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Sr$_2$IrO$_4$ is an extensively studied spin-orbit coupling induced insulator with antiferromagnetic ground state. The delicate balance between competing energy scales plays crucial role for its low temperature phase, and the route of…

强关联电子 · 物理学 2017-10-31 Imtiaz Noor Bhatti , R. S. Dhaka , A. K. Pramanik

The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore…

强关联电子 · 物理学 2017-03-08 Harish Kumar , R. S. Dhaka , A. K. Pramanik

Sr2IrO4 is a magnetic insulator driven by spin-orbit interaction (SOI) whereas the isoelectronic and isostructural Sr2RhO4 is a paramagnetic metal. The contrasting ground states have been shown to result from the critical role of the strong…

强关联电子 · 物理学 2012-09-07 T. F. Qi , O. B. Korneta , L. Li , K. Butrouna , V. S. Cao , Xiangang Wan , P. Schlottmann , R. K. Kaul , G. Cao

The 3$d$-5$d$ based double perovskites are of current interest as they provide model system to study the interplay between electronic correlation ($U$) and spin-orbit coupling (SOC). Here we report detailed structural, magnetic and…

强关联电子 · 物理学 2017-10-30 K C Kharkwal , A K Pramanik

We report a systematical structural, transport and magnetic study of Ca or Ba doped Sr2IrO4single crystals. Isoelectronically substituting Ca2+ (up to 15%) or Ba2+ (up to 4%) ion for the Sr2+ ion provides no additional charge carriers but…

强关联电子 · 物理学 2018-05-04 H. D. Zhao , J. Terzic , H. Zheng , Y. F. Ni , Y. Zhang , Feng Ye , P. Schlottmann , G. Cao

Tuning of spin-orbit coupling and electron correlation effects in pyrochlore iridates is considered for many interesting phenomena. We have investigated the temperature evolution of structural, magnetic and electronic properties in doped…

强关联电子 · 物理学 2019-05-07 Harish Kumar , A. K. Pramanik

We have used a combination of resonant magnetic x-ray scattering (RMXS) and x-ray absorption spectroscopy (XAS) to investigate the properties of the doped spin-orbital Mott insulator Sr2Ir(1-x)Rh(x)O4 (0.07 < x < 0.70). We show that…

强关联电子 · 物理学 2014-02-12 J. P. Clancy , A. Lupascu , H. Gretarsson , Z. Islam , Y. F. Hu , D. Casa , C. S. Nelson , S. C. Lamarra , G. Cao , Young-June Kim

The $f$-$d$ magnetic exchange interaction is considered to be a key ingredient for many exotic topological phases in pyrochlore iridates. Here, we have investigated the evolution of structural, magnetic and electronic properties in doped…

强关联电子 · 物理学 2020-02-07 Harish Kumar , K. C. Kharkwal , Kranti Kumar , K. Asokan , A. Banerjee , A. K. Pramanik

The magnetic excitations in electron doped (Sr$_{1-x}$La$_x$)$_2$IrO$_4$ with $x = 0.03$ were measured using resonant inelastic X-ray scattering at the Ir $L_3$-edge. Although much broadened, well defined dispersive magnetic excitations…

强关联电子 · 物理学 2016-06-15 Xuerong Liu , M. P. M. Dean , Z. Y. Meng , M. H. Upton , T. Qi , T. Gog , Y. Cao , J. Q. Lin , D. Meyers , H. Ding , G. Cao , H. P. Hill

One way to induce insulator to metal transitions in the spin-orbit Mott insulator Sr2IrO4 is to substitute iridium with transition metals (Ru, Rh). However, this creates intriguing inhomogeneous metallic states, which cannot be described by…

The evolution of the electronic properties of electron-doped (Sr{1-x}La{x})2IrO4 is experimentally explored as the doping limit of La is approached. As electrons are introduced, the electronic ground state transitions from a spin-orbit Mott…

Sr2IrO4 is a magnetic insulator assisted by strong spin-orbit coupling (SOC) whereas the Sr2RuO4 is a p-wave superconductor. The contrasting ground states have been shown to result from the critical role of the strong SOC in the iridate.…

强关联电子 · 物理学 2016-04-26 S. J. Yuan , S. Aswartham , J. Terzic , H. Zheng , H. D. Zhao , P. Schlottmann , G. Cao

We have investigated the temperature evolution of magnetism and its interrelation with structural parameters in perovskite-based layered compound Sr$_2$IrO$_4$, which is believed to be a $J_{eff}$ = 1/2 Mott insulator. The structural…

强关联电子 · 物理学 2014-12-15 Imtiaz Noor Bhatti , R. Rawat , A. Banerjee , A. K. Pramanik

We report structural, magnetic, transport and thermal properties of single-crystal Ca2Ru1-xIrxO4 (0 < x< 0.65). Ca2RuO4 is a structurally-driven Mott insulator with a metal-insulator transition at TMI = 357 K, which is well separated from…

强关联电子 · 物理学 2016-04-26 S. J. Yuan , J. Terzic , J. C. Wang , S. Aswartham , W. H. Song , F. Ye , G. Cao

Sr2IrO4 is a spin-orbit coupled insulator with an antiferromagnetic (AFM) transition at TN=240 K. We report results of a comprehensive study of single-crystal Sr2Ir1-xTbxO4. This study found that mere 3% (x=0.03) tetravalent Tb4+(4f7)…

Sr2IrO4 exhibits a novel insulating state driven by spin-orbit interactions. We report two novel phenomena, namely a large magnetoresistivity in Sr2IrO4 that is extremely sensitive to the orientation of magnetic field but exhibits no…

强关联电子 · 物理学 2015-05-28 M. Ge , T. F. Qi , O. B. Korneta , D. E. De Long , P. Schlottmann , W. P. Crummett , G. Cao

We investigate the electronic structure and magnetic properties of a $J_\text{eff} = 1/2$ iridate Ca$_4$IrO$_6$ and the implications of doping electrons and holes using ab initio density functional theory. Our calculations considering…

强关联电子 · 物理学 2022-09-02 Avishek Singh , Jayita Chakraborty , Nirmal Ganguli

The layered 5d transition metal oxide Sr2IrO4 has been shown to host a novel Jeff=1/2 Mott spin orbit insulating state with antiferromagnetic ordering, leading to comparisons with the layered cuprates. Here we study the effect of…

强关联电子 · 物理学 2015-03-20 S. Calder , G. -X. Cao , M. D. Lumsden , J. W. Kim , Z. Gai , B. C. Sales , D. Mandrus , A. D. Christianson

The local structure of correlated spin-orbit insulator Sr$_{2-x}$M$_x$IrO$_4$ (M = K, La) has been investigated by Ir L$_3$-edge extended x-ray absorption fine structure measurements. The measurements were performed as a function of…

Sr2IrO4 is an archetypal spin-orbit-coupled Mott insulator with an antiferromagnetic state below 240 K. Here we report results of our study on single crystals of Sr2Ir1-xFexO4 (0<x<0.32) and Sr2Ir1-xCoxO4 (0<x<0.22). Fe doping retains the…

强关联电子 · 物理学 2020-12-21 Bing Hu , Hengdi Zhao , Yu Zhang , Pedro Schlottmann , Feng Ye , Gang Cao
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