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An excitonic insulator (EI) phase is a consequence of collective many-body effects where an optical band gap is formed by the condensation of electron-hole pairs or excitons. We report pressure-dependent optical pump optical probe…

材料科学 · 物理学 2024-11-28 Vikas Arora , Victor S Muthu , Arijit Sinha , Luminita Harnagea , U V Waghmare , A K Sood

The electron-hole states of semiconductor quantum dots are investigated within the framework of empirical tight-binding descriptions for Si, as an example of an indirect gap material, and InAs and CdSe as examples of typical III-V and II-VI…

凝聚态物理 · 物理学 2009-10-31 Seungwon Lee , Lars Jonsson , John W. Wilkins , Garnett W. Bryant , Gerhard Klimeck

Motivated by the possibility of pressure-induced exciton condensation in intermediate-valence Tm[Se,Te] compounds we study the Falicov-Kimball model extended by a finite f-hole valence bandwidth. Calculating the Frenkel-type exciton…

强关联电子 · 物理学 2009-11-13 D. Ihle , M. Pfafferott , E. Burovski , F. X. Bronold , H. Fehske

TiSe$_2$ is thought to be an insulator with a bandgap of ~0.1eV. It has attracted a much interest because, among of a rich array of unique properties, many have thought TiSe$_2$ is a rare realisation of an excitonic insulator. Below 200 K,…

Half a century ago, Mott noted that tuning the carrier density of a semimetal towards zero produces an insulating state in which electrons and holes form bound pairs. It was later argued that such pairing persists even if a semiconducting…

材料科学 · 物理学 2017-05-23 Z. Zhu , R. D. McDonald , A. Shekhter , B. J. Ramshaw , K. A. Modic , F. F. Balakirev , N. Harrison

Excitonic insulators are electronically-driven phases of matter characterized by the spontaneous condensation of electron-hole pairs. Here we show that La$_3$Cd$_2$As$_6$ undergoes a transition at $T_{0}=278$ K to a highly insulating state…

The bound electron-hole pairs known as excitons govern the optical properties of insulating solids. While their behavior in equilibrium is well-understood theoretically, the nonequilibrium regime at high excitation densities-where phenomena…

介观与纳米尺度物理 · 物理学 2025-10-31 Pushpendra Yadav

The excitonic insulator is an elusive electronic phase exhibiting a correlated excitonic ground state. Materials with such a phase are expected to have intriguing properties such as excitonic high-temperature superconductivity. However,…

强关联电子 · 物理学 2021-12-07 Dominik Christiansen , Malte Selig , Mariana Rossi , Andreas Knorr

Exciton condensation indicating the spontaneous formation of electron-hole pair can cause the phase transition from a semimetal to an excitonic insulator by gap opening at the Fermi surface. While the idea of this excitonic insulator has…

材料科学 · 物理学 2022-08-23 Hsiao-Yi Chen , Takuya Nomoto , Ryotaro Arita

Identifying materials hosting an excitonic insulator ground state has been one of the major pursuits in condensed matter physics in recent years. Promising candidates in transition metal chalcogenide compounds (TMC), including…

强关联电子 · 物理学 2026-03-20 Yao Zeng , Shi-Cong Mo , Wéi Wú

Excitons, quasiparticles of electrons and holes bound by Coulombic attraction, are created transiently by light and play an important role in optoelectronics, photovoltaics and photosynthesis. While they are also predicted to form…

To clarify the origin of a charge-density wave (CDW) phase in 1$T$-TiSe$_2$, we study the ground state property of a half-filled two-band Hubbard model in a triangular lattice including electron-phonon interaction. By using the variational…

强关联电子 · 物理学 2015-06-01 Hiroshi Watanabe , Kazuhiro Seki , Seiji Yunoki

Strong Coulomb interactions can drive electrons to crystallize into a Wigner lattice. Achieving the bosonic analogue - a crystal of excitons - has remained elusive due to their short lifetimes and weaker interactions. Here, we report the…

First-principles calculations reveal an unusual electronic state (dubbed as half excitonic insulator) in monolayer 1T-MX2 (M = Co, Ni and X = Cl, Br). Its one spin channel has a many-body ground state due to excitonic instability, while the…

材料科学 · 物理学 2019-06-19 Zeyu Jiang , Yuanchang Li , Wenhui Duan , Shengbai Zhang

Moir\'e superlattices of transition-metal dichalcogenide bilayers host strong Coulomb interactions residing in narrow electron bands, leading to correlated insulating states at fractional carrier doping densities, known as generalized…

Bose-Einstein condensation (BEC) is a quantum mechanical phenomenon directly linked to the quantum statistics of bosons. While cold atomic gases provide a new arena for exploring the nature of BEC, a long-term quest to confirm BEC of…

量子气体 · 物理学 2011-07-11 Kosuke Yoshioka , Eunmi Chae , Makoto Kuwata-Gonokami

Coulomb attraction between electrons and holes in a narrow-gap semiconductor or a semimetal is predicted to lead to an elusive phase of matter dubbed 'excitonic insulator'. However, direct observation of such electronic instability remains…

强关联电子 · 物理学 2021-08-09 Kwangrae Kim , Hoon Kim , Jonghwan Kim , Changil Kwon , Jun Sung Kim , B. J. Kim

Helium, the second most abundant element in the universe, exhibits an extremely large electronic band gap of about $20$ eV at low pressures ($\le 0.1$ GPa). While the metallization pressure of hcp helium has been accurately predicted, thus…

The opening of an energy gap in the electronic structure generally indicates the presence of interactions. In materials with low carrier density and short screening length, long-range Coulomb interaction favors the spontaneous formation of…

The excitonic insulator (EI) is a more than 60-year-old theoretical proposal that yet remains elusive. It is a purely quantum phenomenon involving the spontaneous generation of excitons in quantum mechanics and the spontaneous condensation…

材料科学 · 物理学 2025-11-03 H. W. Qu , H. T. Liu , Y. C. Li