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Dynamical properties of the lattice structure was studied by optical spectroscopy in ACr2O4 chromium spinel oxide magnetic semiconductors over a broad temperature region of T=10-335K. The systematic change of the A-site ions (A=Mn, Fe, Co,…

强关联电子 · 物理学 2013-07-24 V. Kocsis , S. Bordács , D. Varjas , K. Penc , A. Abouelsayed , C. A. Kuntscher , K. Ohgushi , Y. Tokura , I. Kézsmárki

Lattice and magnetic dynamics of NiWO$_4$ single crystals were studied with the use of polarized Raman spectroscopy in a wide temperature range of 10-300 K including the antiferromagnetic ordering temperature $T_N$=62 K. Static magnetic…

We present a Raman scattering study of Ca$_2$RuO$_4$, in which we investigate the temperature-dependence of the lattice dynamics and the electron-phonon interaction below the metal-insulator transition temperature ({\it T}$_{\rm MI}$).…

强关联电子 · 物理学 2009-11-11 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

Magnetic frustrations and degeneracies profoundly affect ground-state magnetic properties emerging from competing exchange interactions. Controlling such frustrations using orbital and phonon engineering via the Kugel-Khomskii-type…

A structural phase transition from cubic $Fd\bar{3}m$ to tetragonal $I$4$_1$/$amd$ symmetry with $c/a >$ 1 is observed at $T_{\rm{S}}$ = 16 K in spinel GeCo$_2$O$_4$ below the N\'eel temperature $T_N$ = 21 K. Structural and magnetic…

Quasi-2D van der Waals ferromagnet Fe$_4$GeTe$_2$, featuring the simultaneous presence of high Curie temperature ($T_\mathrm{C}$ $\sim 270$ K) and a spin-reorientation transition at $T_\mathrm{SR}$ $\sim 110$ K, is a rare system where…

Fe3GeTe2 has emerged as one of the most fascinating van der Waals crystals due to its two-dimensional (2D) itinerant ferromagnetism, topological nodal lines and Kondo lattice behavior. However, lattice dynamics, chirality of phonons and…

The lattice dynamics of the ferromagnetic spinel CuCr2Se4 (Tc = 430K) was studied experimentally by measuring the Raman spectra and theoretically by calculation of zone center phonon frequencies within a shell model. All Raman allowed modes…

材料科学 · 物理学 2015-05-19 V. G. Ivanov , M. N. Iliev , Y. -H. A. Wang , A. Gupta

Lattice and spin excitations have been studied by Raman scattering in hexagonal YbMnO3 single crystals. The temperature dependences of the phonon modes show that the E2 mode at 256 cm-1 related to the displacement of Mn and O ions in a-b…

强关联电子 · 物理学 2012-11-12 J. Liu , C. Toulouse , P. Rovillain , M. Cazayous , Y. Gallais , M. -A. Measson , S. W. Cheong , N. Lee , A. Sacuto

Reproducing the electronic structure of AM$_4$X$_8$ lacunar spinels with a breathing pyrochlore lattice is a great theoretical challenge due to the interplay of various factors. The character of the M$_4$X$_4$ cluster orbitals is critically…

强关联电子 · 物理学 2020-02-20 S. Reschke , F. Meggle , F. Mayr , V. Tsurkan , L. Prodan , H. Nakamura , J. Deisenhofer , C. A. Kuntscher , I. Kézsmárki

Frustrated magnetic systems exhibit highly degenerate ground states and strong fluctuations, often leading to new physics. An intriguing example of current interest is the antiferromagnet on a diamond lattice, realized physically in A-site…

We report a high-field electron spin resonance study in the sub-THz frequency domain of a single crystal of Sr$_2$IrO$_4$ that has been recently proposed as a prototypical spin-orbital Mott insulator. In the antiferromagnetically (AFM)…

强关联电子 · 物理学 2015-06-18 S. Bahr , A. Alfonsov , G. Jackeli , G. Khaliullin , A. Matsumoto , T. Takayama , H. Takagi , B. Büchner , V. Kataev

Linear and non-linear couplings of magnetic and lattice excitations are at the heart of many fascinating magnetophononic phenomena observed in rare-earth orthoferrites, the distinctive feature of which is the tendency to spin-reorientation…

We investigate the interplay between lattice symmetry, phonons, and magnetism in the quasi-one-dimensional ladder compound BaFe$_2$S$_3$ by combining polarized synchrotron infrared spectroscopy, hybrid-functional density functional theory…

Theoretical DFT calculations using GGA+U and HSE06 frameworks enabled vibrational mode assignment and partial (atomic) phonon DOS determination in KAgF3 perovskite, a low-dimensional magnetic fluoroargentate(II). Twelve bands in the spectra…

材料科学 · 物理学 2021-01-20 Kacper Koteras , Jakub Gawraczynski , Mariana Derzsi , Zoran Mazej , Wojciech Grochala

We report single-crystal neutron diffraction studies on a spinel antiferromagnet GeCo$_2$O$_4$, which exhibits magnetic order with a trigonal propagation vector and tetragonal lattice expansion ($c/a\simeq1.001$) below $T_{\rm N}=21$ K. For…

We report on x-ray diffraction, magnetic susceptibility, electron- spin resonance and heat- capacity studies of Co[Al_1-xCo_x]_2O_4 for Co concentrations 0<x<1. In this spinel system only the A-site Co^2+ cation is magnetic, while the…

材料科学 · 物理学 2009-11-13 N. Tristan , V. Zestrea , G. Behr , R. Klingeler , B. Buechner , H. A. Krug von Nidda , A. Loidl , V. Tsurkan

We report on the structural evolution, spin phonon interactions, and magnetoelastic effects in bulk LaFeO3 perovskite across its antiferromagnetic transition. We found that while the lattice constants exhibit slight deviations at the Neel…

The low temperature lattice structure and magnetic properties of Co$_{2.75}$Fe$_{0.25}$O$_4$ ferrite have been investigated using experimental results from synchrotron x-ray diffraction (SXRD), dc magnetization, ac susceptibility, neutron…

强关联电子 · 物理学 2020-07-09 R. N. Bhowmik , Amit Kumar , A. K. Sinha , S. M. Yusuf

We demonstrate that the onset of complex spin orders in ACr$_2$O$_4$ spinels with magnetic A$=$Co, Fe and Cu ions lowers the lattice symmetry. This is clearly indicated by the emergence of anisotropic lattice dynamics -- as evidenced by the…

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