiation is expected to occur in monolayer graphene due to the nonlinear relationship between the crystal momentum and the current density. In this work, we calculate the terahertz nonlinear response…
Numerical methods are developed to solve the problem of abnormal changes of current (conductivity) in polymer composite films which may be used as current, pressure or temperature sensors. General nonlinear model includes the heat equation,…
Terahertz nonlinear optics is a viable method to interrogate collective phenomena in quantum materials spanning ferroelectrics, charge-density waves, and superconductivity. In superconductors this includes the Higgs amplitude and Josephson…
The interaction of waves in nonlinear Kerr waveguides are, under some circumstances, similar to the physics occurring at the horizon of black and white holes. Here, we investigate this analogy in an integrated nonlinear photonic structure…
A general non-linear response theory is derived for an arbitrary time-dependent Hamiltonian, not necessarily obeying time-reversal symmetry. This allows us to obtain a greatly generalized Kubo type formula. Applied to a mesoscopic system…
We present a detailed theoretical investigation of the linear and non-linear optical response in a model system for a disordered d-wave superconductor, showing that for both quantities the gap symmetry considerably changes the paradigm of…
Nonlinear optical responses are becoming increasingly relevant for characterizing the symmetries and quantum geometry of electronic phases in materials. Here, we develop an expanded diagrammatic scheme for calculating spatially dispersive…
We obtain the conductance of a system of electrons connected to leads, within time-dependent density-functional theory, using a direct relation between the conductance and the density response function. Corrections to the non-interacting…
Coherent nonlinear optical micro-spectroscopy is a frequently used tool in modern material science, as it is sensitive to many different local observables, which comprise, among others, crystal symmetry and vibrational properties. The…
Nonlinear optical processes associated with even-order nonlinear susceptibilities are critical for both classical and quantum technologies. Inversion symmetry, however, prevents nonlinear optical responses mediated by even-order…