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Paramagnetic magnetic resonance, a powerful technique for characterizing and identifying chemical targets, is increasingly used for imaging; however, low spin polarization at room temperature and moderate magnetic fields poses challenges…

介观与纳米尺度物理 · 物理学 2019-09-04 C. M. Purser , V. P. Bhallamudi , C. S. Wolfe , H. Yusuf , B. A. McCullian , C. Jayaprakash , M. E. Flatté , P. C. Hammel

Using an optical tweezers apparatus, we demonstrate three-dimensional control of nanodiamonds in solution with simultaneous readout of ground-state electron-spin resonance (ESR) transitions in an ensemble of diamond nitrogen-vacancy (NV)…

We demonstrate electron spin polarization detection and electron paramagnetic resonance (EPR) spectroscopy using a direct current superconducting quantum interference device (dc-SQUID) magnetometer. Our target electron spin ensemble is…

介观与纳米尺度物理 · 物理学 2024-06-24 Hiraku Toida , Yuichiro Matsuzaki , Kosuke Kakuyanagi , Xiaobo Zhu , William J. Munro , Kae Nemoto , Hiroshi Yamaguchi , Shiro Saito

Electron paramagnetic resonance (EPR) can provide unique insight into the chemical structure and magnetic properties of dopants in oxide and semiconducting materials that are of interest for applications in electronics, catalysis, and…

Performing nanoscale scanning electron paramagnetic resonance (EPR) requires three essential ingredients. First, a static magnetic field together to field gradients to Zeeman split the electronic energy levels with spatial resolution.…

介观与纳米尺度物理 · 物理学 2024-01-16 Carlos A. González-Gutiérrez , David García-Pons , David Zueco , María José Martínez-Pérez

Electron Spin Resonance (ESR) describes a suite of techniques for characterising electronic systems, with applications in physics, materials science, chemistry, and biology. However, the requirement for large electron spin ensembles in…

量子物理 · 物理学 2015-03-04 L. T. Hall , P. Kehayias , D. A. Simpson , A. Jarmola , A. Stacey , D. Budker , L. C. L. Hollenberg

We describe a fully broadband approach for electron spin resonance (ESR) experiments where it is possible to not only tune the magnetic field but also the frequency continuously over wide ranges. Here a metallic coplanar transmission line…

Electron spin resonance (ESR) spectroscopy is the method of choice for characterizing paramagnetic impurities, with applications ranging from chemistry to quantum computing, but it gives access only to ensemble-averaged quantities due to…

An interacting spin system is an excellent testbed for fundamental quantum physics and applications in quantum sensing and quantum simulation. For these investigations, detailed information of the interactions, e.g., the number of spins and…

量子物理 · 物理学 2024-11-12 Yuhang Ren , Susumu Takahashi

Electron spin resonance (ESR) spectroscopy has broad applications in physics, chemistry and biology. As a complementary tool, zero-field ESR (ZF-ESR) spectroscopy has been proposed for decades and shown its own benefits for investigating…

量子物理 · 物理学 2020-02-20 Fei Kong , Pengju Zhao , Xiangyu Ye , Zhecheng Wang , Zhuoyang Qin , Pei Yu , Jihu Su , Fazhan Shi , Jiangfeng Du

High frequency electron spin resonance (ESR) spectroscopy is an invaluable tool for identification and characterization of spin systems. Nanoscale ESR using the nitrogen-vacancy (NV) center has been demonstrated down to the level of a…

介观与纳米尺度物理 · 物理学 2020-05-05 Benjamin Fortman , Junior Pena , Karoly Holczer , Susumu Takahashi

A nitrogen-vacancy (NV) center in diamond is a promising sensor for nanoscale magnetic sensing. Here we report electron spin resonance (ESR) spectroscopy using a single NV center in diamond. First, using a 230 GHz ESR spectrometer, we…

介观与纳米尺度物理 · 物理学 2016-10-05 Chathuranga Abeywardana , Viktor Stepanov , Franklin H. Cho , Susumu Takahashi

A key limitation of electron paramagnetic resonance (EPR), an established and powerful tool for studying atomic-scale biomolecular structure and dynamics is its poor sensitivity, samples containing in excess of 10^12 labeled biomolecules…

Spectral analysis of electron spin resonance (ESR) is a powerful technique for various investigations including characterization of spin systems, measurements of spin concentration, and probing spin dynamics. The nitrogen-vacancy (NV)…

介观与纳米尺度物理 · 物理学 2019-07-19 Benjamin Fortman , Susumu Takahashi

By comparing the signals of electron spin resonance (ESR) from two crystals of a diamond (spin-labels) the demagnetizing field of the Co, Fe, and Ni samples in the shape of strongly elongated ellipsoids of revolution (disks) has been…

材料科学 · 物理学 2010-06-30 N. A. Poklonski , T. M. Lapchuk , N. I. Gorbachuk

We demonstrate electrical detection of the $^{14}$N nuclear spin coherence of NV centers at room temperature. Nuclear spins are candidates for quantum memories in quantum-information devices and quantum sensors, and hence the electrical…

Electron Spin Resonance (ESR) can microscopically probe both conduction electrons (ce) and local moment (LM) spin systems in different materials. A ce spin resonance (CESR) is observed in metallic systems based on light elements or with…

强关联电子 · 物理学 2009-08-04 L. M. Holanda , J. M. Vargas , C. Rettori , S. Nakatsuji , K. Kuga , Z. Fisk , S. B. Oseroff , P. G. Pagliuso

Rare-earth spin ensembles are a promising platform for microwave quantum memory applications due to their hyperfine transitions, which can exhibit exceptionally long coherence times when using an operation point with zero first-order Zeeman…

A new method for detecting the magnetic resonance of electronic spins at low temperature is demonstrated. It consists in measuring the signal emitted by the spins with a superconducting qubit that acts as a single-microwave-photon detector,…

Electron paramagnetic resonance spectroscopy (EPR) is among the most important analytical tools in physics, chemistry, and biology. The emergence of nitrogen-vacancy (NV) centers in diamond, serving as an atomic-sized magnetometer, has…

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